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Plasma Science and Technology

Long Lifetime Ultracold Plasma a Supersoduc Nitric Oxide Produced by a Nanosecond Laser in Molecular Beam Environment

刘金波, 陆荣华, 郭丽, 金玉奇, 郭敬为

Published Jan 1, 2014• 0 citations
OpenAlex

Abstract

Ultracold plasma provides a possible route to approach the strongly-coupled regime under laboratory conditions.Normally,the lifetime of ultracold plasma is very limited due to plasma heating and expansion mechanisms.We present a new method to generate long lifetime ultracold plasmas consisting mainly of cations and anions.This plasma demonstrates a capability of traversing a DC barrier of up to 5(or-3) V.The lifetime of this plasma is expected to be more than 250 μs.Finally,molecular dynamics(MD) simulation is used to explain how anions slow the expansion rate and prolong the lifetime of this plasma.

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Ultracold molecular plasmas represent a new frontier of plasma physics. They offer an easy and accessible laboratory for the study of strongly coupled Coulomb systems. Strong Coulomb coupling can give rise to exotic materials such as Wigner crystals and liquid like plasmas. In this thesis, I present a set of experiments and theoretical models that explore the properties of ultracold plasma in great detail. A supersonic beam of nitric oxide in helium creates a cold ensemble of ground state molecules. Upon two-color excitation, a Rydberg gas of nitric oxide evolves on a time scale of nanoseconds to form an ultracold plasma. The excited volume is imaged using a multichannel plate detector mounted on a movable grid. By moving the detector back and forth, we can observe the expansion dynamics of the plasma and its decay. Selective field ionization captures the relaxation of the Rydberg states to a plasma. We use a very reliable coupled-rate-equation model to understand the decay dynamics and evolution of Rydberg gas to a plasma by accounting for all the major processes that happen during the avalanche process. We find that a plasma evolved from an ultracold Rydberg gas expands very slowly, exhibits long relaxation time, and shows evidence suggesting the development of spatial order.

•Jan 1, 2016•0 citations

Ultracold Neutral Plasma Produced by One-Color Two-Photon Ionization in Supersonic Nitric Oxide Molecular Beam

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Abstract Not long after metastable xenon was photoionized in a magneto-optical trap, groups in Europe and North America found that similar states of ionized gas evolved spontaneously from state-selected, high principal quantum number Rydberg gases. Studies of atomic xenon and molecular nitric oxide entrained in a supersonically cooled molecular beam subsequently showed much the same final state evolved from a sequence of prompt Penning ionization and electron-impact avalanche to plasma, well-described by coupled rate-equation simulations. But, measured over longer times, the molecular ultracold plasma was found to exhibit an anomalous combination of very long lifetime and very low apparent electron temperature. This review first summarizes early developments in the general study of ultracold plasmas formed by atomic and molecular Rydberg gases, and then turns to describe the particular properties of the nitric oxide molecular ultracold plasma that appear to call for an explanation beyond the realm of conventional plasma physics.

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Ultracold nitric oxide molecular plasma : characteristic response to time-varying electric fields

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Not long after metastable xenon was photoionized in a magneto-optical trap, groups in Europe and North America found that similar states of ionized gas evolved spontaneously from state-selected Rydberg gases of high principal quantum number. Studies of atomic xenon and molecular nitric oxide entrained in a supersonically cooled molecular beam subsequently showed much the same final state evolved from a sequence of prompt Penning ionization and electron impact avalanche to plasma, well-described by coupled rate-equation simulations. However, measured over longer times, the molecular ultracold plasma (UCP) was found to exhibit an anomalous combination of very long lifetime and very low apparent electron temperature. In this thesis I summarize early developments in the study of UCP formed by atomic and molecular Rydberg gases, and then I detail observations as they combine to characterize properties of the nitric oxide molecular UCP that appear to call for an explanation beyond the realm of conventional plasma physics. I also explain how I leveraged a radio frequency electric field to understand the causes of classically-unexplainable behavior of our molecular system.

