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Laser Physics

Pulses of 'fast light,' the signal velocity, and giant Kerr nonlinearity

A. M. Akulshin, Andrei I. Sidorov, Russell McLean, Peter Hannaford

Published Jan 1, 2005• 4 citations
OpenAlex

Abstract

We present the results of experimental studies of the propagation of light pulses through a specially prepared atomic medium with steep anomalous dispersion and enhanced Kerr nonlinearity. The observed negative group velocity is consistent with the principle of causality. The long-lived bright Zeeman coherence that is responsible for the steep anomalous dispersion gives rise also to a giant nonlinearity of the atomic susceptibility, which contributes substantially to the pulse propagation process. The enhanced atomic Kerr nonlinearity in the bright coherent state has been estimated.

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We investigate a light-pulse propagation with negative group velocity in a nonlinear coherent medium. We show that the necessary conditions for nonlinear superluminal effects to be observable are realized in a three-level $\ensuremath{\Lambda}$ system interacting with a linearly polarized laser field in the presence of a static magnetic field. The initially prepared Zeeman coherence cancels the resonant absorption of the medium almost completely, but preserves its dispersion anomalous and very high. In this medium the light pulse propagates superluminally in the sense that the peak of the transmitted pulse exits the medium before the peak of the incident pulse enters. At the same time the pulse group velocity is intensity dependent, which leads to the self-steepening of the pulse trailing edge due to the fact that the more intense parts of the pulse travel slower. This is in contrast with the shock wave generation in a nonlinear medium with normal dispersion. The predicted effect can be easily observed in the well-known schemes employed in the studies of nonlinear magneto-optical rotation. The upper bound of sample length is found from the criterion that the pulse self-steepening and group-advance time are observable without pulse distortion caused by the group-velocity dispersion.

arXiv:physics/0209036•Physical Review A•Jun 17, 2003•28 citations
We present the results of experimental studies of the propagation of light pulses through a specially prepared atomic medium with steep anomalous dispersion and enhanced Kerr nonlinearity. The observed negative group velocity is consistent with the principle of causality. The long-lived bright Zeeman coherence that is responsible for the steep anomalous dispersion gives rise also to a giant nonlinearity of the atomic susceptibility, which contributes substantially to the pulse propagation process. The enhanced atomic Kerr nonlinearity in the bright coherent state has been estimated.
We show that long-lived bright Zeeman coherence that is responsible for absorption enhancement and steep anomalous dispersion in an atomic medium gives rise to a giant nonlinearity of the atomic susceptibility, in a similar manner to the dark coherence responsible for the well-known electromagnetically induced transparency. The intensity dependent refractive index of Cs vapour with a ground state Zeeman coherence in the vicinity of the D2 resonance line has been measured at low light intensity. The Kerr nonlinearity in the bright coherent state (n2 approx 1.0 × 10-6 cm2 mW-1) is higher than that in a dark state under the same experimental conditions. Higher order nonlinear components of the refractive index have also been estimated for both coherent states.
Experimental investigation of the optical properties of atomic media with bright and dark long-lived light-induced Zeeman coherence is reported. We have obtained a small negative value for the group velocity of light pulses in Cs vapour ( V g ≃− c /6000), which agrees with direct anomalous dispersion measurements. The intensity dependent components of the refractive index of an atomic vapour with long-lived Zeeman coherence has been estimated. We have shown that such coherence can significantly enhance four-wave mixing, leading to the appearance of a multi-frequency comb-like spectrum at relatively low light intensity.
Atomic media have played a major role in studies of fast light. One of their attractive features is the ability to manipulate experimental parameters to control the dispersive properties that determine the group velocity of a propagating light pulse. We give an overview of the experimental methods, based on both linear and nonlinear atom-light interaction, that have produced superluminal propagation in atomic media, and discuss some of the significant theoretical contributions to the issues of pulse preservation and reconciling faster-than-light propagation and the principle of causality. The comparison of storage of light, enhanced Kerr nonlinearity and efficient wave mixing processes in slow and fast light atomic media illustrates their common and distinct features.
We have observed the propagation of an approximately 35 ns long light pulse with a negative group velocity through a laser-cooled 85Rb atomic medium. The anomalous dispersion results from linear atom–light interaction and is unrelated to long-lived ground-state coherences often associated with fast light in atomic media. The observed negative group velocity (−c/360) in the Rb magneto-optical trap for a pulse attenuated by less than 50% is in good agreement with the value of dispersion measured independently by a rf heterodyne method. The spectral region of anomalous dispersion is between 15 and 40 MHz, which is an order of magnitude wider than that typically associated with ground-state coherences.
Summary form only given. The propagation of light in a dispersive medium is characterized by the group velocity /spl nu//sub g/=c(n+/spl nu//sup dn//d/spl nu/)/sup .1/ where n is the refractive index and /spl nu/ the optical frequency. Depending on the sign and magnitude of /sup dn//d/spl nu/ in the medium, the group velocity can be positive, infinite or negative. The group velocity corresponds to the speed of the propagation of the maximum of an optical pulse travelling into the medium. This remains true whether the dispersion in the medium is normal (/sup dn//d/spl nu/>0) or anomalous (/sup dn//d/spl nu/<0). It has been demonstrated that coherently prepared atomic systems can exhibit steep dispersion leading to small absolute values of the group velocity (slow light). In recent work, we have demonstrated that narrow resonances arising from the coherent interaction of two optical fields with a closed atomic transition between two degenerate levels may correspond to a steep anomalous dispersion and thus to slow and negative group velocity. We report on the experimental study of the propagation of an amplitude modulated wave in a medium presenting negative group velocity.
We investigate a light-pulse propagation with negative group velocity in a nonlinear coherent medium. We show that the necessary conditions for nonlinear superluminal effects to be observable are realized in a three-level $\ensuremath{\Lambda}$ system interacting with a linearly polarized laser field in the presence of a static magnetic field. The initially prepared Zeeman coherence cancels the resonant absorption of the medium almost completely, but preserves its dispersion anomalous and very high. In this medium the light pulse propagates superluminally in the sense that the peak of the transmitted pulse exits the medium before the peak of the incident pulse enters. At the same time the pulse group velocity is intensity dependent, which leads to the self-steepening of the pulse trailing edge due to the fact that the more intense parts of the pulse travel slower. This is in contrast with the shock wave generation in a nonlinear medium with normal dispersion. The predicted effect can be easily observed in the well-known schemes employed in the studies of nonlinear magneto-optical rotation. The upper bound of sample length is found from the criterion that the pulse self-steepening and group-advance time are observable without pulse distortion caused by the group-velocity dispersion.