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Low dimensional magnetism

Jonas A. Kjäll

Published Jan 1, 2012• 0 citations
OpenAlex

Abstract

Magnetism is a subject that has fascinated mankind for countless generations. With the development of quantum mechanics around a century ago a fundamental understanding of many of the underlying causes of magnetism were obtained. However, the long range interaction combined with the complex systems magnetism appears in makes it very hard to investigate it. In our days this research area is more active than ever, mainly due to future demand of the electronic industry for components engineered down to the atomic level. Quantum effects gets more important at short scales, especially in lower dimensional materials like sheets and wires. The rapidly increasing amount of computational power available makes the numerical techniques a more important part of the research effort. Many of these are especially well suited to analyze lower dimensional quantum problems. Three of the most important techniques, (classical) Monte Carlo, Exact Diagonalization (ED) and matrix product states (MPS) based techniques, like density renormalization group (DMRG) and time evolving block decimation (TEBD) will be described in some detail and put to use later in this dissertation.With the rapid development of experimental techniques for ultracold gases in optical traps a new approach to investigate magnetic properties that are hard achieve or control in the solid state has emerged. We first study the ground-state phase diagram of a spin-1 condensate trapped in an optical trap when the magnetic dipole interaction between the atoms is taken into account along with confinement and spin precession. The boundaries between the regions of ferromagnetic and polar phases move as the dipole strength is varied and the ferromagnetic phases can be modulated. The magnetization of the ferromagnetic phase perpendicular to the field becomes modulated as a helix winding around the magnetic field direction, with a wavelength inversely proportional to the dipole strength. This modulation should be observable for current experimental parameters in 87Rb. Hence the much-sought supersolid state, with broken continuous translation invariance in one direction and broken global U(1) invariance, occurs generically as a metastable state in this system as a result of dipole interaction. The ferromagnetic state parallel to the applied magnetic field becomes striped in a finite system at strong dipolar coupling.The development of artificial gauge fields, that can mimic magnetic fields, in ultracold gases suggests that atomic realization of fractional quantum Hall physics will become experimentally practical in the near future. While it is known that bosons on lattices can support quantum Hall states, the universal edge excitations that provide the most likely experimental probe of the topological order have not been obtained. We find that the edge excitations of an interacting boson lattice model are surprisingly sensitive to interedge hybridization and edge-bulk mixing for some confining potentials. With properly chosen potentials and fluxes, the edge spectrum is surprisingly clear even for small systems with strong lattice effects such as bandwidth. Various fractional quantum Hall phases for bosons can be obtained, and the phases ν=1/2 and ν=2/3 have the edge spectra predicted by the chiral Luttinger liquid theory.Also, some of the traditional experimental techniques for detecting magnetic order and dynamics in solid state materials, like neutron scattering has had somewhat of a renaissance lately. In a recent experiment on CoNb2O6, Coldea et. al. found for the first time experimental evidence of the exceptional Lie algebra E8. The emergence of this symmetry was theoretically predicted long ago for the transverse quantum Ising chain in the presence of a weak longitudinal field. We consider an accurate microscopic model of CoNb2O6 incorporating additional couplings and calculate numerically the dynamical structure function using a recently developed matrix-product-state method. The excitation spectra show bound states characteristic of the weakly broken $textrm{E}_8$ symmetry. We compare the observed bound state signatures in this model to those found in the transverse Ising chain in a longitudinal field and to experimental data.Finally, we investigate the ground state phase diagram of a related quantum spin chain, the S=2 XXZ chain with single-ion anisotropy. The interest in this system comes mainly from connecting the highly quantum mechanical spin-1 phase diagram with the classical S=∞ phase diagram. While most of these questions where believed to have been satisfactorily answered mainly with DMRG, some recent studies have questioned some of the conclusions. We use several of the recent advances within DMRG and perform a detailed analysis of the whole phase diagram. We extend the phase diagram by considering different types of single ion anisotropies which help us to answer two important questions: First we show that one can adiabatically move from the isotropic Heisenberg point to the so-called large-D phase with a continuous change of the Hamiltonian. Second, we can tune the model into a predicted intermediate phase which is equivalent to the topologically non-trivial spin-1 Haldane phase. Furthermore, we study the spin-3 XXZ chain to help explaining the development of the classical phase diagram.

Related papers

Magnetic phase diagram of a spin-1 condensate in two dimensions with dipole interaction

Jonas A. Kjäll, Andrew M. Essin, Joel E. Moore

Several new features arise in the ground-state phase diagram of a spin-1 condensate trapped in an optical trap when the magnetic-dipole interaction between the atoms is taken into account along with confinement and spin precession. The boundaries between the regions of ferromagnetic and polar phases move as the dipole strength is varied and the ferromagnetic phases can be modulated. The magnetization of the ferromagnetic phase perpendicular to the field becomes modulated as a helix winding around the magnetic field direction with a wavelength inversely proportional to the dipole strength. This modulation should be observable for current experimental parameters in $^{87}\text{R}\text{b}$. Hence the much-sought supersolid state with broken continuous translation invariance in one direction and broken global $U(1)$ invariance, occurs generically as a metastable state in this system as a result of dipole interaction. The ferromagnetic state parallel to the applied magnetic field becomes striped in a finite system at strong dipolar coupling.

