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Chinese Physics Letters

Non-Classical Correlated Photon Pairs Generation via Cascade Transition of 5S1/2–5P3/2–5D5/2in a Hot85Rb Atomic Vapor

Wei Zhang, Dong-Sheng Ding, Jian-Song Pan, Bao-Sen Shi

Published Jun 1, 2014• 10 citations
Publisher

Abstract

We experimentally prepare the non-classical correlated photon pairs at the wavelengths of 780 and 776 nm via the cascade transition of 5S 1/2 –5P 3/2 –5D 5/2 in a hot 85 Rb atomic ensemble. By measuring the function of cross-correlation and auto-correlation of photons, a violation of Cauchy—Schwarz inequality by a factor of 283 is obtained, which clearly indicates a strong non-classical correlation between the generated photons. We also find that noise photons scattered from pump lasers have a strong effect on the Cauchy—Schwarz inequality factor by changing the intensity of the pump laser, the experimental results are consistent with the theoretical predictions.

DOI
10.1088/0256-307x/31/6/064208

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We experimentally prepare the non-classical correlated photon pairs at the wavelengths of 780 and 776 nm via the cascade transition of 5S 1/2 –5P 3/2 –5D 5/2 in a hot 85 Rb atomic ensemble. By measuring the function of cross-correlation and auto-correlation of photons, a violation of Cauchy—Schwarz inequality by a factor of 283 is obtained, which clearly indicates a strong non-classical correlation between the generated photons. We also find that noise photons scattered from pump lasers have a strong effect on the Cauchy—Schwarz inequality factor by changing the intensity of the pump laser, the experimental results are consistent with the theoretical predictions.
We experimentally generate a non-classical correlated two-color photon pair at 780 and 1529.4 nm in a ladder-type configuration using a hot 85Rb atomic vapor with the production rate of ~10(7)/s. The non-classical correlation between these two photons is demonstrated by strong violation of Cauchy-Schwarz inequality by the factor R = 48 ± 12. Besides, we experimentally investigate the relations between the correlation and some important experimental parameters such as the single-photon detuning, the powers of pumps. We also make a theoretical analysis in detail and the theoretical predictions are in reasonable agreement with our experimental results.
We report on a source of narrowband pairs of time-correlated photons generated via four-wave mixing in a laser-cooled atomic ensemble of87Rb atoms. We employ a cascade decay level scheme in which two copropagating pump beams of 780nm and 776nm excite the atoms to the 5D3/2, F = 3 level and the photon pairs of wavelength 762nm and 795nm from the cascade decay are coupled into single mode fibers and sent to silicon avalanche photodetectors. The photodetection events exhibit a strong correlation in time (g(2)(τ = 0) ≈ 5800), and a high coupling efficiency, as indicated by a pair-to-single ratio of 23%. An instantaneous pair generation rate of 7700 pairs per second (uncompensated for optical losses and detector efficiency) is observed with an increased 776nm pump power of 14mW. The violation of the Cauchy-Schwarz inequality by a factor of 8.4 × 106indicates a strong non-classical correlation between the generated fields, while a Hanbury-Brown-Twiss experiment in the individual photons reveals their thermal nature.
A scheme for the generation of nonclassical pairs of photons in atomic vapors is proposed. The scheme exploits the fact that the cross correlation of the emission of photons from the extreme transitions of a four-level cascade system shows antibunching, unlike the case of the three-level cascade emission, which shows bunching. The Cauchy-Schwarz inequality, which is the ratio of the cross-correlation to the autocorrelation function, in this case is estimated to be 103−−106{10}^{3}--{10}^{6}103−−106 for controllable time delay, and is one to four orders of magnitude larger compared to previous experiments. The choice of Doppler-free geometry, in addition to the fact that at three-photon resonance the excitation and deexcitation processes occur in a very narrow frequency band, ensures cleaner signals.