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Validity of the semiquantum approximation in the ultrastrong coupling regime of cavity QED

Tuomas Jaako

Published Jan 1, 2015• 0 citations
OpenAlex

Abstract

With the recent advancements made in the coupling of quantum systems, reaching the (ultra)strong coupling regime, where the coupling constant exceeds the dissipation rate and approaches the frequencies of the coupled systems, is getting closer. In this regime, the much used semiclassical model is no longer valid, and the solving of the full quantum master equation can be computationally too demanding. Thus, we must develop a new approach to be able to simulate the system. One solution is to use the semiquantum approximation. In this thesis, we present a systematic way of employing the semiquantum approximation and compare it to the full master equation. Our aim is to determine the range for the coupling strength where the semiquantum model is applicable. We chose to do the comparison of the semiquantum approximation and the master equation within the Rabi model, which can be used to describe e.g. the interaction of light and matter. The Rabi model describes a system with a coupled two-level system and a harmonic oscillator. It was chosen because its behaviour is reasonably well known. We compared the semiquantum approximation to the quantum master equation in two cases. First we studied the steady state results from the two models, and then moved on to the spectral properties. The results show that the steady state and the spectrum obtained from the semiquantum model agree with the ones obtained by using the master equation, until the coupling reaches a considerable fraction of the resonant frequency of the oscillator, while still exceeding the experimentally reasonable dissipation rate by an order of magnitude. In the future, one could use the semiquantum approximation in the eld of cavity optomechanics. There a mechanical oscillator is coupled to optical radiation con ned in a cavity, e.g. a Fabry-Perot cavity. Especially in optomechanics, the solving of the master equation can turn out to be a formidable task, and by using the semiquantum approximation one could reduce the computation time considerably.