arXiv:0909.1751•Physical Review B•Dec 8, 2009•7 citations

Non-Abelian gauge fields

Fabrice Gerbier, Nathan Goldman, Maciej Lewenstein +1 more

Building a universal quantum computer is a central goal of emerging quantum technologies, which has the potential to revolutionize science and technology. Unfortunately, this future does not seem to be very close at hand. However, quantum computers built for a special purpose, i.e. quantum simulators , are currently developed in many leading laboratories. Many schemes for quantum simulation have been proposed and realized using, e.g., ultracold atoms in optical lattices, ultracold trapped ions, atoms in arrays of cavities, atoms/ions in arrays of traps, quantum dots, photonic networks, or superconducting circuits. The progress in experimental implementations is more than spectacular. Particularly interesting are those systems that simulate quantum matter evolving in the presence of gauge fields. In the quantum simulation framework, the generated (synthetic) gauge fields may be Abelian, in which case they are the direct analogues of the vector potentials commonly associated with magnetic fields. In condensed matter physics, strong magnetic fields lead to a plethora of fascinating phenomena, among which the most paradigmatic is perhaps the quantum Hall effect. The standard Hall effect consists in the appearance of a transverse current, when a longitudinal voltage difference is applied to a conducting sample. For quasi-two-dimensional semiconductors at low temperatures placed in very strong magnetic fields, the transverse conductivity, the ratio between the transverse current and the applied voltage, exhibits perfect and robust quantization, independent for instance of the material or of its geometry. Such an integer quantum Hall effect, is now understood as a deep consequence of underlying topological order. Although such a system is an insulator in the bulk, it supports topologically robust edge excitations which carry the Hall current. The robustness of these chiral excitations against backscattering explains the universality of the quantum Hall effect. Another interesting and related effect, which arises from the interplay between strong magnetic field and lattice potentials, is the famous Hofstadter butterfly: the energy spectrum of a single particle moving on a lattice and subjected to a strong magnetic field displays a beautiful fractal structure as a function of the magnetic flux penetrating each elementary plaquette of the lattice. When the effects of interparticle interactions become dominant, two-dimensional gases of electrons exhibit even more exotic behaviour leading to the fractional quantum Hall effect. In certain conditions such a strongly interacting electron gas may form a highly correlated state of matter, the prototypical example being the celebrated Laughlin quantum liquid. Even more fascinating is the behaviour of bulk excitations (quasi-hole and quasi-particles): they are neither fermionic nor bosonic, but rather behave as anyons with fractional statistics intermediate between the two. Moreover, for some specific filling factors (ratio between the electronic density and the flux density), these anyons are proven to have an internal structure (several components) and non-Abelian braiding properties. Many of the above statements concern theoretical predictions—they have never been observed in condensed matter systems. For instance, the fractional values of the Hall conductance is seen as a direct consequence of the fractional statistics, but to date direct observation of anyons has not been possible in two-dimensional semiconductors. Realizing these predictions in experiments with atoms, ions, photons etc, which potentially allow the experimentalist to perform measurements complementary to those made in condensed matter systems, is thus highly desirable! Non-Abelian gauge fields couple the motional states of the particles to their internal degrees of freedom (such as hyperfine states for atoms or ions, electronic spins for electrons, etc). In this sense external non-Abelian fields extend the concept of spin–orbit coupling (Rashba and Dresselhaus couplings), familiar from AMO and condensed matter physics. They lead to yet another variety of fascinating phenomena such as the quantum spin Hall effect, three-dimensional topological insulators, topological superconductors and superfluids of various kinds. One also expects here the appearance of excitations in a form of topological edge states that can support robust transport, or entangled Majorana fermions in the case of topological superconductors or superfluids. Again, while many kinds of topological insulators have been realized in condensed matter systems, a controlled way of creating them in AMO systems and studying quantum phase transitions between various kinds of them is obviously very appealing and challenging. The various systems listed so far correspond to static gauge fields, which are externally imposed by the experimentalists. Even more fascinating is the possibility of generating synthetically dynamical gauge fields, i.e. gauge fields that evolve in time according to an interacting gauge theory, e.g., a full lattice gauge theory (LGT). These dynamical gauge fields can also couple to matter fields, allowing the quantum simulation of such complex systems (notoriously hard to simulate using 'traditional' computers), which are particularly relevant for modern high-energy physics. So far, most of the theoretical proposals concern the simulation of Abelian gauge theories, however, several groups have recently proposed extensions to the non-Abelian scenarios. The scope of the present focused issue of Journal of Physics B is to cover all of these developments, with particular emphasis on the non-Abelian gauge fields. The 14 papers in this issue include contributions from the leading theory groups working in this field; we believe that this collection will provide the reference set for quantum simulations of gauge fields. Although the special issue contains exclusively theoretical proposals and studies, it should be stressed that the progress in experimental studies of artificial Abelian and non-Abelian gauge fields in recent years has been simply spectacular. Multiple leading groups are working on this subject and have already obtained a lot of seminal results. The papers in the special issue are ordered according to the date of acceptance. The issue opens with a review article by Zhou et al [1] on unconventional states of bosons with synthetic spin–orbit coupling. Next, the paper by Maldonado-Mundo et al [2] studies ultracold Fermi gases with artificial Rashba spin–orbit coupling in a 2D gas. Anderson and Charles [3], in contrast, discuss a three-dimensional spin–orbit coupling in a trap. Orth et al [4] investigate correlated topological phases and exotic magnetism with ultracold fermions, again in the presence of artificial gauge fields. The paper of Nascimbène [5] does not address the synthetic gauge fields directly, but describes an experimental proposal for realizing one-dimensional topological superfluids with ultracold atomic gases; obviously, this problem is well situated in the general and growing field of topological superfluids, in particular those realized in the presence of non-Abelian gauge fields/spin–orbit coupling. Graß et al [6] consider in their paper fractional quantum Hall states of a Bose gas with spin–orbit coupling induced by a laser. Particular attention is drawn here to the possibility of realizing states with non-Abelian anyonic excitations. Zheng et al [7] study properties of Bose gases with Raman-induced spin–orbit coupling. Kiffner et al [8] in their paper touch on another kind of system, namely ultracold Rydberg atoms. In particular they study the generation of Abelian and non-Abelian gauge fields in dipole–dipole interacting Rydberg atoms. The behaviour of fermions in synthetic non-Abelian gauge potentials is discussed by Shenoy and Vyasanakere [9]. The paper starts with the study of Rashbon condensates (i.e. Bose condensates in the presence of Rashba coupling) and also introduces novel kinds of exotic Hamiltonians. Goldman et al [10] propose a concrete setup for realizing arbitrary non-Abelian gauge potentials in optical square lattices; they discuss how such synthetic gauge fields can be exploited to generate Chern insulators. Zygelman [11], similarly as Kiffner et al [8], discusses in his paper non-Abelian gauge fields in Rydberg systems. Marchukov et al [12] return to the subject of spin–orbit coupling, and investigate spectral gaps of spin–orbit coupled particles in the realistic situations of deformed traps. The last two papers, in contrast, are devoted to different subjects. Edmonds et al [13] consider a 'dynamical' density-dependent gauge potential, and study the Josephson effect in a Bose–Einstein condensate subject to such a potential. Last, but not least, Mazzucchi et al [14] study the properties of semimetal-superfluid quantum phase transitions in 3D lattices with Dirac points. References [1] Zhou X, Li Y, Cai Z and Wu C 2013 J. Phys. B: At. Mol. Opt. Phys. 46 134001 [2] Maldonado-Mundo D, Öhberg P and Valiente M 2013 J. Phys. B: At. Mol. Opt. Phys. 46 134002 [3] Anderson B M and Clark C W 2013 J. Phys. B: At. Mol. Opt. Phys. 46 134003 [4] Orth P P, Cocks D, Rachel S, Buchhold M, Le Hur K and Hofstetter W 2013 J. Phys. B: At. Mol. Opt. Phys. 46 134004 [5] Nascimbène S 2013 J. Phys. B: At. Mol. Opt. Phys. 46 134005 [6] Graß T, Juliá-Díaz B, Burrello M and Lewenstein M 2013 J. Phys. B: At. Mol. Opt. Phys. 46 134006 [7] Zheng W, Yu Z-Q, Cui X and Zhai H 2013 J. Phys. B: At. Mol. Opt. Phys. 46 134007 [8] Kiffner M, Li W and Jaksch D 2013 J. Phys. B: At. Mol. Opt. Phys. 46 134008 [9] Shenoy V B and Vyasanakere J P 2013 J. Phys. B: At. Mol. Opt. Phys. 46 134009 [10] Goldman N, Gerbier F and Lewenstein M 2013 J. Phys. B: At. Mol. Opt. Phys. 46 134010 [11] Zygelman B 2013 J. Phys. B: At. Mol. Opt. Phys. 46 134011 [12] Marchukov O V, Volosniev A G, Fedorov D V, Jensen A S and Zinner N T 2013 J. Phys. B: At. Mol. Opt. Phys. 46 134012 [13] Edmonds M J, Valiente M and Öhberg P 2013 J. Phys. B: At. Mol. Opt. Phys. 46 134013 [14] Mazzucchi G, Lepori L and Trombettoni A 2013 J. Phys. B: At. Mol. Opt. Phys. 46 134014

