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Chinese Physics Letters

Cs 455 nm Nonlinear Spectroscopy with Ultra-narrow Linewidth

Dongying Wang, Yanfei Wang, Zhiming Tao, Shengnan Zhang, Yelong Hong, Wei Zhuang, Jingbiao Chen

Published Jun 1, 2013• 8 citations
Publisher

Abstract

Nonlinear spectroscopy has become a useful tool in laser cooling, frequency stabilization and so on. We use the 455.5 nm light beam output of an external cavity diode laser to perform the saturation spectroscopy signal and polarization spectroscopy signal on the 6S 1/2 → 7P 3/2 transition in cesium. The measured linewidth of the F4 → 4, 5 transition is as narrow as 1.40 MHz and that of the F3 → 2,3 transition is 1.67 MHz. Both of them are very close to the natural linewidth of about 1.2 MHz. Our result is the narrowest measured linewidth of Cs 455 nm saturation spectroscopy signal to our knowledge.

DOI
10.1088/0256-307x/30/6/060601

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Chinese Physics Letters•Mar 1, 2017•3 citations
Nonlinear spectroscopy has become a useful tool in laser cooling, frequency stabilization and so on. We use the 455.5 nm light beam output of an external cavity diode laser to perform the saturation spectroscopy signal and polarization spectroscopy signal on the 6S 1/2 → 7P 3/2 transition in cesium. The measured linewidth of the F4 → 4, 5 transition is as narrow as 1.40 MHz and that of the F3 → 2,3 transition is 1.67 MHz. Both of them are very close to the natural linewidth of about 1.2 MHz. Our result is the narrowest measured linewidth of Cs 455 nm saturation spectroscopy signal to our knowledge.
The features of Doppler-free resonances detected by probing the 133 Cs atom 6S 1/2 → 7P 3/2 transition at 456 nm in a nanometric-thick vapor layer are investigated. The matrix element of this transition is about 11 times smaller than that of the Cs D 2 line (852 nm). When the vapor layer thickness is ℓ = λ /2 ≃ 230 nm, we observe Dicke narrowing of the lines, accompanied by a red frequency shift of the atomic transitions, which is attributed to atom–surface interactions. Realizing optical pumping with ℓ ≃ 460 nm in a single-pass configuration, we observe Doppler-free resonances with a linewidth of <20 MHz, located at the atomic transition frequencies, with a correspondence of the amplitudes to the transition intensities. These narrow resonances are of interest for high-resolution spectroscopy and instrumentation and could serve as a frequency reference.
We demonstrate a nonlinear optical filter with ultranarrow bandwidth in cesium vapor. The optical filter operates on the 6S(1/2)→7P(3/2) transition at 455 nm. The single peak transmission at the 6S(1/2), F=4→7P(31/2), F'=5 transition is 9.7% with a bandwidth of 6.2 MHz, whereas at the 6S(1/2), F=3→7P(3/2), F'=2, 3 (cross-over) transition is 6.1% with a bandwidth of 3.9 MHz. The bandwidth approaching the natural linewidth is improved at least two orders of magnitude compared with conventional Faraday anomalous dispersion optical filters. This technique can also be applied to other alkali atoms.
Nowadays the long-range dipole-dipole interaction between highly-excited Rydberg atoms at micrometer distance become promising way to establish the atom-atom quantum entanglement and to implement the two-qubit logic gate. For alkali metal atoms, single-photon excitation from the ground state to the desired Rydberg state demands powerful narrow-linewidth ultra-violet (UV) laser, which is very challenging. Maybe just because of this, the studies of single-photon Rydberg excitation of alkali metal atoms are rare. Alternatively people have employed the two-photon or three-photon Rydberg excitation scheme. However, comparing with the single-photon Rydberg excitation, the two-photon or three-photon scheme has following drawbacks: atomic decoherence due to the photon scattering from the lower and upper transitions, and light shift of the involved ground state and Rydberg state due to the lower and upper transition laser beams. Thanks to the efficient laser frequency conversion technology with PPXX material and the well-developed commercial fiber laser as well as fiber amplifier, we have implemented a tunable 318.6-nm UV laser system based on the cavity-enhanced second-harmonic generation following the single-pass sum-frequency generation of 1560.5-nm and 1076.9-nm fiber-amplified lasers. More than 2-Watt output of the 318.6-nm UV laser has been achieved with a typical