We survey phenomena of a cavity system in which many atoms coherently interact with a single quantized photon mode driven by the AC external field in a dissipative environment. It has been known that a strong external field causes the so-called optical bistability which is a non-equilibrium phase transition for the balance of excitation and dissipation. On the other hand, a strong interaction causes the Dicke transition, which is a phase transition with a spontaneous appearance of excitations of photons and atoms in the equilibrium system as a consequence of the cooperative phenomena. We study the phenomena in full range of the strength of the interaction and the external field, and present a phase diagram of the stationary state. For the strong interaction region, in order to realize the ground state, appropriate form of the dissipative mechanism in the master equation is necessary instead of the conventional Lindblad form. We provide such an extended master equation. Moreover, the rotating wave approximation may not become appropriate, and thus we study both Tavis-Cummings model with rotating wave approximation and the Dicke model without it, and compare the phase diagrams with each other.
We survey phenomena of a cavity system in which many atoms coherently interact with a single quantized photon mode driven by the AC external field in a dissipative environment. It has been known that a strong external field causes the so-called optical bistability which is a non-equilibrium phase transition for the balance of excitation and dissipation. On the other hand, a strong interaction causes the Dicke transition, which is a phase transition with a spontaneous appearance of excitations of photons and atoms in the equilibrium system as a consequence of the cooperative phenomena. We study the phenomena in full range of the strength of the interaction and the external field, and present a phase diagram of the stationary state. For the strong interaction region, in order to realize the ground state, appropriate form of the dissipative mechanism in the master equation is necessary instead of the conventional Lindblad form. We provide such an extended master equation. Moreover, the rotating wave approximation may not become appropriate, and thus we study both Tavis-Cummings model with rotating wave approximation and the Dicke model without it, and compare the phase diagrams with each other.
We study non-equilibrium stationary states of a cavity system consisting of many atoms interacting with a quantized cavity field mode, under a driving field in a dissipative environment. We derive a quantum master equation which is suitable for treating systems with a strong driving field and a strong atom–photon interaction. We do this by making use of the fact that the mean-field dynamics are exact in the thermodynamic limit thanks to a uniform coupling between atoms and photons. We find ordered states with symmetry-broken components of the photon field and atomic excitation driven by the external field. The mechanism by which these ordered states arise is discussed from the viewpoint of the quantum interference effect.
The dissipative quantum phase transitions experienced by a driven optical system are studied in order to understand the underlying light-matter coupling. The primary system under study is composed of a cavity mode coupled to a two-level system with dissipation being introduced through the interaction with a surrounding environment; an external coherent field is included to drive the system out of the ground state. The coupling is given by a generalized Rabi Hamiltonian, where rotating, gr, and counter-rotating, ngr, couplings are both present and can be adjusted independently. A comprehensive study of the different phases the system can exhibit as gr and n are varied is presented. From this, we construct a bridge between two limiting scenarios: (i) the Jaynes-Cummings limit (n = 0), where the system undergoes a phase transition by means of the breakdown of the photon blockade, and (ii) the driven Dicke limit ( = 1 ), where the normal to super-radiant phase transition is found. Novel behaviour encountered in an intermediate regime (1 > n > 0) is discussed. Attention is drawn towards the strong coupling regime, where changes at the one-photon level induce nonlinear effects and behaviour reminiscent of phase transitions is encountered with just a few photons present. A comparison between weak and strong coupling regimes, and, thus, an exploration of the effect of fluctuations over quantum phase transitions of light, is given through a survey of the phases an auxiliary optical system exhibits. This system is composed of two coupled nonlinear cavities that are driven coherently and damped through the interaction with the environment; it is seen to exhibit three phases. Two phases present high-correlation between the cavities and are differentiated by the photon statistics, transitioning from classical to quantum. The third phase is characterized by a highly localized field in one of the cavities. The departure from mean-field results is highlighted and a new way to characterize the possible phases of the system is proposed. Finally, the crucial role of quantum fluctuations is quantified and used to define the phases at hand.