Journal of Physics B Atomic Molecular and Optical Physics•Jun 24, 2013•11 citations

Emergence of unconventional phases in quantum spin systems

Jean-Sébastien Bernier

In this thesis, we investigate strongly correlated phenomena in quantum spin systems. In the first part of this work, we study geometrically frustrated antiferromagnets (AFMs). Generalizing the SU(2) Heisenberg Hamiltonian to Sp(N) symmetry, we obtain, in the large-N limit, the mean-field phase diagrams for the planar pyrochlore and cubic AFMs. We then use gauge theories to consider fluctuation effects about their respective mean-field configurations. We find, in addition to conventional Neel states, a plethora of novel magnetically disordered phases: two kinds of spin liquids, Z2 in 2+1D and U(1)in 3+1D, and several valence bond solids such as two and three-dimensional plaquette and columnar singlet states. We use the same approach to study the diamond lattice AFM which possesses extended classical ground state degeneracy. We demonstrate that quantum and entropic fluctuations lift this degeneracy in different ways. In the second part of the thesis, we study ultracold spinor atoms confined in optical lattices. We first demonstrate the feasibility of experimental realization of rotor models using ultracold spin-one Bose atoms in a spin-dependent and disordered optical lattice. We show that the ground state of such disordered rotor models with quadrupolar interactions can exhibit biaxial nematic ordering in the disorder-averaged sense, and suggest an imaging experiment to detect the biaxial nematicity in such systems. Finally, using variational wavefunction methods, we study the Mott phases and superfluid-insulator transition of spin-three bosons in an optical lattice with an anisotropic two dimensional optical trap. We chart out the phase diagrams for Mott states with n = 1 and n = 2 atoms per lattice site. We show that the long-range dipolar interaction stabilizes a state characterized by antiferromagnetic chains made of ferromagnetically aligned spins. We also obtain the mean-field phase boundary for the superfluid-insulator transition, and show that inside the superfluid phase and near the superfluid-insulator phase boundary, the system undergoes a first order antiferromagnetic-ferromagnetic spin ordering transition.

•Jan 1, 2008•0 citations

Quantum Gas Microscopy of Strongly Correlated Bosons

Kim, Sooshin

A system of ultracold atoms in an optical lattice provides a powerful platform for quantum simulation. In our laboratory, we use a quantum gas microscope to tune lattice parameters not only in a global scale but also at the level of individual sites. This allows us to control and detect the quantum state of interacting many-body systems as well as to engineer a broad class of Hamiltonians with high fidelity. Leveraging this versatility, we can realize several types of strongly correlated bosonic systems, which present intriguing behaviors and implement novel phases of matter. Analyzing snapshots of the atomic distribution with single-site resolution, we measure correlations and entanglement within these systems to reveal their main features, including non-equilibrium dynamics and quantum phase transitions. In this thesis, I present the works performed by our team for four different types of systems. First of all, I briefly introduce the behavior of a 1D disordered system in the critical regime between the thermal and the many-body-localized phases. In particular, we discuss what happens when a disordered and a non-disordered region are coupled via a single site. We find evidence for accelerated transport of thermal inclusion into the localized region, which shows the existence of a quantum avalanche, i.e. thermalization via accelerated transport throughout the localized system. In the second part, we realize a fractional quantum Hall state using an artificial gauge field, by implementing an adiabatic preparation protocol. We identify a topological phase transition in our system and characterize several key physical features expected for a Laughlin state by measuring density correlations and Hall conductivity. The next topic of this thesis relates to quantum magnetism. Mapping nearest hopping in a tilted optical lattice to spin flips, we realize a finite one-dimensional chain of 1/2-spins with closed boundary conditions. We perform an in-depth investigation on behaviors shown across the quantum phase transition between paramagnetic and antiferromagnetic ground states, including the evolution of the magnetization and Néel order parameter. Also, we find evidence for quantum superposition at the many-body level as a result of geometric frustration. In the last chapter, I report the experimental realization of a novel dipolar Bose-Hubbard Hamiltonian, based on a strongly tilted lattice system. When the tilt becomes the dominant energy scale, the Hamiltonian is fragmented, and the system behaves in a way that conserves dipole moment. Starting from a 1D chain of unity filled sites, we generate individual dipolar and anti-dipolar excitations at desired pinpoints. We observe quantum walks of these dipolar quasi-particles as well as their scattering dynamics, which allows us to study this new type of Hamiltonian using a bottom-up approach.

