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Proceedings of SPIE, the International Society for Optical Engineering/Proceedings of SPIE

Diamond-based field sensor for nEDM experiment

Sarvagya Sharma, Chris Hovde, BECK Douglas howard

Published Feb 13, 2016• 2 citations
Publisher

Abstract

Ensembles of negatively charged nitrogen vacancy centers in diamonds are investigated as optical sensors for electric and magnetic fields in the interaction region of a neutron electric dipole moment experiment. As a first step towards measuring electric fields, the Stark shift is investigated in the ground electronic state, using optically detected magnetic resonance (ODMR) to measure hyperfine-resolved fine structure transitions. One detection approach is to modulate the electric field and demodulate the ODMR signal at the modulation frequency or its harmonic. Models indicate that the ratio of the amplitudes of these signals provides information about the magnitude of the electric field. Experiments show line shapes consistent with the models. Methods are considered for extending this technique to all-optical measurement of fields. Additionally, progress is reported towards an all-optical, fiberized sensor based on electromagnetically-induced transparency (EIT), which may be suitable for measuring magnetic fields. The design uses total internal reflection to provide a long optical path through the diamond for both the 637 nm EIT laser and a green repump laser.

DOI
10.1117/12.2211910

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quant-pharXiv:2606.02749•Jun 3, 2026
Ensembles of negatively charged nitrogen vacancy centers in diamonds are investigated as optical sensors for electric and magnetic fields in the interaction region of a neutron electric dipole moment experiment. As a first step towards measuring electric fields, the Stark shift is investigated in the ground electronic state, using optically detected magnetic resonance (ODMR) to measure hyperfine-resolved fine structure transitions. One detection approach is to modulate the electric field and demodulate the ODMR signal at the modulation frequency or its harmonic. Models indicate that the ratio of the amplitudes of these signals provides information about the magnitude of the electric field. Experiments show line shapes consistent with the models. Methods are considered for extending this technique to all-optical measurement of fields. Additionally, progress is reported towards an all-optical, fiberized sensor based on electromagnetically-induced transparency (EIT), which may be suitable for measuring magnetic fields. The design uses total internal reflection to provide a long optical path through the diamond for both the 637 nm EIT laser and a green repump laser.
We report measurements of optically detected magnetic resonance spectra of ensembles of nitrogen-vacancy (NV-) centers in diamonds in the presence of electromagnetic fields. To reduce inhomogeneous broadening, the spectra are acquired from a region of 20 cubic microns in a CVD(Chemical Vapor Deposition) diamond through a confocal microscope. The Stark shift from transverse electric fields is enhanced at avoided crossings between the hyperfine levels that arise from interaction with 14N(I = 1) nuclei in the diamond lattice. As expected from previous reports, the Stark shift of the spectral lines is stronger when there is no magnetic field along the NV axis. The shift is also strong, but for different transitions, at a field of about 100 uT.
We report measurements of optically detected magnetic resonance spectra of ensembles of negatively charged nitrogen-vacancy (NV) centers in diamonds in the presence of strain and DC external electric fields. The Stark shift of the spectral lines is stronger when the axial magnetic field along the NV centers quantization axis is minimized. The shift is also enhanced at avoided crossings between the hyperfine levels at an axial field of 77 uT. Since the intrinsic strain in the diamond also induces a Stark shift, we are able to calculate the magnitude and direction of the strain within the crystal. We also use the Stark effect to map the electric field in the diamond volume between patterned electrodes.
Diamond nitrogen-vacancy (NV) centers are widely studied for quantum sensing in multiple physical fields due to their long coherence time and room-temperature optical readout. However, accurately decoupling and extracting signals for individual fields from fluorescence remains a major challenge. In this work, by establishing the spatial configuration between the four axes of the NV center and the directions of the externally applied electric and magnetic fields, the resonance frequency shifts of two pairs in the ODMR spectrum are exclusively induced by the electric field, whereas those of the other two pairs are exclusively induced by the magnetic field. Consequently, effective decoupling and readout of the electric field signal are realized. The experiments measure electric fields from 0 to 20 kV/cm in the diamond sample, revealing a linear relationship between the resonance frequency shift and the applied electric field, with coefficients 0.1713MHz/(kV/cm) and 0.1660MHz/(kV/cm) matching the NV center’s linear Stark effect, laying the foundation for subsequent research on electric field measurement.
Precision measurements of electric current flow in motors and power converters is indispensable for efficient digital control by monitoring their energy use. Nitrogen-vacancy (NV) centers in a crystalline diamond are promising candidates for sensitive magnetometry and electric current measurements. In a diamond quantum sensor with NV centers, the Zeeman splitting of the electron spin state of the NV center can be utilized to detect magnetic field. This is because the splitting of the spectral line is proportional to the external magnetic field strength, and the arbitrary constant of the gyromagnetic ratio is independent of both frequency and magnetic field. Then, the Zeeman splitting can be measured with optically detected magnetic resonance (ODMR) spectroscopy.
We use electromagnetically induced transparency (EIT) to probe the narrow electron-spin resonance of nitrogen-vacancy centers in diamond. Working with a multipass diamond chip at temperatures 6--30 K, the zero-phonon absorption line (637 nm) exhibits an optical depth of 6 and inhomogeneous linewidth of $\ensuremath{\sim}30\text{ }\text{ }\mathrm{GHz}$ FWHM. Simultaneous optical excitation at two frequencies separated by the ground-state zero-field splitting (2.88 GHz) reveals EIT resonances with a contrast exceeding 6% and FWHM down to 0.4 MHz. The resonances provide an all-optical probe of external electric and magnetic fields with a projected photon-shot-noise-limited sensitivity of 0.2  V/cm/Hz0.2\text{ }\text{ }\mathrm{V}/\mathrm{cm}/\sqrt{\mathrm{Hz}}0.2  V/cm/Hz​ and 0.1  nT/Hz0.1\text{ }\text{ }\mathrm{nT}/\sqrt{\mathrm{Hz}}0.1  nT/Hz​, respectively. Operation of a prototype diamond-EIT magnetometer measures a noise floor of $\ensuremath{\lesssim}1\text{ }\text{ }\mathrm{nT}/\sqrt{\mathrm{Hz}}$ for frequencies above 10 Hz and Allan deviation of $1.3\ifmmode\pm\else\textpm\fi{}1.1\text{ }\text{ }\mathrm{nT}$ for 100 s intervals. The results demonstrate the potential of diamond-EIT devices for applications ranging from quantum-optical memory to precision measurement and tests of fundamental physics.
We present a novel method for full vector magnetometry using nitrogen-vacancy (NV) centers. In contrast to conventional optically detected magnetic resonance techniques, our method employs two distinct broadband microwave pulses and measures them after transmission through the NV sensor medium, thus capturing the line splitting of the ground state triplet due to the Zeeman effect. Two orthogonally polarized microwave pulses allow resolving all magnetic field components independently by reading out differently oriented NV centers. Simulated data is analyzed using deep neural networks, whose efficacy we expect to translate very well to experiments. Our method yields sensitivities between 5 pT/Hz5~\mathrm{pT}/\sqrt{\mathrm{Hz}}5 pT/Hz​ and 100 pT/Hz100~\mathrm{pT}/\sqrt{\mathrm{Hz}}100 pT/Hz​ across different magnetic field vector components, while achieving approximately nT\mathrm{nT}nT accuracy at a signal-to-noise (SNR) ratio of 70 dB70~\mathrm{dB}70 dB. By being capable of accurately measuring magnetic fields down to 25 μT25~\mathrm{μT}25 μT, the need for a bias field beyond Earth's magnetic field is eliminated.