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Magic wavelengths for the State-insensitive Optical Trapping of Cs Atoms: case studies using the linearly and circularly polarized lights

Sukhjit Singh Sehra, Kiranpreet Kaur, B. K. Sahoo, Bindiya Arora

Published Jan 4, 2016• 0 citations
OpenAlex

Abstract

We demonstrate magic wavelengths for the $6s ~ {^2}S_{1/2}-6p ~ {^2}P_{3/2,1/2}$ transitions in the Cs atom due to the circularly polarized light. In addition, we also obtain magic wavelengths using the linearly polarized light in order to verify the previously reported values and make a comparative study with the values obtained for the circularly polarized light. Most of these wavelengths are found to be in the optical region and could be of immense interest to the experimentalists for carrying out high precision measurements. To obtain these wavelengths, we have calculated dynamic dipole polarizabilities of the ground, $6p ~{^2}P_{1/2}$ and $6p ~{^2}P_{3/2}$ states. We use the available precise values of the electric dipole (E1) matrix elements for the most dominantly contributing transitions from the lifetime measurements of the above excited states and obtain other relevant important E1 matrix elements by employing a relativistic coupled-cluster method approximating at the singles and doubles level. Accuracies in these quantities are substantiated by comparing our evaluated scalar polarizability values with the corresponding experimental results.

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Magic wavelengths for optical cooling and trapping of potassium

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We carry out a systematic study of the static and dynamic polarizabilities of the potassium atom using a first-principles high-precision relativistic all-order method in which all single, double, and partial triple excitations of the Dirac-Fock wave functions are included to all orders of perturbation theory. Recommended values and uncertainties are provided for the relevant electric-dipole matrix elements. Polarizabilities of the $4s$, $4{p}_{j}$, $5s$, $5{p}_{j}$, and $3{d}_{j}$ states are compared with other theoretical and experimental values when possible. We identify magic wavelengths for the $4s\ensuremath{-}np$ transitions for $n=4,5$, i.e., those wavelengths for which the two levels have the same ac Stark shifts. The magic wavelengths for the $4s\ensuremath{-}5p$ transitions are of particular interest for attaining a quantum gas of potassium at high phase-space density. We find 20 such wavelengths in the technically interesting region of $1050--1130$ nm.