•Jan 1, 2023•0 citations

Hydrodynamics of Bose gases with internal degrees of freedom

J. Armaitis

Just a couple decades ago bosonic low-temperature physics was synonymous with one particular liquid at a temperature of several degrees Kelvin. This liquid, helium-4, and its famous Helium-II phase, has revealed remarkable quantum properties such as quantized vortices and second sound. Yet, despite many things learned by investigating helium, its study has certain limitations. On the one hand, helium is a strongly interacting liquid, which makes first-principles theoretical research challenging. To name one example, establishing a connection between the non-interacting condensate state described by Bose and Einstein, and the helium properties observed in the lab took decades. Furthermore, helium is a specific chemical element, and hence there is no surprise that its physical properties are fixed by nature. However, every particular chemical element has particular physical properties, so for a long time it seemed that it was as good as it gets. The picture has changed drastically when the first Bose-Einstein condensate (BEC) was observed in an ultracold atomic gas. “Low temperature” has become synonymous with “ultracold”, and the latter implies temperatures on the order of nanokelvins. Most strikingly, the relationship between what is fixed by nature and what is experimentally changeable has evolved. In particular, systems of different particle statistics, spin, and interactions have been engineered using ultracold vapours of various alkali atoms. This versatile manipulation not only makes emulating various condensed-matter physics models in a controlled system without impurities possible, but also opens a path towards novel phenomena that are at present not achievable in any other manner. In this thesis, we have explored some of the novel phenomena that arise in systems of bosonic particles with internal degrees of freedom, such as (pseudo)spin and electric dipole moment. In the introduction, we describe a ferromagnetically coupled spin-1/2 Bose gas with contact interactions in the mean- field approximation. In particular, we compute and discuss the phase diagram of this gas, since it is a simple system which nevertheless has two order parameters. In the chapters that follow, the ideas touched upon in the introduction are developed in more detail. In Chapter 2 we develop a hydrodynamic description of the ferromagnetic spin-1/2 Bose gas at arbitrary temperatures. We study magnetization relaxation and geometric forces. In particular, we consider the topological Hall effect due to the presence of a skyrmion. In Chapter 3 we investigate the miscible (non-ferromagnetic) spin-1/2 Bose gas at arbitrary temperatures, construct its hydrodynamic description, calculate the thermodynamic properties, and study the collective modes of this system. In Chapter 4 we discuss the influence of the off-diagonal Berry curvature on the Bose-Einstein condensation temperature. Finally, in Chapter 5 we study a Bose-Einstein condensate of dipolar molecules in a weak electric field and find it to be described by a quantum rotor model. Moreover, we show that the molecular Bose-Einstein condensate is a ferroelectric material that is fully disordered by quantum fluctuations.

•Jun 3, 2015•0 citations

Topics in ultracold atomic gases: Strong interactions and quantum Hall physics

Weiran Li

This thesis discusses two important topics in ultracold atomic gases: strong interactions in quantum gases, and quantum Hall physics in neutral atoms.First we give a brief introduction on basic scattering models in atomic physics, and an approach to adjust the interactions between atoms.We also include a list of experimental probes in cold atom physics.After these introductions, in Chapter 3, we report a few interesting problems in strongly interacting quantum gases.We introduce the BCS-BEC crossover model and relevant many-body techniques at the beginning, and discuss the details of several specific systems.We find the Fermi gases across narrow Feshbach resonances are strongly interacting at low temperature even when the magnetic field is several widths away from the resonance.We also discuss an approach to describe the metastable repulsive branch of Bose and Fermi gases across the resonance, and find a stable region of repulsive Bose gas close to unitarity.Some studies in two dimensional Fermi gases with spin imbalance are also included, and they are closely related to a number of recent experiments.In Chapter 4, we discuss quantum Hall physics in the context of neutral atomic gases.After illustrating how the Berry phase experienced by neutral atoms is equivalent to the magnetic field in electrons, we introduce the newly developed synthetic gauge field scheme in which a gauge potential is coupled to the neutral atoms.We give a detail introduction to this Raman coupling scheme developed by NIST group, and derive the theoretical model of the system.Then we make some predictions on the evolution of quantum Hall states when an extra anisotropy is applied from the external trap.Finally, we propose some experiments to verify our predictions.4.9 Phase diagram of the cloud in rotating anisotropic traps: two phases of the BEC and QH are identified. . . . . . . . . . . . . . . . . . . . . . . . . . . .4.10 Distortion and transition in vortex lattices of a rapidly rotating BEC in an anisotropic trap. . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . .4.11 Density profiles at cut x = 0 and y = 0 of the Laughlin wavefunctions at different positions in figure 4.9. . . . . . . . . . . . . . . . . . . . . . . . . .4.12 Distribution of zeros in the relative coordinate of the ground state of two body problem in rotating anisotropic traps. . . . . . . . . . . . . . . . . . .4.13 Variation in the distance of splitting zeros as a function of inverse interaction strength, for fixed anisotropy α = 0.96. . . . . . . . . . . . . . . . . . . . . .4.14 Density profiles after TOF expansion of the gas in a rotating isotropic trap.4.15 Density profiles after TOF expansion of anisotropy α = 0.94. . . . . . . . .4.16 Second order correlation in equation 4.64, in a rotating isotropic (left) and anisotropic (right) trap. . . . . . . . . . . . . . . . . . . . . . . . . . . . . .4.17 A sketch of high-resolution in situ imaging technique in neutral atoms. . . .4.18 In situ images of the quantity |ψ(r/2, -r/2)| for an anisotropy α = 0.96. .x

