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Chinese Physics B

Highly efficient four-wave mixing induced by quantum constructive interference in rubidium vapour

Gang Wang, Yan Xue, Cui-Li Cui, Yi Qu, Jin-Yue Gao

Published Mar 1, 2012• 10 citations
Publisher

Abstract

We demonstrate efficient four-wave mixing with an intensity conversion efficiency of nearly 100% in theory without considering the Doppler-broadening effect in a four-level double-Λ system of hot 87 Rb gas. The corresponding experimental value of about 73% was reported in our earlier work under the same conditions. This dramatic efficiency is critically dependent on the constructive interference between two four-wave mixing processes relevant to the internally generated four-wave mixing signal.

DOI
10.1088/1674-1056/21/3/034205

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Optics Express•Oct 18, 2011•8 citations
We demonstrate efficient four-wave mixing with an intensity conversion efficiency of nearly 100% in theory without considering the Doppler-broadening effect in a four-level double-Λ system of hot 87 Rb gas. The corresponding experimental value of about 73% was reported in our earlier work under the same conditions. This dramatic efficiency is critically dependent on the constructive interference between two four-wave mixing processes relevant to the internally generated four-wave mixing signal.
In a four-level system of ultracold 87 Rb atoms, through analytical and numerical calculations we propose an efficient scheme to achieve the enhanced four-wave mixing process and demonstrate its dynamical control by various parameters such as the travel distance z , probe detuning δ and the probe pulse width τ. In particular, we find that the maximal intensity of the nonlinearly generated signal pulse can be about 80% of the initial input probe under the optimal condition. This greatly enhanced conversion efficiency occurs due to the constructive quantum interference between two different components of the generated signal pulse.
Electromagnetically-induced-transparency-based four-wave mixing (FWM) in a resonant four-level double-Λ system has a maximum conversion efficiency (CE) of 25% due to spontaneous emission. Herein, we demonstrate that spontaneous emission can be considerably suppressed by arranging the applied laser beams in a backward configuration. With the backward double-Λ FWM scheme, we observe a CE of 63% in cold rubidium atoms with an optical depth (OD) of 48. To the best of our knowledge, this is the first observation of a CE exceeding the conversion limit in resonant FWM processes. Furthermore, we present a theoretical model that includes the phase-mismatch effect in the backward double-Λ FWM system. According to the theoretical model, the present scheme can achieve 96% CE using a medium with a large OD of 200 under ideal conditions. Such an efficient frequency conversion scheme has potential applications in optical quantum information technology.
We observed electromagnetically induced transparency-based four-wave mixing (FWM) in the pulsed regime at low light levels. The FWM conversion efficiency of 3.8(9)3.8(9)%3.8(9) was observed in a four-level system of cold 87Rb{}^{87}\mathrm{Rb}87Rb atoms using a driving laser pulse with a peak intensity of $\ensuremath{\approx}80$ $\ensuremath{\mu}\mathrm{W}/{\mathrm{cm}}^{2}$, corresponding to an energy of $\ensuremath{\approx}60$ photons per atomic cross section. Comparison between the experimental data and the theoretical predictions proposed by Harris and Hau [Phys. Rev. Lett. 82, 4611 (1999)] showed good agreement. Additionally, a high conversion efficiency of 46(2)46(2)%46(2) was demonstrated when applying this scheme using a driving laser intensity of $\ensuremath{\approx}1.8$ mW/cm2\mathrm{mW}/{\mathrm{cm}}^{2}mW/cm2. According to our theoretical predictions, this FWM scheme can achieve a conversion efficiency of nearly 100100%100 when using a dense medium with an optical depth of 500.
In this work, we present a set of experiments involving four-wave mixing processes in rubidium atoms. We employ several experimental configurations exploring two- and three-level systems in cascade or Λ configurations, all of which are in a copropagating geometry, to investigate different physical phenomena present in each scenario. In the first experiment, we combine a cw diode laser and a 1 GHz femtosecond pulse train to generate coherent blue light through the four-wave mixing process in hot rubidium vapor. The generated coherent signal is analyzed by scanning either the diode frequency or the repetition rate of the frequency comb. In both cases, the cw laser induces an Autler- Townes splitting with a wide separation in the doublet structure due to the configuration of copropagating fields. To model these results, we employ the density matrix formalism to write the Bloch equations and solve them numerically. The solutions allow us to explore other cases beyond those involving our experimental setup, comparing the response of the upper-level population and the generated signal coherence for homogeneously and non-homogeneously broadened systems. Moreover, in this same experiment, we also observed an unexpected interference effect between excitation routes of the four-wave mixing process when the repetition rate of the pulse train is scanned. The theoretical model demonstrates that the interfering effect appears only when the repetition rate is carefully chosen to produce a pair of modes of the frequency comb resonant with both one- and two-photon transitions for the same atomic velocity group. In the second experiment, still with a hot rubidium vapor, we explore two symmetrical degenerate four- wave mixing signals induced by two almost copropagating laser beams, with~ka and~kb wave-vectors, and detected simultaneously in the 2~ka −~kb and 2~kb −~ka directions. Each spectrum has a single peak with a short frequency separation between them, which our model indicates is due to the nonlinear behavior of the refractive indexes, a consequence of the high intensity of both input fields. Finally, we use the same experimental setup for the two symmetrical signals to study the field intensity fluctuations of the degenerate four-wave mixing signals and the transmission signals. In this case, the sample is an ensemble of cold rubidium atoms in a magneto-optical trap. There is an intensity- intensity cross-correlation between the signals due to the resonant phase-noise to amplitude-noise conversion. In this type of cold system, we can neglect the Doppler- broadening, allowing a straightforward study of the dependency of the correlations on the laser detuning. In these measurements, we observe a type of oscillation in the correlation curves that the theoretical model indicates to be connected with Rabi oscillations, revealed by the fluctuations long after the transient period.
We extend the study on a four-wave mixing (FWM) scheme of contiuous-wave lasers in a hot rubidium vapor when the probe and coupling fields work in the electromagnetically induced transparency (EIT) regime while the pump and signal fields work in the two-photon Raman regime. Our experimental results show that the generated signal field is well contained in an EIT dip of the incident probe field as a result of efficient FWM. We find, in particular, that an optimal FWM process can only be attained when the coupling and pump fields are well matched in intensity. If the probe intensity is far beyond the EIT condition, however, the nonlinear efficiency of energy transfer from the probe field to the signal field will be greatly reduced.