In this paper, the quantum phase transitions caused by the interactions between light and atoms, as well as between light and mechanical oscillators, are discussed theoretically in a coupled optomechanical cavity containing two optical field modes (N atoms and mechanical oscillator). By using Holstein-Primak off transformation method, new translational boson operators and four parameters are assumed. The ground state energy functional of the system and a set of equations composed of four parameters are given. The correctness of the assumed translation boson operators is proved by two special cases. In the case of resonance, the characteristics of the obtained solutions are shown by solving the equations, graphical method and Hessian matrix judgment. The stable zero solution is called the normal phase, the unstable zero solution is named the unstable vacuum macroscopic phase, and the stable non-zero solution is referred to as the superradiation phase. The phase can transition from normal phase to superradiation phase, and the point of phase transition can be changed by adjusting the coupling intensity of the two cavity light fields. When the nonlinear photon-phonon interaction caused by radiation pressure is considered, the phase diagram of the system is expanded from the original two phase regions to three phase regions, including the coexistent normal phase and superradiation phase, the bistable superradiation phase, and the unstable vacuum macroscopic phase region, where the bistable superradiation phase is similar to the optical bistable phenomenon. At the same time, there is also a turning point curve, which overlaps with the phase transition point curve, indicating the existence of multiple quantum phase transitions in the system. These predictions can be detected by measuring the average number of photons. The coupled optomechanical cavity that we studied, when considering the coupling of the two-mode optical field and the atomic ensemble but no mechanical oscillator, reflects the interaction between the two-mode optical field and the atom, thus concluding that the transformation point is small and the quantum phase transition is easy to occur. When the coupling between the mechanical oscillator and the two-mode optical field is not considered, the interaction between the single-mode optical field and the atom is reflected, returning to the quantum phase transition of the Dicke model under rotating wave approximation.
Present-day experiments have started to couple traditional simulations of ultracold atom experiments with quantum light-fields in cavities. This has provided a wealth of op- portunities to enlarge the number of interaction potentials: cavity mediated long-range interactions compete with kinetic energies, longitudinal fields, short-ranged collisional or magnetic spin-spin interactions. The intracavity many-body lattice models often have to be maintained far from equilibrium through the presence of external driving lasers that help to boost and engineer the various interaction potentials. The steady influx of energy is compensated by a steady stream of energy out of the atom-cavity system for example by photon losses or atomic spontaneous emission. Several experiments have demonstrated that such environments can give rise to new competing quantum phases. \nBut this long-standing ambition to push for models with tailorable interaction potentials can bring with it also considerable challenges in their theoretical description, since sponta- neous symmetry breaking transitions in many body lattice systems coupled to dynamical light-fields with single-photon character occur in the presence of drive and dissipation for the photonic force carriers. This clearly calls for model systems where the above men- tioned interplay of interactions, drive, dissipation and cooperative many-body behaviour can be theoretically studied to provide simple, experimentally verifiable predictions. \nThe Dicke model is, through its simplicity (an exactly solved ferromagnet with infinite range atom-atom interactions mediated by a single cavity mode), an exceptionally well- suited candidate. As the generic model for atom-light interactions, it has been experimen- tally realized in a variety of modern quantum optical systems, highlighting its relevance for present-day research. The Dicke model is also highly versatile itself. It has been extended into the dissipative realm, was promoted to account for multiple optical light modes and was used to describe multiple, coupled single-mode cavity structures. It was adapted to treat spin-selective coupling to a cavity to describe superradiance phase tran- sitions in multi-level atomic systems. Moreover, it was realised in electronic circuits where the dipole coupling of real atoms to single mode fields is replaced by a capacitive cou- pling of artificial atoms to a resonator mode. This illustrates that the Dicke model and its extended variants are ’future-proof’ and continue to be of relevance for fundamental light-matter interactions and for driven-dissipative phase transitions. \nIn this thesis, we investigate magnetic phase transitions in driven-dissipative atomic en- sembles interacting with quantum light. We present three research projects on variants of cooperative radiation of an ensemble of laser driven two-level atoms in a single mode optical cavity, as described by the Dicke model. \nThroughout the chapters 2,3 and 4 that contain the main body of research of this thesis, we investigate phase transitions between non-equilibrium stationary states in engineered quantum-optical systems each of which extends the conventional Dicke model physics. As a starting point, we map the quantum equations of motion onto a set of semiclassical nonlinear stochastic equations and analyse their stationary states and instabilities with master equations for atomic spin and photon mean-field amplitudes. These are used to obtain experimentally relevant parameters such as critical atom-light couplings for phase transitions, phase diagrams and properties of stationary non-equilibrium states in addition to cavity output spectra that identify the imprint of magnetic correlations in the light-field. \nIn chapter 2, we help resolve a discrepancy between earlier experimental investigations of the critical atom-light coupling strength for the superradiance transition in the Dicke model: higher external pumping strengths than theoretically predicted were needed to observe a coherent, superradiant state of the light field in an optical cavity. By including incoherent spontaneous emission of atomic excitations, we extend the dissipative Dicke model to a two loss channel variant containing both photon leakage and atomic decay that reproduces the experimentally observed critical atom-light coupling. \nRecent experiments have started to interface quantum many body lattice models with coherent cavity fields, thereby allowing to realize new quantum phases through competing atom-cavity and atom-atom interactions. In chapter 3, we consider a simplified model for such a set-up where a single quantized mode of the light-field interacts with an ensemble of Rydberg-dressed atoms inside a high finesse optical cavity. This model provides a base case for further studies of quantum magnets in optical cavities. At the heart of this model is a competition of short- (dipolar atom-atom) and long-range (atom-light) interactions at the Hamiltonian level in the presence of both spontaneous emission and photon leak- age through the cavity mirrors. We show that different magnetic phases can coexist with coherent atomic radiation and provide clear experimental signatures to identify the mag- netic structure and intra-cavity dynamics. We suggest an experimental level-scheme for a quantum optical implementation of our model. \nIn chapter 4 we consider a generic, collective decay for many-body excitations in the paradigmatic Dicke model. This extension drastically enriches the dynamics as it induces a bicritical point and a bistable regime dominated by true non-equilibrium fluctuations that induce a dissipative first-order phase transition that can only be resolved by including finite fluctuation corrections with the help of stochastic Langevin equations. We investigate the hysteretic response to time-dependent ramps of the atom-light coupling. Discontinuous first-order phase transitions where metastable states coexist in a hysteresis domain have been investigated in recent dissipative quantum-optical experiments. We review noise- activation far from thermal equilibrium in chapter 5.
