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Bulletin of the American Physical Society

Resonance Fluorescence Spectrum from a Quantum Dot Driven by a Periodically-Pulsed Laser

Kumarsiri Konthasinghe, M. Peiris, Benjamin Petrak, Ying Yu, Zhichuan Niu, Andreas Müller

Published Mar 2, 2015• 0 citations
OpenAlex

Abstract

We report the measurement of the resonance fluorescence spectrum from a quantum dot under periodically-pulsed excitation. The evolution of multiple sidebands and Rabi oscillations for coherently and incoherently scattered light were observed.

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We investigated the first and second-order correlations of the light scattered near-resonantly by a quantum dot under excitation by a frequency comb, i.e., a periodically pulsed laser source. In contrast to its monochromatic counterpart, the pulsed resonance fluorescence spectrum features a superposition of sidebands distributed around a central peak with maximal sideband intensity near the Rabi frequency. Distinguishing between the coherently and incoherently scattered light reveals pulse-area dependent Rabi oscillations evolving with different phase for each component. Our observations, which can be reproduced theoretically, may impact schemes for remote entanglement based on pulsed two-photon interference.
Optical Rabi oscillations are coherent population oscillations of a two-level system coupled by an electric dipole transition when driven by a strong nearly resonant optical field. In quantum dot structures, these measurements have typically been performed as a function of the total pulse area $\ensuremath{\int}{\ensuremath{\Omega}}_{0}(t)\phantom{\rule{0.16em}{0ex}}\mathrm{d}t$ where the pulse area varies as a function of Rabi frequency. Here, we report direct detection of the time-resolved coherent transient response of the resonance fluorescence to measure the time evolution of the optical Rabi oscillations in a single charged InAs quantum dot. We extract a decoherence rate consistent with the limit from the excited state lifetime.
We show that resonance fluorescence, i.e., the resonant emission of a coherently driven two-level system, can be realized with a semiconductor quantum dot. The dot is embedded in a planar optical microcavity and excited in a waveguide mode so as to discriminate its emission from residual laser scattering. The transition from the weak to the strong excitation regime is characterized by the emergence of oscillations in the first-order correlation function of the fluorescence, g(tau), as measured by interferometry. The measurements correspond to a Mollow triplet with a Rabi splitting of up to 13.3 microeV. Second-order correlation measurements further confirm nonclassical light emission.
The interaction of a resonant light field with a quantum two-level system is of key interest both for fundamental quantum optics and quantum technological applications employing resonant excitation. While emission under resonant continuous-wave excitation has been well-studied, the more complex emission spectrum of dynamically dressed states, a quantum two-level system driven by resonant pulsed excitation, has so far been investigated in detail only theoretically. Here, we present the first experimental observation of the complete resonance fluorescence emission spectrum of a single quantum two-level system, in form of an excitonic transition in a semiconductor quantum dot, driven by finite Gaussian pulses. We observe multiple emerging sidebands as predicted by theory with an increase of their number and spectral detuning with excitation pulse intensity and a dependence of their spectral shape and intensity on the pulse length. Detuning-dependent measurements provide additional insights into the emission features. The experimental results are in excellent agreement with theoretical calculations of the emission spectra, corroborating our findings.
The interaction of a resonant light field with a quantum two-level system is of key interest both for fundamental quantum optics and quantum technological applications employing resonant excitation. While emission under resonant continuous-wave excitation has been well studied, the more complex emission spectrum of dynamically dressed states-a quantum two-level system driven by resonant pulsed excitation-has so far been investigated in detail only theoretically. Here, we present the first experimental observation of the complete resonance fluorescence emission spectrum of a single quantum two-level system, in the form of an excitonic transition in a semiconductor quantum dot, driven by finite Gaussian pulses. We observe multiple emerging sidebands as predicted by theory, with an increase of their number and spectral detuning with excitation pulse intensity and a dependence of their spectral shape and intensity on the pulse length. Detuning-dependent measurements provide additional insights into the emission features. The experimental results are in excellent agreement with theoretical calculations of the emission spectra, corroborating our findings.