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Chinese Physics Letters

Spectra of 4 2 S 1/2 →3 2 D 5/2 Transitions of a Single Trapped 40 Ca+ Ion

Shijie Gong, Fei Zhou, Haoyu Wu, Wei Wan, Liang Chen, Mang Feng

Published Jan 1, 2015• 2 citations
Publisher

Abstract

We investigate the spectra of the electric quadrupole 4 2 S 1/2 →3 2 D 5/2 transitions in a single 40 Ca + ion confined in a home-built linear trap. We probe the transitions with an ultra-narrow bandwidth laser at 729 nm. In a weak magnetic field, the quadrupole transition splits into ten components with the maximal line strength proportional to their squared Clebsch—Gordan factors. In a magnetic field of the order of Gauss, the observed equidistant sideband reflects the Zeeman substructure modulated by the quantized oscillation due to the secular motion in the trap. The temperature of the trapped ion can be determined by the envelope of the sideband spectrum. We also demonstrate the Rabi oscillation in a carrier transition after the ion has been Doppler cooled, which can be fitted by the model with the thermal state of motion.

DOI
10.1088/0256-307x/32/1/013201

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Chinese Physics Letters•Dec 1, 2010•8 citations
We investigate the spectra of the electric quadrupole 4 2 S 1/2 →3 2 D 5/2 transitions in a single 40 Ca + ion confined in a home-built linear trap. We probe the transitions with an ultra-narrow bandwidth laser at 729 nm. In a weak magnetic field, the quadrupole transition splits into ten components with the maximal line strength proportional to their squared Clebsch—Gordan factors. In a magnetic field of the order of Gauss, the observed equidistant sideband reflects the Zeeman substructure modulated by the quantized oscillation due to the secular motion in the trap. The temperature of the trapped ion can be determined by the envelope of the sideband spectrum. We also demonstrate the Rabi oscillation in a carrier transition after the ion has been Doppler cooled, which can be fitted by the model with the thermal state of motion.
A single 40Ca+{}^{40}{\mathrm{Ca}}^{+}40Ca+ ion is confined in a linear Paul trap and Doppler-cooled on the S1/2{S}_{1/2}S1/2​ to P1/2{P}_{1/2}P1/2​ dipole transition. Then the narrow quadrupole S1/2{S}_{1/2}S1/2​ to D5/2{D}_{5/2}D5/2​ transition at 729 nm is probed. The observed spectrum is interpreted in terms of the Zeeman substructure superimposed with oscillation sidebands due to the harmonic motion in the trap. The height of the motional sidebands provides a sensitive method to determine the ion's temperature and thus allows us to test sub-Doppler laser cooling schemes needed for quantum state preparation and quantum computation. We also observe the dynamics induced by Rabi oscillations on a carrier transition and interpret it in terms of the thermal state which is reached after Doppler cooling.
We perform resolved optical sideband spectroscopy on a single 40Ca+ ion in a Penning trap. We probe the electric quadrupole allowed S1/2↔D5/2 transition at 729 nm and observe equally spaced sidebands for the three motional modes. The axial mode, parallel to the trap axis, is a one-dimensional harmonic oscillator, whereas the radial cyclotron and magnetron modes are circular motions perpendicular to the magnetic field. The total energy associated with the magnetron motion is negative, but here we probe only the (positive) kinetic energy. From the equivalent Doppler widths of the sideband spectra corresponding to the three motions we find effective temperatures of 1.1±0.2 mK, 7±3 mK, and 42±8 μK for the axial, modified cyclotron, and magnetron modes, respectively. These should be compared to the cooling limits, estimated using optimal laser parameters, of 0.38 mK, 0.8 mK, and ∼10 μK. In future work we aim to perform resolved-sideband cooling of the ion on the 729-nm transition.Received 3 December 2013DOI:https://doi.org/10.1103/PhysRevA.89.032502©2014 American Physical Society
The National Institute of Information and Communications Technology in Japan is proceeding with development of an optical frequency standard using an electric quadrupole transition of Ca+ ions in a small radio-frequency trap. The single, trapped 40Ca+ ions are laser cooled to a temperature of <10 mK using extended-cavity diode lasers at 397 nm and 866 nm. In order to measure the electric quadrupole transition, the linewidth of the clock laser diode at 729 nm is reduced to ~66 Hz using an ultra-low-expansion (ULE) cavity. We observed the electric quadrupole transition with a linewidth of ~600 kHz, together with the ionic motional sidebands. We are also developing optical frequency combs without photonic fibers broadening the spectrum. The experimental is now improved in order to observe the narrower linewidth of the quadrupole transition.
We report the laser cooling of a single 40Ca+^{40}\text{Ca}^+40Ca+ ion in a Penning trap to the motional ground state in one dimension. Cooling is performed in the strong binding limit on the 729-nm electric quadrupole S1/2↔D5/2S_{1/2}\leftrightarrow D_{5/2}S1/2​↔D5/2​ transition, broadened by a quench laser coupling the D5/2D_{5/2}D5/2​ and P3/2P_{3/2}P3/2​ levels. We find the final phonon number to be nˉ=0.014±0.009\bar{n}=0.014\pm0.009nˉ=0.014±0.009. We measure the heating rate of the trap to be very low with nˉ˙=2.5±0.3s−1\dot{\bar{n}}=2.5\pm 0.3\textrm{s}^{-1}nˉ˙=2.5±0.3s−1 and a scaled spectral noise density of ωSE(ω)∼1.6−8V2m−2Hz−1s−1\omega S_{E}(\omega)\sim1.6^{-8}\textrm{V}^2\textrm{m}^{-2}\textrm{Hz}^{-1}\textrm{s}^{-1}ωSE​(ω)∼1.6−8V2m−2Hz−1s−1, which is consistent with the large ion-electrode distance. We perform Rabi oscillations on the sideband-cooled ion and observe a coherence time of 0.7±0.1ms0.7\pm 0.1\textrm{ms}0.7±0.1ms, noting that the practical performance is currently limited by the intensity noise of the probe laser.
We experimentally demonstrate laser spectroscopy of the electric-quadrupole transition 6s2S1/2−−5d2D3/26s{}^{2}{S}_{1/2}--5d{}^{2}{D}_{3/2}6s2S1/2​−−5d2D3/2​ of a single trapped 171Yb{}^{171}\mathrm{Yb}171Yb ion. The probed transition has a natural linewidth of 3.1 Hz, and is at a wavelength of 435.5 nm. A 171Yb{}^{171}\mathrm{Yb}171Yb ion is laser cooled to the range of the Doppler limit in a radio-frequency Paul trap. The $F=0--{F}^{\ensuremath{'}}=2,$ ${m}_{{F}^{\ensuremath{'}}}=0$ hyperfine component of the 2S1/2−−2D3/2{}^{2}{S}_{1/2}{--}^{2}{D}_{3/2}2S1/2​−−2D3/2​ transition is excited by a laser source whose frequency is controlled by an optical reference cavity of high intrinsic stability. The recoilless carrier component of the vibrational sideband spectrum is resolved with a minimum linewidth of approximately 80 Hz, corresponding to a fractional frequency resolution of $1.2\ifmmode\times\else\texttimes\fi{}{10}^{\ensuremath{-}13}.$ This resolution limit is attributed to laser frequency instability. The effective decoherence rates of the residual ion motion are inferred from the observation that the axial and two radial low-frequency first-order secular-vibration sidebands show minimum linewidths in the range of 0.2--1 kHz. Prospects for an optical frequency standard based on the investigated atomic system are discussed.