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Advances in magnetic and optical resonance

Long-Time Limitations of the Average Hamiltonian Theory: A Dressed-States Viewpoint

M. Matti Maricq

Published Jan 1, 1990• 29 citations
Publisher
DOI
10.1016/b978-0-12-025514-6.50013-7

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Quantum transitions and dressed unstable states

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We consider the problem of the meaning of quantum unstable states including their dressing. According to both Dirac and Heitler this problem has not been solved in the usual formulation of quantum mechanics. A precise definition of excited states is still needed to describe quantum transitions. We use our formulation given in terms of density matrices outside the Hilbert space. We obtain a dressed unstable state for the Friedrichs model, which is the simplest model that incorporates both bare and dressed quantum states. The excited unstable state is derived from the stable states through analytic continuation. It is given by an irreducible density matrix with broken time symmetry. It can be expressed by a superposition of Gamow density operators. The main difference from previous studies is that excited states are not factorizable into wave functions. The dressed unstable state satisfies all the criteria that we can expect: it has a real average energy and a nonvanishing trace. The average energy differs from Green's function energy by a small effect starting with fourth order in the coupling constant. Our state decays following a Markovian equation. There are no deviations from exponential decay neither for short nor for long times, as is the case for the bare state. The dressed state satisfies an uncertainty relation between energy and lifetime. We can also define dressed photon states and describe how the energy of the excited state is transmitted to the photons. There is another very important aspect: deviations from exponential decay would be in contradiction with indiscernibility as one could define, e.g., old mesons and young mesons according to their lifetime. This problem is solved by showing that quantum transitions are the result of two processes: a dressing process, discussed in a previous publication, and a decay process, which is much slower for electrodynamic systems. During the dressing process the unstable state is prepared. Then the dressed state decays in a purely exponential way. In the Hilbert space the two processes are not separated. Therefore it is not astonishing that we obtain for the unstable dressed state an irreducible density matrix outside the Liouville-Hilbert-space. This is a limit of Hilbert space states that are arbitrarily close to the decaying state. There are experiments that could verify our proposal. A typical one would be the study of the line shape, which is due to the superposition of the short-time process and the long-time process. The long-time process taken separately leads to a much sharper line shape, and avoids the divergence of the fluctuation predicted by the Lorentz line shape.

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Theory of dressed-state lasers in the bad-cavity limit

Jakub Zakrzewski, Maciej Lewenstein

We present a theory of dressed-state lasers, i.e., lasers that operate on an inverted transition between dressed states of a coupled atom-field system, in the bad-cavity limit. We discuss the validity of the effective Hamiltonian approach in such a case and generalize the theory beyond secular and effective Hamiltonian approximations. We demonstrate that higher-order instabilities that lead to self-pulsing and optical chaos may occur in experiments on dressed-state lasers. With the help of the generalized theory we study the competition between the resonant one-photon and two-photon processes and try to understand it physically by looking at the spectrum of the emitted radiation.

Physical Review A•Feb 1, 1992•21 citations
We show that Floquet states can be constructed as strong-field limits of cavity-dressed states. The interaction between laser beams propagating outside the cavity with atoms or molecules are described by Floquet states, constructed from dressed states of average photon number quantized in a cavity of volume V, by taking the limit , , while keeping the photon density constant. Thus, Floquet theory can be seen as a fully quantum-mechanical model in the sense that it describes the photon exchanges between matter and radiation containing a large amount of photons. We discuss in this context adiabatic Floquet theory to treat a slow time dependence of the laser amplitude, to describe pulses, and of its frequency (chirping).
We consider the problem of the meaning of quantum unstable states including their dressing. According to both Dirac and Heitler this problem has not been solved in the usual formulation of quantum mechanics. A precise definition of excited states is still needed to describe quantum transitions. We use our formulation given in terms of density matrices outside the Hilbert space. We obtain a dressed unstable state for the Friedrichs model, which is the simplest model that incorporates both bare and dressed quantum states. The excited unstable state is derived from the stable states through analytic continuation. It is given by an irreducible density matrix with broken time symmetry. It can be expressed by a superposition of Gamow density operators. The main difference from previous studies is that excited states are not factorizable into wave functions. The dressed unstable state satisfies all the criteria that we can expect: it has a real average energy and a nonvanishing trace. The average energy differs from Green's function energy by a small effect starting with fourth order in the coupling constant. Our state decays following a Markovian equation. There are no deviations from exponential decay neither for short nor for long times, as is the case for the bare state. The dressed state satisfies an uncertainty relation between energy and lifetime. We can also define dressed photon states and describe how the energy of the excited state is transmitted to the photons. There is another very important aspect: deviations from exponential decay would be in contradiction with indiscernibility as one could define, e.g., old mesons and young mesons according to their lifetime. This problem is solved by showing that quantum transitions are the result of two processes: a dressing process, discussed in a previous publication, and a decay process, which is much slower for electrodynamic systems. During the dressing process the unstable state is prepared. Then the dressed state decays in a purely exponential way. In the Hilbert space the two processes are not separated. Therefore it is not astonishing that we obtain for the unstable dressed state an irreducible density matrix outside the Liouville-Hilbert-space. This is a limit of Hilbert space states that are arbitrarily close to the decaying state. There are experiments that could verify our proposal. A typical one would be the study of the line shape, which is due to the superposition of the short-time process and the long-time process. The long-time process taken separately leads to a much sharper line shape, and avoids the divergence of the fluctuation predicted by the Lorentz line shape.
We present a theory of dressed-state lasers, i.e., lasers that operate on an inverted transition between dressed states of a coupled atom-field system, in the bad-cavity limit. We discuss the validity of the effective Hamiltonian approach in such a case and generalize the theory beyond secular and effective Hamiltonian approximations. We demonstrate that higher-order instabilities that lead to self-pulsing and optical chaos may occur in experiments on dressed-state lasers. With the help of the generalized theory we study the competition between the resonant one-photon and two-photon processes and try to understand it physically by looking at the spectrum of the emitted radiation.