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Springer eBooks

G(2)(0) and the Two-Photon Transition Rate: An Experimental Study

M. Rankin, Jon P. Davis, Christopher Giranda, M. Squicciarini, Lloyd C. Bobb

Published Jan 1, 1990• 0 citations
Publisher
DOI
10.1007/978-1-4613-0847-8_175

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The photon statistics of several different laser systems operating at 226 nm are probed by measuring absolutely the fluorescence following two-photon absorption in atomic oxygen. The integrated fluorescence, obtained by scanning the laser frequency through the two-photon resonance, is theoretically shown to be proportional to G(2) (0) σ0(2). The second-order intensity-correlation function at time zero, G(2)(0), characterizes the laser, and σ0(2) is a fundamental atomic property. Measurement of the integrated fluorescence permits determination of the relative value of G(2) (0) for each laser. The assumption that G(2)(0) = 1 for one of the lasers, a single-frequency source, allows G(2)(0) for the other lasers to be placed on an absolute scale. The values thereby obtained range from 0.8 ± 0.2 to 3.2 ± 0.4. Different values are obtained when the radiation is generated by frequency mixing or Raman shifting of the same frequency-doubled visible dye laser, suggesting that frequency-conversion processes have a significant effect on G(2)(0).

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VARIOUS APPROACHES TO PHOTON ANTIBUNCHING IN SECOND-HARMONIC GENERATION 1

Adam Miranowicz, J. Bajer

We analyze the most popular approaches to photon antibunching as exemplified in a sim-ple model of second-harmonic generation. We find the exact evolution of the fundamental and harmonic fields for initial Fock states with small photon numbers. We show explicitly that definitions of photon antibunching based on the unnormalized, G(2)(t, t′), and normal-ized, g(2)(t, t′), two-time correlation functions describe distinct phenomena for nonstationary fields. For completeness, we also compare antibunching effects defined by the two-time and single-time correlations. 1 Photon antibunching Photon antibunching and sub-Poisson photon statistics (also called antibunching) reveal the quan-tum nature of light and therefore have received a great deal of attention during the last decades. The first detection of antibunched light by Kimble, Dagenais and Mandel [1] and first detection of sub-Poisson light by Short and Mandel [2] are regarded as milestones in the progress in quantum optics. In spite of many experimental and theoretical achievements, a deeper analysis of these effects seems to be necessary, particularly in the case of nonstationary fields. We shall clarify some of these aspects by referring to an example of second-harmonic generation. There are several commonly used definitions of photon antibunching for a single-mode radiation field (e.g., Refs. [1]–[9]): Definition I: The photon antibunching (see, e.g., Ref. [3]) occurs if the two-time light intensity correlation function G(2)(t, t+ τ) increases from its initial value at τ = 0,

•Jan 1, 1998•1 citation

Adiabatic Following in Two-Photon Transition

Munir Hasan Nayfeh, Ali Hasan Nayfeh

Springer eBooks•Jan 1, 1978•0 citations
The photon statistics of several different laser systems operating at 226 nm are probed by measuring absolutely the fluorescence following two-photon absorption in atomic oxygen. The integrated fluorescence, obtained by scanning the laser frequency through the two-photon resonance, is theoretically shown to be proportional to G(2) (0) σ0(2). The second-order intensity-correlation function at time zero, G(2)(0), characterizes the laser, and σ0(2) is a fundamental atomic property. Measurement of the integrated fluorescence permits determination of the relative value of G(2) (0) for each laser. The assumption that G(2)(0) = 1 for one of the lasers, a single-frequency source, allows G(2)(0) for the other lasers to be placed on an absolute scale. The values thereby obtained range from 0.8 ± 0.2 to 3.2 ± 0.4. Different values are obtained when the radiation is generated by frequency mixing or Raman shifting of the same frequency-doubled visible dye laser, suggesting that frequency-conversion processes have a significant effect on G(2)(0).
We demonstrate spectral amplitude and phase modulation of time-energy entangled photon pairs by means of a spatial light modulator (SLM) [1]. Coincidences are detected by sum frequency generation in a nonlinear crystal which has been applied in several experiments as an ultrafast coincidence detection method to temporally resolve entangled photons on a timescale of fs [2,3]. By taking into account the properties of the detection crystal, we derive an expression for the up-converted frequency signal in the form of a second-order correlation function G(1)[3]. This detection scheme is in contrast to a perfect coincidence detection described by the fourth-order correlation function G(2). However, in former two photon shaping experiments [1,2] the detected signal was compared to simulations based on G(2). We investigate here under which conditions the G(2)ceases to provide an accurate description of the measurements.
We analyze the most popular approaches to photon antibunching as exemplified in a sim-ple model of second-harmonic generation. We find the exact evolution of the fundamental and harmonic fields for initial Fock states with small photon numbers. We show explicitly that definitions of photon antibunching based on the unnormalized, G(2)(t, t′), and normal-ized, g(2)(t, t′), two-time correlation functions describe distinct phenomena for nonstationary fields. For completeness, we also compare antibunching effects defined by the two-time and single-time correlations. 1 Photon antibunching Photon antibunching and sub-Poisson photon statistics (also called antibunching) reveal the quan-tum nature of light and therefore have received a great deal of attention during the last decades. The first detection of antibunched light by Kimble, Dagenais and Mandel [1] and first detection of sub-Poisson light by Short and Mandel [2] are regarded as milestones in the progress in quantum optics. In spite of many experimental and theoretical achievements, a deeper analysis of these effects seems to be necessary, particularly in the case of nonstationary fields. We shall clarify some of these aspects by referring to an example of second-harmonic generation. There are several commonly used definitions of photon antibunching for a single-mode radiation field (e.g., Refs. [1]–[9]): Definition I: The photon antibunching (see, e.g., Ref. [3]) occurs if the two-time light intensity correlation function G(2)(t, t+ τ) increases from its initial value at τ = 0,