•Jan 1, 2013•0 citations
Magnetism is a subject that has fascinated mankind for countless generations. With the development of quantum mechanics around a century ago a fundamental understanding of many of the underlying causes of magnetism were obtained. However, the long range interaction combined with the complex systems magnetism appears in makes it very hard to investigate it. In our days this research area is more active than ever, mainly due to future demand of the electronic industry for components engineered down to the atomic level. Quantum effects gets more important at short scales, especially in lower dimensional materials like sheets and wires. The rapidly increasing amount of computational power available makes the numerical techniques a more important part of the research effort. Many of these are especially well suited to analyze lower dimensional quantum problems. Three of the most important techniques, (classical) Monte Carlo, Exact Diagonalization (ED) and matrix product states (MPS) based techniques, like density renormalization group (DMRG) and time evolving block decimation (TEBD) will be described in some detail and put to use later in this dissertation.With the rapid development of experimental techniques for ultracold gases in optical traps a new approach to investigate magnetic properties that are hard achieve or control in the solid state has emerged. We first study the ground-state phase diagram of a spin-1 condensate trapped in an optical trap when the magnetic dipole interaction between the atoms is taken into account along with confinement and spin precession. The boundaries between the regions of ferromagnetic and polar phases move as the dipole strength is varied and the ferromagnetic phases can be modulated. The magnetization of the ferromagnetic phase perpendicular to the field becomes modulated as a helix winding around the magnetic field direction, with a wavelength inversely proportional to the dipole strength. This modulation should be observable for current experimental parameters in 87Rb. Hence the much-sought supersolid state, with broken continuous translation invariance in one direction and broken global U(1) invariance, occurs generically as a metastable state in this system as a result of dipole interaction. The ferromagnetic state parallel to the applied magnetic field becomes striped in a finite system at strong dipolar coupling.The development of artificial gauge fields, that can mimic magnetic fields, in ultracold gases suggests that atomic realization of fractional quantum Hall physics will become experimentally practical in the near future. While it is known that bosons on lattices can support quantum Hall states, the universal edge excitations that provide the most likely experimental probe of the topological order have not been obtained. We find that the edge excitations of an interacting boson lattice model are surprisingly sensitive to interedge hybridization and edge-bulk mixing for some confining potentials. With properly chosen potentials and fluxes, the edge spectrum is surprisingly clear even for small systems with strong lattice effects such as bandwidth. Various fractional quantum Hall phases for bosons can be obtained, and the phases ν=1/2 and ν=2/3 have the edge spectra predicted by the chiral Luttinger liquid theory.Also, some of the traditional experimental techniques for detecting magnetic order and dynamics in solid state materials, like neutron scattering has had somewhat of a renaissance lately. In a recent experiment on CoNb2O6, Coldea et. al. found for the first time experimental evidence of the exceptional Lie algebra E8. The emergence of this symmetry was theoretically predicted long ago for the transverse quantum Ising chain in the presence of a weak longitudinal field. We consider an accurate microscopic model of CoNb2O6 incorporating additional couplings and calculate numerically the dynamical structure function using a recently developed matrix-product-state method. The excitation spectra show bound states characteristic of the weakly broken textrmE8textrm{E}_8textrmE8​ symmetry. We compare the observed bound state signatures in this model to those found in the transverse Ising chain in a longitudinal field and to experimental data.Finally, we investigate the ground state phase diagram of a related quantum spin chain, the S=2 XXZ chain with single-ion anisotropy. The interest in this system comes mainly from connecting the highly quantum mechanical spin-1 phase diagram with the classical S=∞ phase diagram. While most of these questions where believed to have been satisfactorily answered mainly with DMRG, some recent studies have questioned some of the conclusions. We use several of the recent advances within DMRG and perform a detailed analysis of the whole phase diagram. We extend the phase diagram by considering different types of single ion anisotropies which help us to answer two important questions: First we show that one can adiabatically move from the isotropic Heisenberg point to the so-called large-D phase with a continuous change of the Hamiltonian. Second, we can tune the model into a predicted intermediate phase which is equivalent to the topologically non-trivial spin-1 Haldane phase. Furthermore, we study the spin-3 XXZ chain to help explaining the development of the classical phase diagram.
Several new features arise in the ground-state phase diagram of a spin-1 condensate trapped in an optical trap when the magnetic-dipole interaction between the atoms is taken into account along with confinement and spin precession. The boundaries between the regions of ferromagnetic and polar phases move as the dipole strength is varied and the ferromagnetic phases can be modulated. The magnetization of the ferromagnetic phase perpendicular to the field becomes modulated as a helix winding around the magnetic field direction with a wavelength inversely proportional to the dipole strength. This modulation should be observable for current experimental parameters in 87Rb^{87}\text{R}\text{b}87Rb. Hence the much-sought supersolid state with broken continuous translation invariance in one direction and broken global U(1)U(1)U(1) invariance, occurs generically as a metastable state in this system as a result of dipole interaction. The ferromagnetic state parallel to the applied magnetic field becomes striped in a finite system at strong dipolar coupling.