•Jan 1, 2021•0 citations

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Ultracold neutral plasmas (UNPs) are highly correlated, charged-particle systems studied in standard atomic-molecular optical physics laboratories. Advances in ultracold physics techniques have led to the development of magneto-optical traps that permit the localization of micro-Kelvin temperature atomic samples (10⁸ - 10¹⁰ cm -³ that can be photoionized with a defined excess laser energy. Magneto-optical trapping of molecules proves difficult, and to date, lags in reaching conditions attainable for atoms. Molecules possess additional degrees of freedom where energy can flow during laser trapping and cooling. Alternatively, elastic collisions with inert gases offer another route to low temperatures. Super-sonic expansions of target molecules seeded in a noble gas can reduced the translational temperature to values as low as 0.1 K. Here I report on the formation of a molecular ultracold plasma in a molecular beam of nitric oxide seeded in an inert gas. Our method does not directly form a plasma, but instead, I create a Rydberg gas that spontaneously evolves to a plasma. I have verified the transition to a collective plasma state by applying pulsed-fields to the field-free flight region, and observe a signal that persists well beyond classical field amplitudes required to ionize individual Rydberg states. Electric field screening is a collective effect occurring over a characteristic distance, quantified by the Debye length, λ_D. Molecular ultracold plasmas described here exhibit Debye lengths smaller than the overall size, λ_D<<σ. Plasmas of this nature offer an exotic environment for which to study fundamental phenomena. While plasmas are generally thought of as hot, UNPs exist at low enough temperatures that electrostatic interaction energy between particles is greater than their kinetic energy. At this point, charged particles begin to find themselves in local potential energy minima. Over the entire sample this translates to long-range order, or correlation. It is of great interest for researchers studying UNPs to maximize particle correlation, which requires UNPs to remain very cold, and dense through their lifetime.

•Jan 1, 2013•0 citations

Very slow expansion of an ultracold plasma formed in a seeded supersonic molecular beam of NO

J. P. Morrison, Chris Rennick, Edward R. Grant

The double-resonant laser excitation of nitric oxide, cooled to 1 K in a seeded supersonic molecular beam, yields a gas of $\ensuremath{\approx}{10}^{12}$ molecules per cubic centimeter in a single selected Rydberg state. This population evolves to produce prompt free electrons, and a durable cold plasma of electrons and intact ${\text{NO}}^{+}$ ions. This plasma travels with the molecular beam through a field-free region to encounter a grid. The atomic weight of the expansion gas controls the beam velocity and hence the flight time from the interaction region to the grid. Monitoring electron production as the plasma traverses this grid measures its longitudinal width as a function of flight time. Comparing these widths to the width of the laser beam that defines the initial size of the illuminated volume allows us to gauge the rate of expansion of the plasma. We find that the plasma created from the evolution of a Rydberg gas of NO expands at a small but measurable rate, and that this rate of expansion accords with the Vlasov equations for an initial electron temperature of ${T}_{e}\ensuremath{\approx}7\text{ }\text{K}$.