The Dicke model describes the coherent interaction of a laser-driven ensemble of two-level atoms with a quantized light field. It is realized within cavity QED experiments, which in addition to the coherent Dicke dynamics feature dissipation due to, e.g., atomic spontaneous emission and cavity photon loss. Spontaneous emission supports the uncorrelated decay of individual atomic excitations as well as the enhanced collective decay of an excitation that is shared by N atoms and whose strength is determined by the cavity geometry. We derive a many-body master equation for the dissipative Dicke model including both spontaneous emission channels and analyze its dynamics on the basis of Heisenberg-Langevin and stochastic Bloch equations. We find that the collective loss channel leads to a region of bistability between the empty and the superradiant state. Transitions between these states are driven by nonthermal Markovian noise. The interplay between dissipative and coherent elements leads to a genuine nonequilibrium dynamics in the bistable regime, which is expressed via a nonconservative force and a multiplicative noise kernel appearing in the stochastic Bloch equations. We present a semiclassical approach, based on stochastic nonlinear optical Bloch equations, which for the infinite-range Dicke model become exact in the large-N-limit. The absence of an effective free-energy functional, however, necessitates the inclusion of fluctuation corrections with O(1/N) for finite $N<\ensuremath{\infty}$ to locate the nonthermal first-order phase transition between the superradiant and the empty cavity.
Dicke model, as an important many-body model in quantum optics, describes the interaction between multiple identical two-level atoms and a quantized electromagnetic field. This spin-boson model shows collective phenomena in light-matter interaction systems and can undergo a second-order quantum phase transition from a normal phase to a superradiant phase when the coupling strength between the two-level atoms and the optical field exceeds a critical value. Dicke model embodies unique many-body quantum theories. And it has been widely studied and obtained many significant research results in quantum information, quantum process, and other quantum systems. Meanwhile, Dicke model also has wide applications in quantum optics and condensed matter physics. The extended Dicke model, describing the interaction of a Bose-Einstein condensate in an optical cavity, provides a remarkable platform for studying extraordinary quantum phase transitions in theory and experiment. Based on the recent experiment on non-Hermitian coupling between two long-lived atomic spin waves in an optical cavity, in this work we use spin-coherent-state variational method and present the macroscopic quantum-state energy of the non-Hermitian Dicke model. The spin coherent state variational method has an advantage in the theoretical research of macroscopic quantum states, especially in the normal and the inverted pseudospin states. In the variational method, optical coherent states and atomic extremum spin coherent states are used as the trial wave functions. A Hermitian transformation operator is proposed to diagonalize the non-Hermitian Hamiltonian, which is different from the ordinary quantum mechanics where the transformation operator must be unitary. Herein, the energy function is not necessarily real in the entire coupling region. Beyond an exceptional point, the spectrum becomes complex and introducing biorthogonal sets of atomic extremum states is necessary to evaluate the average quantities. The normal phase (for the zero average photon number) possesses real energy and atomic population. The non-Hermitian interaction destroys the superradiant phase (for the stable nonzero average photon number) and leads to the absence of quantum phase transition. However, the introduced atom-photon interaction, which is induced by the pump field experimentally, can change the situation, dramatically. The pump field can balance the loss by the non-Hermitian atom-photon interaction to achieve the superradiant phase. An interesting double exceptional point are observed in the energy functional. There is the real spectrum below the first exceptional point and beyond the second exceptional point, while there is a complex spectrum between these two exceptional points. The superradiant phase appears only beyond a critical value, which is related to the nonlinear interaction and the pump laser. A new and inverted quantum phase transition from the superradiant phase to the normal phase, is observed by modulating the atom-field coupling strength. The superradiant phase of the population inversion state appears for a negative effective frequency and a large atom-photon interaction. The influence of the dissipative coupling may be observed in cold atom experiment in an optical cavity. All the parameters adopted in this work are the actual experimental parameters.