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•Jan 1, 2010•0 citations
With the recent advancements made in the coupling of quantum systems, reaching the (ultra)strong coupling regime, where the coupling constant exceeds the dissipation rate and approaches the frequencies of the coupled systems, is getting closer. In this regime, the much used semiclassical model is no longer valid, and the solving of the full quantum master equation can be computationally too demanding. Thus, we must develop a new approach to be able to simulate the system. One solution is to use the semiquantum approximation. In this thesis, we present a systematic way of employing the semiquantum approximation and compare it to the full master equation. Our aim is to determine the range for the coupling strength where the semiquantum model is applicable. We chose to do the comparison of the semiquantum approximation and the master equation within the Rabi model, which can be used to describe e.g. the interaction of light and matter. The Rabi model describes a system with a coupled two-level system and a harmonic oscillator. It was chosen because its behaviour is reasonably well known. We compared the semiquantum approximation to the quantum master equation in two cases. First we studied the steady state results from the two models, and then moved on to the spectral properties. The results show that the steady state and the spectrum obtained from the semiquantum model agree with the ones obtained by using the master equation, until the coupling reaches a considerable fraction of the resonant frequency of the oscillator, while still exceeding the experimentally reasonable dissipation rate by an order of magnitude. In the future, one could use the semiquantum approximation in the eld of cavity optomechanics. There a mechanical oscillator is coupled to optical radiation con ned in a cavity, e.g. a Fabry-Perot cavity. Especially in optomechanics, the solving of the master equation can turn out to be a formidable task, and by using the semiquantum approximation one could reduce the computation time considerably.
The prototypical system constituted by a two-level atom interacting with a quantized single-mode electromagnetic field is described by the quantum Rabi model (QRM). The QRM is potentially valid at any light-matter interaction regime, ranging from the weak (where the decay rates exceeds the coupling rate) to the deep strong coupling (where the interaction rate exceeds the bare transition frequencies of the subsystems). However, when reaching the ultrastrong coupling regime, several theoretical issues may prevent the correct description of the observable dynamics of such a system: (i) the standard quantum optics master equation fails to correctly describe the interaction of this system with the reservoirs; (ii) the correct output photon rate is no longer proportional to the intracavity photon number; and (iii) they appear to violate gauge invariance. Here, we study the photon flux emission rate of this system under the incoherent excitation of the two-level atom for any light-matter interaction strength and consider different effective temperatures. The dependence of the emission spectra on the coupling strength is the result of the interplay between energy levels, matrix elements of the observables, and the density of states of the reservoirs. Within this approach, we also study the occurrence of light-matter decoupling in the deep strong-coupling regime and show how all of the obtained results are gauge invariant.
The interaction among the components of a hybrid quantum system is often neglected when considering the coupling of these components to an environment. However, if the interaction strength is large, this approximation leads to unphysical predictions, as has been shown for cavity-QED and optomechanical systems in the ultrastrong-coupling regime. To deal with these cases, master equations with dissipators retaining the interaction between these components have been derived for the quantum Rabi model and for the standard optomechanical Hamiltonian. In this article, we go beyond these previous derivations and present a general master equation approach for arbitrary hybrid quantum systems interacting with thermal reservoirs. Specifically, our approach can be applied to describe the dynamics of open hybrid systems with harmonic, quasiharmonic, and anharmonic transitions. We apply our approach to study the influence of temperature on multiphoton vacuum Rabi oscillations in circuit QED. We also analyze the influence of temperature on the conversion of mechanical energy into photon pairs in an optomechanical system, which has been recently described at zero temperature. We compare our results with previous approaches, finding that these sometimes overestimate decoherence rates and underestimate excited-state populations.
Environmental influences on the dynamics of a coupled qubit-oscillator system are studied analytically in a regime where deviations from the exactly solvable Jaynes–Cummings model are important. We investigate the case of a quasi-degenerate qubit within the ultra-strong coupling regime for which the qubit frequency is much smaller than the frequency of the oscillator, and the coupling between the qubit and the oscillator is large, both of which invalidate the usually employed rotating wave approximation. In contrast to the standard quantum optics master equation, we explicitly take the qubit-oscillator coupling into account while microscopically deriving a dressed state master equation. Using the derived master equation, we discuss a spectroscopic technique which can be used to probe the dressed energy-level structure of the qubit-oscillator system.
Cavity and circuit QED study light-matter interaction at its most fundamental level. Yet, this interaction is most often neglected when considering the coupling of this system with an environment. In this paper, we show how this simplification, which leads to the standard quantum optics master equation, is at the root of unphysical effects. Including qubit relaxation and dephasing, and cavity relaxation, we derive a master equation that takes into account the qubit-resonator coupling. Special attention is given to the ultrastrong coupling regime, where the failure of the quantum optical master equation is manifest. In this situation, our model predicts an asymmetry in the vacuum Rabi splitting that could be used to probe dephasing noise at unexplored frequencies. We also show how fluctuations in the qubit frequency can cause sideband transitions, squeezing, and Casimir-like photon generation.
Phenomenological approaches to photon loss have long been the workhorse of cavity-QED, but prove inadequate in the presence of sufficiently broadband light-matter interactions. We present a rigorous and ab initio derivation of a quantum master equation for a quantized optical cavity mode coupled to a dipole, using a quasinormal mode (QNM) quantization procedure for plasmonic and dielectric open-system cavity-QED, which is valid in broadband light-matter interaction regimes, including ultrastrong coupling (USC). The theory supports general three-dimensional resonators with arbitrary dispersion and loss, and thus can be applied to a wide range of realistic open cavities. Our ab initio and gauge-invariant approach fully recovers a recent result for the spectral density of a quantized cavity with a single dipole and reveals important departures from previous heuristic assumptions about system-reservoir coupling. We identify a new criterion for what we term the "broadband dissipative" regime of cavity-QED, where phenomenological models require corrections in accordance with the intrinsic and spatially-dependent complex phase of the QNM, and also shed light on fundamental limits to single-mode models in extreme coupling regimes. Using experimentally motivated plasmonic and dielectric cavity examples, we show validity ranges of our QNM master equation and spectral USC calculations, and discuss prospects for near-term experimental observation of the broadband dissipative effects.
The model of a two-level system (TLS) coupled to a harmonic oscillator has found a widespread application in physics and chemistry. In this thesis we focus on the field of circuit quantum electrodynamics where the TLS stands for a quantum bit (qubit), which is the basic building unit of a potential quantum computer, and the oscillator represents a transmission-line resonator, which can be used, e.g., to store information contained on the qubit or for communication between several qubits. Furthermore, the oscillator can model a superconducting quantum interference device (SQUID) determining the state of the qubit. In first experimental realizations the coupling between the qubit and the oscillator was small compared to characteristic frequencies of the two devices. In such a situation the Jaynes-Cummings model provides a realistic and completely analytical description of the energy spectrum and the dynamics of the setup. However, it relies on a rotating-wave approximation (RWA) which neglects counter-rotating terms in the full qubit-oscillator Hamiltonian. These counter-rotating terms become important under increase of the coupling strength, as it has been achieved in recent experiments. We present two analytical approaches to take these additional contributions into account: The first one treats the qubit-oscillator Hamiltonian perturbatively in the coupling strength and predicts a frequency shift in its energy spectrum, the Bloch-Siegert shift. The second one considers the qubit's tunneling splitting as small parameter and thus treats the problem to all orders in the coupling allowing to enter the ultrastrong coupling regime, where the coupling strength becomes comparable to the qubit's and/or oscillator's frequency. For both cases we give a thorough analysis of the qubit's dynamics. In order to perform operations the qubit is usually probed by an external driving force. We model this situation by coupling the TLS to a classical oscillator and examine the resulting time dependent Hamiltonian using a combination of Floquet theory and Van Vleck perturbation theory. Thus, we provide an analysis of the qubit's energy spectrum and dynamics which is nonperturbative in the driving amplitude. We investigate effects like coherent destruction of tunneling and driving-inducing tunneling oscillations. By coupling the driven TLS to a quantized oscillator we give for the first time an analytical treatment of the qubit-oscillator system being simultaneously exposed to both ultrastrong coupling and extreme driving. We observe interesting phenomena in the dynamics like the suppression of specific frequencies under a variation of the coupling strength. To mimic environmental influences on the qubit we apply the Caldeira-Leggett master equation approach to the driven TLS and to the qubit-oscillator system and provide for both cases analytical expressions for the relaxation and dephasing rates.