Multiphoton intrashell transitions in strongly driven Li (
n=25) Rydberg atoms are studied experimentally. Orthogonal dc electric and magnetic fields lift the degeneracy of the
n shell and define the eccentricity
e of the initial coherent elliptic states, which are formed by laser excitation and subsequent adiabatic transformation. The intrashell transitions are driven by a time-harmonic electric field linearly polarized parallel to the major axis of the ellipse.
N-photon resonances with $N=1\ensuremath{-}9$ are studied as a function of
e. All resonances with $N\ensuremath{\geqslant}3$ are suppressed at certain
e values in between
0 and
1. A similar system was analyzed by Yabuzaki et al. [Phys. Rev. A 10, 1955 (1974)] who found a simple pattern of suppressions that applies also for the present experiments. The results of these experimentally confirm that each time
N is increased by two, an additional suppression is observed.
Electron capture cross sections for coherent elliptic Rydberg states have been measured as a function of eccentricity. The ion impact velocity was parallel to the minor axis of the associated, classical elliptic orbit and both clockwise and anticlockwise orbital motion of the electron were studied. The incoming ions were 2.5 keV 23 Na + and the Rydberg target, with principal quantum number n=25, was formed by laser excitation of Li atoms with subsequent adiabatic switching of crossed, external electric and magnetic fields. A strong dependence on eccentricity and sense of orbital motion was found.