Building a universal quantum computer is a central goal of emerging quantum technologies, which has the potential to revolutionize science and technology. Unfortunately, this future does not seem to be very close at hand. However, quantum computers built for a special purpose, i.e. quantum simulators , are currently developed in many leading laboratories. Many schemes for quantum simulation have been proposed and realized using, e.g., ultracold atoms in optical lattices, ultracold trapped ions, atoms in arrays of cavities, atoms/ions in arrays of traps, quantum dots, photonic networks, or superconducting circuits. The progress in experimental implementations is more than spectacular. Particularly interesting are those systems that simulate quantum matter evolving in the presence of gauge fields. In the quantum simulation framework, the generated (synthetic) gauge fields may be Abelian, in which case they are the direct analogues of the vector potentials commonly associated with magnetic fields. In condensed matter physics, strong magnetic fields lead to a plethora of fascinating phenomena, among which the most paradigmatic is perhaps the quantum Hall effect. The standard Hall effect consists in the appearance of a transverse current, when a longitudinal voltage difference is applied to a conducting sample. For quasi-two-dimensional semiconductors at low temperatures placed in very strong magnetic fields, the transverse conductivity, the ratio between the transverse current and the applied voltage, exhibits perfect and robust quantization, independent for instance of the material or of its geometry. Such an integer quantum Hall effect, is now understood as a deep consequence of underlying topological order. Although such a system is an insulator in the bulk, it supports topologically robust edge excitations which carry the Hall current. The robustness of these chiral excitations against backscattering explains the universality of the quantum Hall effect. Another interesting and related effect, which arises from the interplay between strong magnetic field and lattice potentials, is the famous Hofstadter butterfly: the energy spectrum of a single particle moving on a lattice and subjected to a strong magnetic field displays a beautiful fractal structure as a function of the magnetic flux penetrating each elementary plaquette of the lattice. When the effects of interparticle interactions become dominant, two-dimensional gases of electrons exhibit even more exotic behaviour leading to the fractional quantum Hall effect. In certain conditions such a strongly interacting electron gas may form a highly correlated state of matter, the prototypical example being the celebrated Laughlin quantum liquid. Even more fascinating is the behaviour of bulk excitations (quasi-hole and quasi-particles): they are neither fermionic nor bosonic, but rather behave as anyons with fractional statistics intermediate between the two. Moreover, for some specific filling factors (ratio between the electronic density and the flux density), these anyons are proven to have an internal structure (several components) and non-Abelian braiding properties. Many of the above statements concern theoretical predictions—they have never been observed in condensed matter systems. For instance, the fractional values of the Hall conductance is seen as a direct consequence of the fractional statistics, but to date direct observation of anyons has not been possible in two-dimensional semiconductors. Realizing these predictions in experiments with atoms, ions, photons etc, which potentially allow the experimentalist to perform measurements complementary to those made in condensed matter systems, is thus highly desirable! Non-Abelian gauge fields couple the motional states of the particles to their internal degrees of freedom (such as hyperfine states for atoms or ions, electronic spins for electrons, etc). In this sense external non-Abelian fields extend the concept of spin–orbit coupling (Rashba and Dresselhaus couplings), familiar from AMO and condensed matter physics. They lead to yet another variety of fascinating phenomena such as the quantum spin Hall effect, three-dimensional topological insulators, topological superconductors and superfluids of various kinds. One also expects here the appearance of excitations in a form of topological edge states that can support robust transport, or entangled Majorana fermions in the case of topological superconductors or superfluids. Again, while many kinds of topological insulators have been realized in condensed matter systems, a controlled way of creating them in AMO systems and studying quantum phase transitions between various kinds of them is obviously very appealing and challenging. The various systems listed so far correspond to static gauge fields, which are externally imposed by the experimentalists. Even more fascinating is the possibility of generating synthetically dynamical gauge fields, i.e. gauge fields that evolve in time according to an interacting gauge theory, e.g., a full lattice gauge theory (LGT). These dynamical gauge fields can also couple to matter fields, allowing the quantum simulation of such complex systems (notoriously hard to simulate using 'traditional' computers), which are particularly relevant for modern high-energy physics. So far, most of the theoretical proposals concern the simulation of Abelian gauge theories, however, several groups have recently proposed extensions to the non-Abelian scenarios. The scope of the present focused issue of Journal of Physics B is to cover all of these developments, with particular emphasis on the non-Abelian gauge fields. The 14 papers in this issue include contributions from the leading theory groups working in this field; we believe that this collection will provide the reference set for quantum simulations of gauge fields. Although the special issue contains exclusively theoretical proposals and studies, it should be stressed that the progress in experimental studies of artificial Abelian and non-Abelian gauge fields in recent years has been simply spectacular. Multiple leading groups are working on this subject and have already obtained a lot of seminal results. The papers in the special issue are ordered according to the date of acceptance. The issue opens with a review article by Zhou et al [1] on unconventional states of bosons with synthetic spin–orbit coupling. Next, the paper by Maldonado-Mundo et al [2] studies ultracold Fermi gases with artificial Rashba spin–orbit coupling in a 2D gas. Anderson and Charles [3], in contrast, discuss a three-dimensional spin–orbit coupling in a trap. Orth et al [4] investigate correlated topological phases and exotic magnetism with ultracold fermions, again in the presence of artificial gauge fields. The paper of Nascimbène [5] does not address the synthetic gauge fields directly, but describes an experimental proposal for realizing one-dimensional topological superfluids with ultracold atomic gases; obviously, this problem is well situated in the general and growing field of topological superfluids, in particular those realized in the presence of non-Abelian gauge fields/spin–orbit coupling. Graß et al [6] consider in their paper fractional quantum Hall states of a Bose gas with spin–orbit coupling induced by a laser. Particular attention is drawn here to the possibility of realizing states with non-Abelian anyonic excitations. Zheng et al [7] study properties of Bose gases with