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Brazilian Journal of Physics

Non-Linear Excit at ions in Antiferromagnet ic C hains

Antonio S. T. Pires, M. E. Gouvêa

Published Jan 1, 1992• 6 citations
OpenAlex

Abstract

RRcent theoretical and experimental results on non-linear excitations in one dimensional classical antiferromagnetic chains are reviewed with a particular emphasis on dynamic properties. The main investigated substance is TMMC which can be regarded as a quasi-onedimensional antiferromagnet with easy plane anisotropy. A discussion of Haldane's conjecture that there is an excitation gap for integer, but not half-integer spin is given. The open questions and possible investigation for the future are discussed.

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Haldane Gap in the Spin-1/2Double Chain Anisotropic Heisenberg Antiferromagnet

Kazuo Hida

The double chain Heisenberg antiferromagnet with anisotropy is studied using the mapping onto the coupled anisotropic nonlinear σ model. This model consists of two anisotropic antiferromagnetic quantum Heisenberg chains with half-integer spin coupled with each other via the ferromagnetic interchain coupling J '. For small J ', our analysis suggests that J ' is an irrelevant parameter and consequently the two chains behave independently and no gap is generated. On the other hand, for large enough J ', the two chains behave as a single Heisenberg chain with integer spin which has a gap in the excitation spectrum. The expected behavior in the isotropic limit is also discussed.

Journal of the Physical Society of Japan•Jun 15, 1991•13 citations
RRcent theoretical and experimental results on non-linear excitations in one dimensional classical antiferromagnetic chains are reviewed with a particular emphasis on dynamic properties. The main investigated substance is TMMC which can be regarded as a quasi-onedimensional antiferromagnet with easy plane anisotropy. A discussion of Haldane's conjecture that there is an excitation gap for integer, but not half-integer spin is given. The open questions and possible investigation for the future are discussed.
Integer-spin Heisenberg antiferromagnetic chains are expected to have a singlet groundstate and a gap to the first excited state, as first argued by Haldane. We review rigorous results on this conjecture and discuss experimental realizations. Theoretical and experimental aspects of three recent developments in this field are then reviewed: chainend excitations and the non-local order parameter, a field theory mapping and behavior near zero wave-vector, high-field behavior and one-dimensional Bose condensation.
The authors study the dynamic spin correlation function of a spin-1 antiferromagnetic chain with easy-plane single-ion anisotropy. They use exact diagonalization by the Lanczos method for chains of length up to N=16 spins. They show that a single-mode approximation is an excellent description of the dynamical properties. A variational calculation allows them to clarify the nature of the excitations. The existence of a two-particle continuum near-zero wavevector is clearly seen, both in finite-size effects and in the dynamical structure factor. The recent neutron scattering experiments on the quasi-one-dimensional antiferromagnet NENP are fully explained by the results.
A full description of a series of spin-wave measurements in CsNiCl3{\mathrm{CsNiCl}}_{3}CsNiCl3​ in the three-dimensional (3D) and one-dimensional (1D) phases and their analysis to provide the first experimental evidence for the Haldane gap is presented. Neutron scattering experiments were performed on a single crystal of CsNiCl3{\mathrm{CsNiCl}}_{3}CsNiCl3​ with both (h,0,l) and (h,h,l) as the scattering plane. The order parameter in both 3D phases was measured and the spin-wave dispersion determined in the lower phase. The spin-wave spectrum calculated from a dynamic susceptibility method was compared with the experimental response in the lower 3D phase to obtain the following values for the exchange and anisotropy constants: J=0.345\ifmmode\pm\else\textpm\fi{}0.008 THz, J'=0.0060\ifmmode\pm\else\textpm\fi{}0.005 THz, and D=-0.0130\ifmmode\pm\else\textpm\fi{}0.0015 THz. These parameters confirm that CsNiCl3{\mathrm{CsNiCl}}_{3}CsNiCl3​ in its disordered phase is a good approximation to a one-dimensional Heisenberg antiferromagnet. In the 1D phase the gap frequency for an isolated chain of Ni2+{\mathrm{Ni}}^{2+}Ni2+ ions is found to be 0.32 THz close to the gap estimated in finite-chain calculations. The results constitute experimental support for the Haldane conjecture that the excitations of integer-spin chains, unlike half-integer--spin chains, exhibit an apparent anisotropy that arises not from the underlying isotropic Hamiltonian, but from many-body effects.
In the present work low energy excitations in various antiferromagnetic systems are investigated.The first part is devoted to the antiferromagnetic Heisenberg chain with two different alternating magnetic ions having spins S A and S B .The system can be characterised as a ferrimagnet with a long range ordered ground state.Linear spin wave theory (LSWT) leads to a qualitatively correct description of two excitation branches.The low energy spectrum contains ferromagnetic magnons which are discussed in the introductory chapter.The LSWT results are compared with the numerical data from exact diagonalisation for the case S A =1 and S B =1/2.In the second part of the thesis, the quantum phase transitions from the Néel phase to the Heisenberg phase and from the Néel phase to the Haldane phase for half-odd-integer spins S =1 /2, 3/2 and integer spins S =1 , 2, respectively, are studied in context of the Haldane conjecture.The models are analysed by means of high-order series expansions for the ground state properties and excitation energies.The expansion parameter is the anisotropy λ where the unperturbed case λ =0corresponds to the Ising model.For the integer-S systems the following scenario is obtained: The phase transitions from the Néel phase to the Haldane phase are determined by the condensation of the so-called spin zero defects (SZD) at finite anisotropy.These domain wall type excitations can be characterised as S z =0states embedded in the antiferromagnetic order.The critical exponents β of the order parameter and η of the correlation function are those of the two-dimensional Ising model.In contrast to the above scenario, the half-odd-integer S =1/2 chain undergoes the Kosterlitz-Thouless phase transition at the isotropic point.In the case of the S =3/2 chain the critical behaviour of the static structure factor S (zz) (π) is consistent with the exponentially divergent correlation length at the isotropic point.Finally, kink excitations of the S =1 /2 Heisenberg antiferromagnet chain with nearest and next nearest neighbour interactions (the zigzag chain) are investigated.Here a kink is defined as a free spin S =1 /2 mediating two dimerised ground states.The phase diagram of the zigzag chain contains the Majumdar-Ghosh model as well as the S =1/2 spin ladder and the S =1Heisenberg antiferromagnet.Starting from the Majumdar-Ghosh model, a two-kink variational wave function with S tot =1is constructed.The variational parameter is the characteristic distance between the two kinks.The variational wave function describes the low energy triplet excitation of the gapped zigzag chain in a qualitatively correct way.Within this approach, the elementary excitation of the spin ladder as well as the Haldane triplet of the S =1chain appears as a bound state of two kinks.The phase diagram of the zigzag chain contains the incommensurate phase where the wave vector of the lowest mode k 0 runs from k 0 =0to k 0 = π.At the qualitative level, this behaviour is correctly described by the variational approach.
The double chain Heisenberg antiferromagnet with anisotropy is studied using the mapping onto the coupled anisotropic nonlinear σ model. This model consists of two anisotropic antiferromagnetic quantum Heisenberg chains with half-integer spin coupled with each other via the ferromagnetic interchain coupling J '. For small J ', our analysis suggests that J ' is an irrelevant parameter and consequently the two chains behave independently and no gap is generated. On the other hand, for large enough J ', the two chains behave as a single Heisenberg chain with integer spin which has a gap in the excitation spectrum. The expected behavior in the isotropic limit is also discussed.