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Bulletin of the American Physical Society

Preserving electron spin coherence in solids by optimal dynamical decoupling

Jiangfeng Du

Published Mar 25, 2011• 0 citations
OpenAlex

Abstract

Quantum computing: cutting out the noise If electron spins in solid materials are to be exploited in quantum computers, there is a need to minimize the quantum 'noise' that inevitably accompanies the interaction of the spins with their environment. Experiments in single crystals of malonic acid undergoing pulsed electron paramagnetic resonance now show how this can be achieved. The use of external pulses to induce the electron spins to 'flip' an optimal number of times causes their noisy interaction with the environment to be averaged towards zero, and the timescale over which spin coherence is maintained is markedly increased — from 0.04 to 30 microseconds in the system studied.

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Quantum computing: cutting out the noise If electron spins in solid materials are to be exploited in quantum computers, there is a need to minimize the quantum 'noise' that inevitably accompanies the interaction of the spins with their environment. Experiments in single crystals of malonic acid undergoing pulsed electron paramagnetic resonance now show how this can be achieved. The use of external pulses to induce the electron spins to 'flip' an optimal number of times causes their noisy interaction with the environment to be averaged towards zero, and the timescale over which spin coherence is maintained is markedly increased — from 0.04 to 30 microseconds in the system studied.
In quantum information processing, it is vital to protect the coherence of qubits in noisy environments. Dynamical decoupling (DD), which applies a sequence of flips on qubits and averages the qubit-environment coupling to zero, is a promising strategy compatible with other desired functionalities, such as quantum gates. Here, we review the recent progresses in theories of dynamical decoupling and experimental demonstrations. We give both semiclassical and quantum descriptions of the qubit decoherence due to coupling to noisy environments. Based on the quantum picture, a geometrical interpretation of DD is presented. The periodic Carr-Purcell-Meiboom-Gill DD and the concatenated DD are reviewed, followed by a detailed exploration of the recently developed Uhrig DD, which employs the least number of pulses in an unequally spaced sequence to suppress the qubit-environment coupling to a given order of the evolution time. Some new developments and perspectives are also discussed.
Quantum computing set a goal to harness the quantum laws of physics and create \ncomputers more powerful than ever imagined. Different technologies can be chosen to implement quantum bits (qubits), each with their advantages and drawbacks. The idea of combining different technologies then seems natural in order to come up with an optimal quantum computer. \n \nIn this sense, Nuclear Magnetic Resonance (NMR) and Electron Spin Resonance (ESR) seem to be the perfect marriage. Indeed, while electron spins can perform quantum gates within nanoseconds, they have to fight very fast decoherence phenomena, the nuclear spins, on the other hand, require longer electromagnetic pulses to be rotated but can be controlled longer without loss of quantum information. Using electron spins as actuators and nuclear spins as memory then appears as the optimal use of this hybrid system. Another fact accounting for this association is that the control of the system through the electron spin requires techniques very similar to the well-known NMR ones. \n \nThis work focuses on characterizing as precisely as possible the Hamiltonian of a hybrid spin system in a solid-state single crystal, especially the electron-nuclear interactions, to perform high-fidelity control in a home-built pulsed ESR spectrometer. Using this knowledge, we show that we can choose the orientation of the magnetic field with respect to our crystal to obtain optimal experimental conditions. Indeed, with a good knowledge of the Hamiltonian of the system, we want demonstrate high-fidelity quantum control. \n \nThe final aim of this work is to dynamically supply highly polarized ancilla qubits that can be used in a Quantum Error Correction (QEC) experiment by implementing heat bath algorithmic cooling using a cold electron spin bath. This is an important step towards demonstrating the viability of spin systems for building quantum computers.
Spin qubit coherence is a fundamental resource for the realization of quantum technologies. For solid-state platforms, spin decoherence is dominated by the magneto-active environment in the lattice, limiting their applicability. While standard dynamical decoupling techniques, such as the Hahn echo, extend central spin coherence, they fail to suppress the fast noise arising from strong dipolar interactions within the bath. Here, we present a decoupling mechanism, Hybrid-LG, that suppresses intra-bath dipolar interactions -- thus, fast noise acting on spin qubits- and demonstrate its effectiveness in extending spin coherence through efficient in-house CCE simulations. Specifically, we investigate one of the most widely exploited solid-state quantum platforms: an ensemble of nitrogen-vacancy (NV) centers in diamond coupled to a large and dense bath of substitutional nitrogen paramagnetic impurities (P1 centers). Our results reveal at least a twofold enhancement in NV coherence time relative to standard techniques including P1 center driving, without requiring additional control power.
Realistic quantum computing is subject to noise. Therefore, an important frontier in quantum computing is to implement noise-resilient quantum control over qubits. At the same time, dynamical decoupling can protect the coherence of qubits. Here we demonstrate non-trivial quantum evolution steered by dynamical decoupling control, which simultaneously suppresses noise effects. We design and implement a self-protected controlled-NOT gate on the electron spin of a nitrogen-vacancy centre and a nearby carbon-13 nuclear spin in diamond at room temperature, by employing an engineered dynamical decoupling control on the electron spin. Final state fidelity of 0.91(1) is observed in preparation of a Bell state using the gate. At the same time, the qubit coherence time is elongated at least 30 fold. The design scheme does not require the dynamical decoupling control to commute with the qubit interaction and therefore works for general qubit systems. This work marks a step towards implementing realistic quantum computing systems. Realistic quantum computers require a high degree of qubit control and must also be resilient to noise. Using dynamical decoupling control techniques, Liuet al.implement a self-protected controlled-NOT gate for electron and nuclear spins that retains a high final state fidelity.
The coherence time of an electron spin decohered by the nuclear spin environment in a quantum dot can be substantially increased by subjecting the electron to suitable dynamical decoupling sequences. We analyze the performance of high-level decoupling protocols by using a combination of analytical and exact numerical methods, and by paying special attention to the regimes of large interpulse delays and long-time dynamics, which are outside the reach of standard average Hamiltonian theory descriptions. We demonstrate that dynamical decoupling can remain efficient far beyond its formal domain of applicability, and find that a protocol exploiting concatenated design provides best performance for this system in the relevant parameter range. In situations where the initial electron state is known, protocols able to completely freeze decoherence at long times are constructed and characterized. The impact of system and control nonidealities is also assessed, including the effect of intrabath dipolar interaction, magnetic field bias and bath polarization, as well as systematic pulse imperfections. While small bias field and small bath polarization degrade the decoupling fidelity, enhanced performance and temporal modulation result from strong applied fields and high polarizations. Overall, we find that if the relative errors of the control pulse flip angles do not exceed 3%, decoupling protocols can still prolong the coherence time by up to 2 orders of magnitude.
Implementing precise operations on quantum systems is one of the biggest challenges for building quantum devices in a noisy environment. Dynamical decoupling attenuates the destructive effect of the environmental noise, but so far, it has been used primarily in the context of quantum memories. Here, we experimentally demonstrate a general scheme for combining dynamical decoupling with quantum logical gate operations using the example of an electron-spin qubit of a single nitrogen-vacancy center in diamond. We achieve process fidelities >98% for gate times that are 2 orders of magnitude longer than the unprotected dephasing time T2.