Abstract Recent experiments on ultracold atoms in optical lattices have synthesized a variety of tunable bands with degenerate double-well structures in momentum space. Such degeneracies in the single-particle spectrum strongly enhance quantum fluctuations, and often lead to exotic many-body ground states. Here we consider weakly interacting spinor Bose gases in such bands, and discover a universal quantum ‘order by disorder’ phenomenon which selects a novel superfluid with chiral spin order displaying remarkable properties such as spontaneous spin Hall effect and momentum space antiferromagnetism. For bosons in the excited Dirac band of a hexagonal lattice, such a state supports staggered spin loop currents in real space. We show that Bloch oscillations provide a powerful dynamical route to quantum state preparation of such a chiral spin superfluid. Our predictions can be readily tested in spin-resolved time-of-flight experiments.
Abstract Recent experiments on ultracold atoms in optical lattices have synthesized a variety of tunable bands with degenerate double-well structures in momentum space. Such degeneracies in the single-particle spectrum strongly enhance quantum fluctuations, and often lead to exotic many-body ground states. Here we consider weakly interacting spinor Bose gases in such bands, and discover a universal quantum ‘order by disorder’ phenomenon which selects a novel superfluid with chiral spin order displaying remarkable properties such as spontaneous spin Hall effect and momentum space antiferromagnetism. For bosons in the excited Dirac band of a hexagonal lattice, such a state supports staggered spin loop currents in real space. We show that Bloch oscillations provide a powerful dynamical route to quantum state preparation of such a chiral spin superfluid. Our predictions can be readily tested in spin-resolved time-of-flight experiments.
Abstract Topological superfluidity is an important concept in electronic materials as well as ultracold atomic gases1. However, although progress has been made by hybridizing superconductors with topological substrates, the search for a material—natural or artificial—that intrinsically exhibits topological superfluidity has been ongoing since the discovery of the superfluid 3He-A phase2. Here we report evidence for a globally chiral atomic superfluid, induced by interaction-driven time-reversal symmetry breaking in the second Bloch band of an optical lattice with hexagonal boron nitride geometry. This realizes a long-lived Bose–Einstein condensate of 87Rb atoms beyond present limits to orbitally featureless scenarios in the lowest Bloch band. Time-of-flight and band mapping measurements reveal that the local phases and orbital rotations of atoms are spontaneously ordered into a vortex array, showing evidence of the emergence of global angular momentum across the entire lattice. A phenomenological effective model is used to capture the dynamics of Bogoliubov quasi-particle excitations above the ground state, which are shown to exhibit a topological band structure. The observed bosonic phase is expected to exhibit phenomena that are conceptually distinct from, but related to, the quantum anomalous Hall effect3–7 in electronic condensed matter.
We study a spinor (two-component) Bose gas confined in a one-dimensional double-valley optical lattice which has a double-well structure in momentum space. Based on field theory analysis, it is found that spinor bosons in the double-valley band may form a spin-charge mixed chiral spin quasicondensate under certain conditions. Our numerical calculations in a concrete $\ensuremath{\pi}$-flux triangular ladder system confirm the robustness of the chiral spin order against interactions and quantum fluctuations. This exotic atomic Bose-Einstein condensate exhibits spatially staggered spin loop currents without any charge dynamics despite the complete absence of spin-orbit coupling in the system, creating an interesting approach to atom spintronics. The entanglement entropy scaling allows us to extract conformal-field-theory central charge and establish the low-energy effective field theory for the chiral spin condensate as a two-component Luttinger liquid. Our predictions should be detectable in atomic experiments through spin-resolved time-of-flight techniques.
Ultracold atoms loaded into higher Bloch bands provide an elegant setting for realizing many-body quantum states that spontaneously break time-reversal symmetry through the formation of chiral orbital order. The applicability of this strategy remains nonetheless limited due to the finite lifetime of atoms in high-energy bands. Here we introduce an alternative framework, suitable for bosonic gases, which builds on assembling square plaquettes pierced by a $\ensuremath{\pi}$ flux (half a magnetic-flux quantum). This setting is shown to be formally equivalent to an interacting bosonic gas loaded into p orbitals, and we explore the consequences of the resulting chiral orbital order, both for weak and strong on-site interactions. We demonstrate the emergence of a chiral superfluid vortex lattice, exhibiting a long-lived gapped collective mode that is characterized by local chiral currents. This chiral superfluid phase is shown to undergo a phase transition to a chiral Mott insulator for sufficiently strong interactions. Our work establishes coupled $\ensuremath{\pi}$-flux plaquettes as a practical route for the emergence of orbital order and chiral phases of matter.