arXiv:0812.4051•Physical Review A•Jun 9, 2009•29 citations
Ultracold plasma provides a possible route to approach the strongly-coupled regime under laboratory conditions.Normally,the lifetime of ultracold plasma is very limited due to plasma heating and expansion mechanisms.We present a new method to generate long lifetime ultracold plasmas consisting mainly of cations and anions.This plasma demonstrates a capability of traversing a DC barrier of up to 5(or-3) V.The lifetime of this plasma is expected to be more than 250 μs.Finally,molecular dynamics(MD) simulation is used to explain how anions slow the expansion rate and prolong the lifetime of this plasma.
Ultracold molecular plasmas represent a new frontier of plasma physics. They offer an easy and accessible laboratory for the study of strongly coupled Coulomb systems. Strong Coulomb coupling can give rise to exotic materials such as Wigner crystals and liquid like plasmas. In this thesis, I present a set of experiments and theoretical models that explore the properties of ultracold plasma in great detail. A supersonic beam of nitric oxide in helium creates a cold ensemble of ground state molecules. Upon two-color excitation, a Rydberg gas of nitric oxide evolves on a time scale of nanoseconds to form an ultracold plasma. The excited volume is imaged using a multichannel plate detector mounted on a movable grid. By moving the detector back and forth, we can observe the expansion dynamics of the plasma and its decay. Selective field ionization captures the relaxation of the Rydberg states to a plasma. We use a very reliable coupled-rate-equation model to understand the decay dynamics and evolution of Rydberg gas to a plasma by accounting for all the major processes that happen during the avalanche process. We find that a plasma evolved from an ultracold Rydberg gas expands very slowly, exhibits long relaxation time, and shows evidence suggesting the development of spatial order.
Nitric oxide (NO) is cooled to 1 K in a seeded Ar supersonic molecular beam. NO molecules are ionized by one-color two-photon resonant enhanced multiphoton ionization (REMPI) process to form an ultracold plasma. The density of the ionized molecules in the illuminated volume approaches to 1.5 × 10 13 cm −3 . Prompt electrons, plasma electrons and intact NO + ions are produced during this process. Experimental results confirm that the lifetime of this ultracold plasma is longer than 18.3 μs. This is the first report of NO ultracold plasma with significant lifetime produced by one-color two-photon REMPI process.
Abstract Not long after metastable xenon was photoionized in a magneto-optical trap, groups in Europe and North America found that similar states of ionized gas evolved spontaneously from state-selected, high principal quantum number Rydberg gases. Studies of atomic xenon and molecular nitric oxide entrained in a supersonically cooled molecular beam subsequently showed much the same final state evolved from a sequence of prompt Penning ionization and electron-impact avalanche to plasma, well-described by coupled rate-equation simulations. But, measured over longer times, the molecular ultracold plasma was found to exhibit an anomalous combination of very long lifetime and very low apparent electron temperature. This review first summarizes early developments in the general study of ultracold plasmas formed by atomic and molecular Rydberg gases, and then turns to describe the particular properties of the nitric oxide molecular ultracold plasma that appear to call for an explanation beyond the realm of conventional plasma physics.
Not long after metastable xenon was photoionized in a magneto-optical trap, groups in Europe and North America found that similar states of ionized gas evolved spontaneously from state-selected Rydberg gases of high principal quantum number. Studies of atomic xenon and molecular nitric oxide entrained in a supersonically cooled molecular beam subsequently showed much the same final state evolved from a sequence of prompt Penning ionization and electron impact avalanche to plasma, well-described by coupled rate-equation simulations. However, measured over longer times, the molecular ultracold plasma (UCP) was found to exhibit an anomalous combination of very long lifetime and very low apparent electron temperature. In this thesis I summarize early developments in the study of UCP formed by atomic and molecular Rydberg gases, and then I detail observations as they combine to characterize properties of the nitric oxide molecular UCP that appear to call for an explanation beyond the realm of conventional plasma physics. I also explain how I leveraged a radio frequency electric field to understand the causes of classically-unexplainable behavior of our molecular system.
Ultracold neutral plasmas (UNPs) are highly correlated, charged-particle systems studied in standard atomic-molecular optical physics laboratories. Advances in ultracold physics techniques have led to the development of magneto-optical traps that permit the localization of micro-Kelvin temperature atomic samples (10⁸ - 10¹⁰ cm -³ that can be photoionized with a defined excess laser energy. Magneto-optical trapping of molecules proves difficult, and to date, lags in reaching conditions attainable for atoms. Molecules possess additional degrees of freedom where energy can flow during laser trapping and cooling. Alternatively, elastic collisions with inert gases offer another route to low temperatures. Super-sonic expansions of target molecules seeded in a noble gas can reduced the translational temperature to values as low as 0.1 K. Here I report on the formation of a molecular ultracold plasma in a molecular beam of nitric oxide seeded in an inert gas. Our method does not directly form a plasma, but instead, I create a Rydberg gas that spontaneously evolves to a plasma. I have verified the transition to a collective plasma state by applying pulsed-fields to the field-free flight region, and observe a signal that persists well beyond classical field amplitudes required to ionize individual Rydberg states. Electric field screening is a collective effect occurring over a characteristic distance, quantified by the Debye length, λ_D. Molecular ultracold plasmas described here exhibit Debye lengths smaller than the overall size, λ_D<<σ. Plasmas of this nature offer an exotic environment for which to study fundamental phenomena. While plasmas are generally thought of as hot, UNPs exist at low enough temperatures that electrostatic interaction energy between particles is greater than their kinetic energy. At this point, charged particles begin to find themselves in local potential energy minima. Over the entire sample this translates to long-range order, or correlation. It is of great interest for researchers studying UNPs to maximize particle correlation, which requires UNPs to remain very cold, and dense through their lifetime.
The double-resonant laser excitation of nitric oxide, cooled to 1 K in a seeded supersonic molecular beam, yields a gas of $\ensuremath{\approx}{10}^{12}$ molecules per cubic centimeter in a single selected Rydberg state. This population evolves to produce prompt free electrons, and a durable cold plasma of electrons and intact NO+{\text{NO}}^{+}NO+ ions. This plasma travels with the molecular beam through a field-free region to encounter a grid. The atomic weight of the expansion gas controls the beam velocity and hence the flight time from the interaction region to the grid. Monitoring electron production as the plasma traverses this grid measures its longitudinal width as a function of flight time. Comparing these widths to the width of the laser beam that defines the initial size of the illuminated volume allows us to gauge the rate of expansion of the plasma. We find that the plasma created from the evolution of a Rydberg gas of NO expands at a small but measurable rate, and that this rate of expansion accords with the Vlasov equations for an initial electron temperature of ${T}_{e}\ensuremath{\approx}7\text{ }\text{K}$.