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Bulletin of the American Physical Society

Non-classical Rydberg states for metrology experiments

Eva-Katharina Dietsche, Adrien Facon, Dorian Grosso, Adrien Signoles, I. Dotsenko, S. Haroche, J. M. Raimond, M. Brune, S. Gleyzes

Published Jun 10, 2015• 0 citations
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Interacting many-body systems display enhanced sensitivity close to critical transition points due to diverging quantum fluctuations. This criticality-based enhancement has been suggested as a potential resource for applications in precision metrology. Here we demonstrate many-body critical enhanced metrology for the sensing of external microwave electric fields in a non-equilibrium Rydberg atomic gas. We show that small variations in external driving lead to a large variation in the population of Rydberg states around criticality and to a notable change in the optical transmission signal. For continuous optical transmission at the critical point, we quantify the enhanced sensitivity extracting the Fisher information, which shows a three orders of magnitude increase due to many-body effects compared with single-particle systems. These results demonstrate that critical properties of many-body systems are promising resources for sensing and metrology applications. Interacting quantum systems near criticality have been proposed as potential probes for quantum metrology. An experiment with Rydberg atoms now proves the enhanced sensitivity of critical many-body systems to small variations in external parameters.
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Rydberg states of atoms in vacuum are now well recognized as a resource for quantum technologies. Donors in semiconductors also display analogous states, which have been proposed for similar applications. While they benefit from permanent locations in their host crystals, electron-lattice coupling leads to much shorter excited-state lifetimes than for neutral atoms in vacuum. Here we provide a quantitative description of donor-phonon kinetics, creating a basis for engineering donor systems in realistic material stacks for quantum devices. Our theory incorporates both form factors for the Rydberg states, which given their large extents in real space provide strong selectivity in momentum space, and tabulated deformation potentials for all six phonon branches throughout the Brillouin zone. By confronting this framework with carefully controlled time-resolved free electron laser measurements, we show that the widely quoted position of the silicon conduction band minimum, k0k_0k0​, is inconsistent with observed donor relaxation rates and that quantitative agreement is obtained for a value further from the X-point than commonly assumed. This stringent experiment-theory comparison establishes donor relaxation as a precision metrology for conduction band parameters and scattering processes in silicon, with consequences spanning from quantum devices to classical electronics.
Circular atoms, i.e., Rydberg atoms with maximum angular momentum, are semiclassical atoms of great interest for Rydberg constant metrology and QED tests. Following a suggestion by Delande and Gay, we have prepared circular atoms by a new method, involving the adiabatic switching of crossed electric and magnetic fields. The method, which is demonstrated for Rydberg states of lithium (principal quantum number n=20to25n=20 \mathrm{to} 25n=20to25, is applicable over a wide variety of experiment conditions.