Raman-induced spin–orbit coupling. Kiffner et al [8] in their paper touch on another kind of system, namely ultracold Rydberg atoms. In particular they study the generation of Abelian and non-Abelian gauge fields in dipole–dipole interacting Rydberg atoms. The behaviour of fermions in synthetic non-Abelian gauge potentials is discussed by Shenoy and Vyasanakere [9]. The paper starts with the study of Rashbon condensates (i.e. Bose condensates in the presence of Rashba coupling) and also introduces novel kinds of exotic Hamiltonians. Goldman et al [10] propose a concrete setup for realizing arbitrary non-Abelian gauge potentials in optical square lattices; they discuss how such synthetic gauge fields can be exploited to generate Chern insulators. Zygelman [11], similarly as Kiffner et al [8], discusses in his paper non-Abelian gauge fields in Rydberg systems. Marchukov et al [12] return to the subject of spin–orbit coupling, and investigate spectral gaps of spin–orbit coupled particles in the realistic situations of deformed traps. The last two papers, in contrast, are devoted to different subjects. Edmonds et al [13] consider a 'dynamical' density-dependent gauge potential, and study the Josephson effect in a Bose–Einstein condensate subject to such a potential. Last, but not least, Mazzucchi et al [14] study the properties of semimetal-superfluid quantum phase transitions in 3D lattices with Dirac points. References [1] Zhou X, Li Y, Cai Z and Wu C 2013 J. Phys. B: At. Mol. Opt. Phys. 46 134001 [2] Maldonado-Mundo D, Öhberg P and Valiente M 2013 J. Phys. B: At. Mol. Opt. Phys. 46 134002 [3] Anderson B M and Clark C W 2013 J. Phys. B: At. Mol. Opt. Phys. 46 134003 [4] Orth P P, Cocks D, Rachel S, Buchhold M, Le Hur K and Hofstetter W 2013 J. Phys. B: At. Mol. Opt. Phys. 46 134004 [5] Nascimbène S 2013 J. Phys. B: At. Mol. Opt. Phys. 46 134005 [6] Graß T, Juliá-Díaz B, Burrello M and Lewenstein M 2013 J. Phys. B: At. Mol. Opt. Phys. 46 134006 [7] Zheng W, Yu Z-Q, Cui X and Zhai H 2013 J. Phys. B: At. Mol. Opt. Phys. 46 134007 [8] Kiffner M, Li W and Jaksch D 2013 J. Phys. B: At. Mol. Opt. Phys. 46 134008 [9] Shenoy V B and Vyasanakere J P 2013 J. Phys. B: At. Mol. Opt. Phys. 46 134009 [10] Goldman N, Gerbier F and Lewenstein M 2013 J. Phys. B: At. Mol. Opt. Phys. 46 134010 [11] Zygelman B 2013 J. Phys. B: At. Mol. Opt. Phys. 46 134011 [12] Marchukov O V, Volosniev A G, Fedorov D V, Jensen A S and Zinner N T 2013 J. Phys. B: At. Mol. Opt. Phys. 46 134012 [13] Edmonds M J, Valiente M and Öhberg P 2013 J. Phys. B: At. Mol. Opt. Phys. 46 134013 [14] Mazzucchi G, Lepori L and Trombettoni A 2013 J. Phys. B: At. Mol. Opt. Phys. 46 134014
In this thesis, we investigate strongly correlated phenomena in quantum spin systems. In the first part of this work, we study geometrically frustrated antiferromagnets (AFMs). Generalizing the SU(2) Heisenberg Hamiltonian to Sp(N) symmetry, we obtain, in the large-N limit, the mean-field phase diagrams for the planar pyrochlore and cubic AFMs. We then use gauge theories to consider fluctuation effects about their respective mean-field configurations. We find, in addition to conventional Neel states, a plethora of novel magnetically disordered phases: two kinds of spin liquids, Z2 in 2+1D and U(1)in 3+1D, and several valence bond solids such as two and three-dimensional plaquette and columnar singlet states. We use the same approach to study the diamond lattice AFM which possesses extended classical ground state degeneracy. We demonstrate that quantum and entropic fluctuations lift this degeneracy in different ways. In the second part of the thesis, we study ultracold spinor atoms confined in optical lattices. We first demonstrate the feasibility of experimental realization of rotor models using ultracold spin-one Bose atoms in a spin-dependent and disordered optical lattice. We show that the ground state of such disordered rotor models with quadrupolar interactions can exhibit biaxial nematic ordering in the disorder-averaged sense, and suggest an imaging experiment to detect the biaxial nematicity in such systems. Finally, using variational wavefunction methods, we study the Mott phases and superfluid-insulator transition of spin-three bosons in an optical lattice with an anisotropic two dimensional optical trap. We chart out the phase diagrams for Mott states with n = 1 and n = 2 atoms per lattice site. We show that the long-range dipolar interaction stabilizes a state characterized by antiferromagnetic chains made of ferromagnetically aligned spins. We also obtain the mean-field phase boundary for the superfluid-insulator transition, and show that inside the superfluid phase and near the superfluid-insulator phase boundary, the system undergoes a first order antiferromagnetic-ferromagnetic spin ordering transition.
A system of ultracold atoms in an optical lattice provides a powerful platform for quantum simulation. In our laboratory, we use a quantum gas microscope to tune lattice parameters not only in a global scale but also at the level of individual sites. This allows us to control and detect the quantum state of interacting many-body systems as well as to engineer a broad class of Hamiltonians with high fidelity. Leveraging this versatility, we can realize several types of strongly correlated bosonic systems, which present intriguing behaviors and implement novel phases of matter. Analyzing snapshots of the atomic distribution with single-site resolution, we measure correlations and entanglement within these systems to reveal their main features, including non-equilibrium dynamics and quantum phase transitions. In this thesis, I present the works performed by our team for four different types of systems. First of all, I briefly introduce the behavior of a 1D disordered system in the critical regime between the thermal and the many-body-localized phases. In particular, we discuss what happens when a disordered and a non-disordered region are coupled via a single site. We find evidence for accelerated transport of thermal inclusion into the localized region, which shows the existence of a quantum avalanche, i.e. thermalization via accelerated transport throughout the localized system. In the second part, we realize a fractional quantum Hall state using an artificial gauge field, by implementing an adiabatic preparation protocol. We identify a topological phase transition in our system and characterize several key physical features expected for a Laughlin state by measuring density correlations and Hall conductivity. The next topic of this thesis relates to quantum magnetism. Mapping nearest hopping in a tilted optical lattice to spin flips, we realize a finite one-dimensional chain of 1/2-spins with closed boundary conditions. We perform an in-depth investigation on behaviors shown across the quantum phase transition between paramagnetic and antiferromagnetic ground states, including the evolution of the magnetization and Néel order parameter. Also, we find evidence for quantum superposition at the many-body level as a result of geometric frustration. In the last chapter, I report the experimental realization of a novel dipolar Bose-Hubbard Hamiltonian, based on a strongly tilted lattice system. When the tilt becomes the dominant energy scale, the Hamiltonian is fragmented, and the system behaves in a way that conserves dipole moment. Starting from a 1D chain of unity filled sites, we generate individual dipolar and anti-dipolar excitations at desired pinpoints. We observe quantum walks of these dipolar quasi-particles as well as their scattering dynamics, which allows us to study this new type of Hamiltonian using a bottom-up approach.