Physical Review A•May 6, 2013•29 citations
We demonstrate magic wavelengths for the 6s 2S1/2−6p 2P3/2,1/26s ~ {^2}S_{1/2}-6p ~ {^2}P_{3/2,1/2}6s 2S1/2​−6p 2P3/2,1/2​ transitions in the Cs atom due to the circularly polarized light. In addition, we also obtain magic wavelengths using the linearly polarized light in order to verify the previously reported values and make a comparative study with the values obtained for the circularly polarized light. Most of these wavelengths are found to be in the optical region and could be of immense interest to the experimentalists for carrying out high precision measurements. To obtain these wavelengths, we have calculated dynamic dipole polarizabilities of the ground, 6p 2P1/26p ~{^2}P_{1/2}6p 2P1/2​ and 6p 2P3/26p ~{^2}P_{3/2}6p 2P3/2​ states. We use the available precise values of the electric dipole (E1) matrix elements for the most dominantly contributing transitions from the lifetime measurements of the above excited states and obtain other relevant important E1 matrix elements by employing a relativistic coupled-cluster method approximating at the singles and doubles level. Accuracies in these quantities are substantiated by comparing our evaluated scalar polarizability values with the corresponding experimental results.
We study the cancellation of differential ac Stark shifts in the 5s5s5s and 5p5p5p states of the rubidium atom using the linearly and circularly polarized lights by calculating their dynamic polarizabilities. Matrix elements were calculated using a relativistic coupled-cluster method at the single and double excitations and at the important valence triple excitation approximation including all possible nonlinear correlation terms. Some of the important matrix elements were further optimized using the experimental results available for the lifetimes and static polarizabilities of atomic states. ``Magic wavelengths'' are determined from the differential Stark shifts and results for the linearly polarized light are compared with the previously available results. The possible scope of facilitating state-insensitive optical trapping schemes using the magic wavelengths for circularly polarized light is discussed. Using the optimized matrix elements, the lifetimes of the 4d4d4d and 6s6s6s states of this atom are ameliorated.
Magic wavelengths for the Li, Na, and K alkali-metal atoms are determined using the circularly polarized light for the nsnsns-np1/2,3/2n{p}_{1/2,3/2}np1/2,3/2​ transitions, with nnn denoting their ground-state principal quantum numbers, by studying their differential ac dynamic polarizabilities. These wavelengths for all possible sublevels are given linearly as well as circularly polarized lights and are further compared with the available results for the linearly polarized light. The present study suggests that it is possible to carry out state-insensitive trapping of different alkali-metal atoms using the circularly polarized light.
For the trapped pre-cooled atoms in an optical dipole trap (ODT), the magic-wavelength ODT can eliminate the differential light shift of the transition between two atomic states, so that the transition frequency between the two states is the same as that of atoms in the free space, which is of great significance for improving the experimental repetition rate and reducing the atomic decoherence in the fields of cold atom physics, quantum optics, and precision measurement. Here we calculate the dynamic polarizabilities of cesium 6S ground state and 7P excited state by using the multi-level model for the ODT with laser wavelength from 1200 to 2000 nm. The magic wavelengths of ODT are obtained for the linearly and circularly polarized laser beams at the intersection of dynamic polarizabilities of two atomic states. Furthermore, we analyze the robustness of the magic trapping conditions and the feasibility of the experimental operation near the telecom C-band wavelength.
Extensive calculations of the electric-dipole matrix elements in alkali-metal atoms are conducted using the relativistic all-order method. This approach is a linearized version of the coupled-cluster method, which sums infinite sets of many-body perturbation theory terms. All allowed transitions between the lowest nsnsns, np1∕2n{p}_{1∕2}np1∕2​, np3∕2n{p}_{3∕2}np3∕2​ states and a large number of excited states are considered in these calculations and their accuracy is evaluated. The resulting electric-dipole matrix elements are used for the high-precision calculation of frequency-dependent polarizabilities of the excited states of alkali-metal atoms. We find ``magic'' wavelengths in alkali-metal atoms for which the nsnsns and np1∕2n{p}_{1∕2}np1∕2​ and np3∕2n{p}_{3∕2}np3∕2​ atomic levels have the same ac Stark shifts, which facilitates state-insensitive optical cooling and trapping.
The frequency dependent polarizabilities of the francium atom are calculated from the available data of energy levels and transition rates. Magic wavelengths for the state insensitive optical dipole trapping are identified from the calculated light shifts of the 7s7s7s 2S1/2^{2}{S}_{1/2}2S1/2​, 7p7p7p 2P1/2,3/2^{2}{P}_{1/2,3/2}2P1/2,3/2​, and 8s8s8s 2S1/2^{2}{S}_{1/2}2S1/2​ levels of the 7s7s7s $^{2}{S}_{1/2}\ensuremath{-}7p$ 2P1/2,3/2^{2}{P}_{1/2,3/2}2P1/2,3/2​ and 7s7s7s $^{2}{S}_{1/2}\ensuremath{-}8s$ 2S1/2^{2}{S}_{1/2}2S1/2​ transitions, respectively. Wavelengths in the ultraviolet, visible, and near infrared region are identified that are suitable for cooling and trapping. Magic wavelengths between the 600--700 nm and 700--1000 nm regions, which are blue and red detuned with the $7s\ensuremath{-}7p$ and $7s\ensuremath{-}8s$ transitions, are feasible to implement as lasers with sufficient power are available. In addition, we calculated the tune-out wavelengths where the ac polarizability of the ground 7s7s7s 2S1/2^{2}{S}_{1/2}2S1/2​ state in francium is zero. These results are beneficial as laser cooled and trapped francium has been in use for fundamental symmetry investigations like searches for an electron permanent electric dipole moment in an atom and for atomic parity nonconservation.
We carry out a systematic study of the static and dynamic polarizabilities of the potassium atom using a first-principles high-precision relativistic all-order method in which all single, double, and partial triple excitations of the Dirac-Fock wave functions are included to all orders of perturbation theory. Recommended values and uncertainties are provided for the relevant electric-dipole matrix elements. Polarizabilities of the 4s4s4s, 4pj4{p}_{j}4pj​, 5s5s5s, 5pj5{p}_{j}5pj​, and 3dj3{d}_{j}3dj​ states are compared with other theoretical and experimental values when possible. We identify magic wavelengths for the $4s\ensuremath{-}np$ transitions for n=4,5n=4,5n=4,5, i.e., those wavelengths for which the two levels have the same ac Stark shifts. The magic wavelengths for the $4s\ensuremath{-}5p$ transitions are of particular interest for attaining a quantum gas of potassium at high phase-space density. We find 20 such wavelengths in the technically interesting region of 1050−−11301050--11301050−−1130 nm.