linewidth of smaller than 10 kHz. Employing the UV laser system we have demonstrated a single-photon Rydberg excitation spectroscopy of cesium (Cs) atoms. Partial Cs atoms can be directly excited from 6S_1/2 ground state to nP_3/2 (n = 70 - 100) Rydberg states, and Rydberg excitation spectra are obtained with transmission enhancement of a probe beam locked to Cs 6S_1/2 (F = 4) - 6P_3/2 (F’ = 5) cycling transition because partial population on the ground state (F = 4) are transferred to Rydberg state. The quantum defect for Cs nP_3/2 (n = 70 -100) Rydberg states is determined experimentally. Further more, the demodulated single-photon Rydberg excitation spectrum is employed to stabilize the UV laser to specific Cs Rydberg transition to improve the laser frequency stability. References: [1] Opt. Express 25 (2017) p.22510; [2] J. Opt. 19 (2017) 045501; [3] J. Opt. Soc. Am. B 33 (2016) p.2020; [4] Opt. Commun. 370 (2016) p.150. Funding: the National Natural Science Foundation of China (61475091).
High-power, narrow-linewidth light sources in the visible and UV spectra are in growing demand, particularly as quantum information and sensing research proliferates. Vertical external-cavity surface-emitting lasers (VECSELs) with intra-cavity frequency conversion are emerging as an attractive platform to fill these needs. Using such a device, we demonstrate 3.5 MHz full-width half-maximum Rydberg-state spectroscopy via electromagnetically induced transparency (EIT). The laser's 690 mW of output power at a wavelength of 475 nm enables large Rabi frequencies and strong signal-to-noise ratio in shorter measurement times. In addition, we characterize the frequency stability of the VECSEL using the delayed self-heterodyne technique and direct comparison with a commercial external-cavity diode laser (ECDL). We measure the pre-doubled light's Lorentzian linewidth to be 2π × 5.3(2) kHz, and the total linewidth to be 2π × 23(2) kHz. These measurements provide evidence that intra-cavity frequency-doubled VECSELs can perform precision spectroscopy at and below the MHz level, and are a promising tool for contemporary, and future, quantum technologies.
The utilization of atomic or molecular spectroscopy for frequency locking of single-frequency laser to improve laser frequency stability plays an important role in the experimental investigation of optically pumped atomic magnetometers, atomic clocks, laser cooling and trapping of atoms, etc. We have experimentally demonstrated a technique for frequency stabilization of a single-frequency laser employing the bright state spectroscopy (BSS) with a rubidium atomic vapor cell. By utilizing the counter-propagating dual-frequency 795 nm laser beams with mutually orthogonal linear polarization and a frequency difference of 6.834 GHz, which is equal to the hyperfine splitting of rubidium-87 ground state 5S1/2, an absorption-enhanced signal with narrow linewidth at the center of Doppler-broadened transmission spectroscopy is observed when continuous scanning the laser frequency over rubidium-87 D1 transition. This is the so-called BSS. Amplitude of the absorption-enhanced signal in the BSS is much larger compared with the conventional saturation absorption spectroscopy (SAS). The relationship between linewidth and amplitude of the BSS signal and laser beam intensity has been investigated. This high-contrast absorption-enhanced BSS signal has been employed for the laser frequency stabilization. The experimental results show that the frequency stability is 4.4×10−11 with an integration time of 40 s, near one order of magnitude better than that for using the SAS.
The sub-Doppler absorption laser spectroscopy at 728 nm transition from the 5 D 5 / 2 state to the 6 F state of cesium with linewidth near 10 MHz is first experimentally performed with indirect pumping from the ground state 6 S 1 / 2 to the state 7 P 3 / 2 by a 455.5 nm diode laser. Using a 455.5 nm diode laser as an indirect pump laser, several excited states will be populated due to spontaneous decay from the 7 P state. We first implement the sub-Doppler absorption laser spectroscopy at 728 nm from the 5 D 5 / 2 state to the 6 F state when Cs atoms within thermal glass cell decay to the 5 D 5 / 2 state. Due to velocity transfer effect, the hyperfine structure of 5 D 5 / 2 shows a mixed and complicated pattern but very clear structure when the 455.5 nm pumping laser is counter-propagating (or co-propagating) with the 728 nm probing laser.