In injected lasers, only synchronization of the order $1/1$ (when a frequency of laser oscillations becomes equal to the master laser frequency) is usually observed. Such locking appears due to single-photon transitions in a laser. We show that with the use of multiple-photon transitions a higher-order synchronization can arise. We present the results of numerical simulations and the preliminary experimental observations, which demonstrate that in the mercury NMR laser, with the use of triple-photon transitions, a frequency of locked laser oscillations becomes three times higher than the frequency of an external rf magnetic field. Such synchronization appears only in the case of a linearly polarized (oscillating) external magnetic field. For the circularly polarized (rotating) external field, only synchronization of the order $1/1$ is possible.In injected lasers, only synchronization of the order $1/1$ (when a frequency of laser oscillations becomes equal to the master laser frequency) is usually observed. Such locking appears due to single-photon transitions in a laser. We show that with the use of multiple-photon transitions a higher-order synchronization can arise. We present the results of numerical simulations and the preliminary experimental observations, which demonstrate that in the mercury NMR laser, with the use of triple-photon transitions, a frequency of locked laser oscillations becomes three times higher than the frequency of an external rf magnetic field. Such synchronization appears only in the case of a linearly polarized (oscillating) external magnetic field. For the circularly polarized (rotating) external field, only synchronization of the order $1/1$ is possible.

Physical Review ASep 8, 20102 citations

Synchronization of Atomic Quantum Transitions by Light Pulses

Veniamin P. Chebotayev, V. A. Ulybin

NATO ASI series. Series B : PhysicsJan 1, 199011 citations

Synchronization of atomic quantum transitions by light pulses

Veniamin P. Chebotayev, V. A. Ulybin

Applied Physics BJan 1, 19909 citations

Picosecond synchronization of mode-locked lasers for metropolitan-scale quantum networks

Cory M. Nunn, Nijil Lal, Ivan A. Burenkov +4 more

We demonstrate picosecond-level synchronization of two actively mode-locked Ti:Sapphire lasers via the white rabbit precision time protocol (WR-PTP), tested over 120 km of deployed optical fiber. This synchronization capability, in combination with the highly single-mode, transform-limited pulses produced by each laser, enables their use as pump lasers for indistinguishable photon sources at remote locations in a quantum network. Here, the WR-PTP serves as a scalable network synchronization protocol, and its performance is compared to traditional methods of local synchronization. We demonstrate pulse-to-pulse synchronization better than 3 ps and time deviation (TDEV) values below 4 ps for all averaging times up to 10 s. With a designed coherence time of 35 ps for single photon sources utilizing these lasers, the achievable temporal overlap corresponds to 98% Hong-Ou-Mandel (HOM) interference visibility between independent sources.We demonstrate picosecond-level synchronization of two actively mode-locked Ti:Sapphire lasers via the white rabbit precision time protocol (WR-PTP), tested over 120 km of deployed optical fiber. This synchronization capability, in combination with the highly single-mode, transform-limited pulses produced by each laser, enables their use as pump lasers for indistinguishable photon sources at remote locations in a quantum network. Here, the WR-PTP serves as a scalable network synchronization protocol, and its performance is compared to traditional methods of local synchronization. We demonstrate pulse-to-pulse synchronization better than 3 ps and time deviation (TDEV) values below 4 ps for all averaging times up to 10 s. With a designed coherence time of 35 ps for single photon sources utilizing these lasers, the achievable temporal overlap corresponds to 98% Hong-Ou-Mandel (HOM) interference visibility between independent sources.

arXiv:2504.13773Optics ExpressJun 27, 20251 citation

Phase synchronization dynamics of a mutually coupled laser system for quantum random number generation

Berta Martínez-Pàmias, Miquel Rudé, Cristina Masoller

We performed an experimental and numerical study of an Indium Phosphide photonic integrated circuit designed for quantum random number generation. We investigated the dynamics of two weakly mutually coupled semiconductor lasers and the transient evolution towards the synchronization of the lasers’ optical phases. The simulated dynamics with the experimentally adjusted parameters were found to be in qualitatively good agreement with the experimental time traces. The results provide a better understanding of the evolution towards synchronization and a foundation for the optimization of the photonic quantum random number generation system.We performed an experimental and numerical study of an Indium Phosphide photonic integrated circuit designed for quantum random number generation. We investigated the dynamics of two weakly mutually coupled semiconductor lasers and the transient evolution towards the synchronization of the lasers’ optical phases. The simulated dynamics with the experimentally adjusted parameters were found to be in qualitatively good agreement with the experimental time traces. The results provide a better understanding of the evolution towards synchronization and a foundation for the optimization of the photonic quantum random number generation system.

EPJ Web of ConferencesJan 1, 20250 citations

Synchronization of Atomic Quantum Transitions by Light Pulses

Veniamin P. Chebotayev, V. A. Ulybin, V. M. Klementiev +2 more

Springer eBooksJan 1, 19910 citations

In injected lasers, only synchronization of the order

1/1

(when a frequency of laser oscillations becomes equal to the master laser frequency) is usually observed. Such locking appears due to single-photon transitions in a laser. We show that with the use of multiple-photon transitions a higher-order synchronization can arise. We present the results of numerical simulations and the preliminary experimental observations, which demonstrate that in the mercury NMR laser, with the use of triple-photon transitions, a frequency of locked laser oscillations becomes three times higher than the frequency of an external rf magnetic field. Such synchronization appears only in the case of a linearly polarized (oscillating) external magnetic field. For the circularly polarized (rotating) external field, only synchronization of the order

1/1

is possible.