The anomalous Hall effect has had a profound influence on the understanding of many electronic topological materials but is much less studied in their bosonic counterparts. We predict that an intrinsic anomalous Hall effect exists in a recently realized bosonic chiral superfluid, a p-orbital Bose-Einstein condensate in a 2D hexagonal boron nitride optical lattice [Wang et al., Nature (London) 596, 227 (2021)NATUAS0028-083610.1038/s41586-021-03702-0]. We evaluate the frequency-dependent Hall conductivity within a multi-orbital Bose-Hubbard model that accurately captures the real experimental system. We find that in the high frequency limit, the Hall conductivity is determined by finite loop current correlations on the s-orbital residing sublattice, the latter a defining feature of the system's chirality. In the opposite limit, the dc Hall conductivity can trace its origin back to the noninteracting band Berry curvature at the condensation momentum, although the contribution from atomic interactions can be significant. We discuss available experimental probes to observe this intrinsic anomalous Hall effect at both zero and finite frequencies.
Quantum degenerate atomic gases offer a unique platform for the exploration of a wide variety of interacting many-body systems in a pristine environment, based on a set of powerful tools for the coherent control of the atoms' internal and external degrees of freedom. Here, we present experimental studies of strongly interacting bosonic mixtures in one-dimensional (1D) systems, in which the mobilities of the two species are independently controlled with a state-selective optical lattice. In a first experiment, we freeze out the tunneling of one species from a binary mixture, and study the formation of ``quantum emulsion'' states, where immobile atoms serve as a static, random disorder for a more mobile species. We investigate the 1D superfluid-to-insulator transition in the presence of this disorder, and make comparisons to the effects of quasi-disorder from an incommensurate optical lattice. We observe enhanced localization in the more random potential, highlighting the important role of correlations in disordered systems. Through a combined measurement of transport, localization, and excitation spectra, we are able to obtain strong evidence for observation of a disordered, insulating quantum phase, the 1D Bose glass. In a second experiment, we introduce a new experimental technique for the characterization of ultracold gases held in optical lattices. In analogy to neutron diffraction from solids, we use atomic de Broglie waves to non-destructively probe the spatial structure of 1D Mott insulators through elastic Bragg diffraction, and to probe inelastic band-structure excitations of more weakly interacting 1D Bose gases. Furthermore, we use the diffraction of matter waves to detect the formation of forced-antiferromagnetic ordering in a crystalline atomic spin mixture. Lastly, we study the dynamical response of matter waves to a periodically pulsed, incommensurate optical lattice, a situation that realizes a system of two coupled kicked quantum rotors. We observe that the coupling induces a suppression of energy growth at quantum resonances, and a localization-to-delocalization transition in momentum space for off-resonant driving. Our observations confirm a long-standing theoretical prediction for the two-rotor system, and illustrate how classical behavior can emerge from the evolution of a simple quantum system. | 193 pages
Motivated by experiments on Josephson junction arrays in a magnetic field and ultracold interacting atoms in an optical lattice in the presence of a ``synthetic'' orbital magnetic field, we study the ``fully frustrated'' Bose-Hubbard model and quantum XY model with half a flux quantum per lattice plaquette. Using Monte Carlo simulations and the density matrix renormalization group method, we show that these kinetically frustrated boson models admit three phases at integer filling: a weakly interacting chiral superfluid phase with staggered loop currents which spontaneously break time-reversal symmetry, a conventional Mott insulator at strong coupling, and a remarkable ``chiral Mott insulator'' (CMI) with staggered loop currents sandwiched between them at intermediate correlation. We discuss how the CMI state may be viewed as an exciton condensate or a vortex supersolid, study a Jastrow variational wave function which captures its correlations, present results for the boson momentum distribution across the phase diagram, and consider various experimental implications of our phase diagram. Finally, we consider generalizations to a staggered flux Bose-Hubbard model and a two-dimensional (2D) version of the CMI in weakly coupled ladders.