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NATO ASI series. Series B : Physics

Silver Atoms Isolated in Rare Gas Crystals: Time Resolved Investigation of Excited State Dynamics

R. Kometer

Published Jan 1, 1994• 0 citations
Publisher
DOI
10.1007/978-1-4899-1190-2_34

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Narrow excitation features present on the [Ar]3d64s1aD(J=9∕2−1∕2)6←[Ar]3d54s2aS1∕26 transitions of manganese atoms isolated in solid Kr are analyzed within the framework of weak crystal field splitting. Use of the Wp optical lineshape function allowed identification of multiple zero-phonon lines for individual spin-orbit J states of the a aD6←aS6 transition recorded with laser-induced excitation spectroscopy. Excellent agreement exists between the predicted crystal field splitting patterns for the J levels of the aD6 state isolated in the «red» tetravacancy site of solid Kr. The tetrahedral crystal field of the «red» trapping site splits J>3∕2 levels of the aDJ6 and aD7∕24 states by approximately 30cm−1. This report represents the first definitive evidence of crystal field splitting, induced by the weak van der Waals interactions between a neutral metal atom and the rare gas atoms surrounding it in a well-defined solid-state site.
We describe the basic principles underlying resonant nonlinear magneto-optical spectroscopy of alkali atoms and show how the technique can be applied for high resolution investigations of weak and strongly suppressed processes in spin coherent atomic ensembles. We illustrate this by a detailed discussion of four distinct applications, viz. the detection of small biomagnetic fields, the space and time resolved tomographic study of gas phase diffusion, the measurement of linear and quadratic Stark effects in atomic ground states and the study of (quantum) crystal field effects on solid helium-isolated atomic defect structures.