Just a couple decades ago bosonic low-temperature physics was synonymous with one particular liquid at a temperature of several degrees Kelvin. This liquid, helium-4, and its famous Helium-II phase, has revealed remarkable quantum properties such as quantized vortices and second sound. Yet, despite many things learned by investigating helium, its study has certain limitations. On the one hand, helium is a strongly interacting liquid, which makes first-principles theoretical research challenging. To name one example, establishing a connection between the non-interacting condensate state described by Bose and Einstein, and the helium properties observed in the lab took decades. Furthermore, helium is a specific chemical element, and hence there is no surprise that its physical properties are fixed by nature. However, every particular chemical element has particular physical properties, so for a long time it seemed that it was as good as it gets. The picture has changed drastically when the first Bose-Einstein condensate (BEC) was observed in an ultracold atomic gas. “Low temperature” has become synonymous with “ultracold”, and the latter implies temperatures on the order of nanokelvins. Most strikingly, the relationship between what is fixed by nature and what is experimentally changeable has evolved. In particular, systems of different particle statistics, spin, and interactions have been engineered using ultracold vapours of various alkali atoms. This versatile manipulation not only makes emulating various condensed-matter physics models in a controlled system without impurities possible, but also opens a path towards novel phenomena that are at present not achievable in any other manner. In this thesis, we have explored some of the novel phenomena that arise in systems of bosonic particles with internal degrees of freedom, such as (pseudo)spin and electric dipole moment. In the introduction, we describe a ferromagnetically coupled spin-1/2 Bose gas with contact interactions in the mean- field approximation. In particular, we compute and discuss the phase diagram of this gas, since it is a simple system which nevertheless has two order parameters. In the chapters that follow, the ideas touched upon in the introduction are developed in more detail. In Chapter 2 we develop a hydrodynamic description of the ferromagnetic spin-1/2 Bose gas at arbitrary temperatures. We study magnetization relaxation and geometric forces. In particular, we consider the topological Hall effect due to the presence of a skyrmion. In Chapter 3 we investigate the miscible (non-ferromagnetic) spin-1/2 Bose gas at arbitrary temperatures, construct its hydrodynamic description, calculate the thermodynamic properties, and study the collective modes of this system. In Chapter 4 we discuss the influence of the off-diagonal Berry curvature on the Bose-Einstein condensation temperature. Finally, in Chapter 5 we study a Bose-Einstein condensate of dipolar molecules in a weak electric field and find it to be described by a quantum rotor model. Moreover, we show that the molecular Bose-Einstein condensate is a ferroelectric material that is fully disordered by quantum fluctuations.
This thesis discusses two important topics in ultracold atomic gases: strong interactions in quantum gases, and quantum Hall physics in neutral atoms.First we give a brief introduction on basic scattering models in atomic physics, and an approach to adjust the interactions between atoms.We also include a list of experimental probes in cold atom physics.After these introductions, in Chapter 3, we report a few interesting problems in strongly interacting quantum gases.We introduce the BCS-BEC crossover model and relevant many-body techniques at the beginning, and discuss the details of several specific systems.We find the Fermi gases across narrow Feshbach resonances are strongly interacting at low temperature even when the magnetic field is several widths away from the resonance.We also discuss an approach to describe the metastable repulsive branch of Bose and Fermi gases across the resonance, and find a stable region of repulsive Bose gas close to unitarity.Some studies in two dimensional Fermi gases with spin imbalance are also included, and they are closely related to a number of recent experiments.In Chapter 4, we discuss quantum Hall physics in the context of neutral atomic gases.After illustrating how the Berry phase experienced by neutral atoms is equivalent to the magnetic field in electrons, we introduce the newly developed synthetic gauge field scheme in which a gauge potential is coupled to the neutral atoms.We give a detail introduction to this Raman coupling scheme developed by NIST group, and derive the theoretical model of the system.Then we make some predictions on the evolution of quantum Hall states when an extra anisotropy is applied from the external trap.Finally, we propose some experiments to verify our predictions.4.9 Phase diagram of the cloud in rotating anisotropic traps: two phases of the BEC and QH are identified. . . . . . . . . . . . . . . . . . . . . . . . . . . .4.10 Distortion and transition in vortex lattices of a rapidly rotating BEC in an anisotropic trap. . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . .4.11 Density profiles at cut x = 0 and y = 0 of the Laughlin wavefunctions at different positions in figure 4.9. . . . . . . . . . . . . . . . . . . . . . . . . .4.12 Distribution of zeros in the relative coordinate of the ground state of two body problem in rotating anisotropic traps. . . . . . . . . . . . . . . . . . .4.13 Variation in the distance of splitting zeros as a function of inverse interaction strength, for fixed anisotropy α = 0.96. . . . . . . . . . . . . . . . . . . . . .4.14 Density profiles after TOF expansion of the gas in a rotating isotropic trap.4.15 Density profiles after TOF expansion of anisotropy α = 0.94. . . . . . . . .4.16 Second order correlation in equation 4.64, in a rotating isotropic (left) and anisotropic (right) trap. . . . . . . . . . . . . . . . . . . . . . . . . . . . . .4.17 A sketch of high-resolution in situ imaging technique in neutral atoms. . . .4.18 In situ images of the quantity |ψ(r/2, -r/2)| for an anisotropy α = 0.96. .x