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Resonantly Enhanced Four-Wave Parametric

Michael J. Pellin, James T. Yardley

Published Jan 1, 1977• 0 citations
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Abstract

The pump intensity required to achieve operation of an optical parametric oscillator based upon a resonantly enhanced four- wave mixing process is examined. The effects of a finite phase mismatch and of absorption of the generated waves are treated. Numexical calculations for an atomic system ma) and two molecular systems (HQ, CO) reveal acceptably low pump intensity requirements and suggest that such a device is potentidly an efficient, scalable source of tunable coherent radiation.

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Journal of the Optical Society of America B•Aug 1, 1990•5 citations
The pump intensity required to achieve operation of an optical parametric oscillator based upon a resonantly enhanced four- wave mixing process is examined. The effects of a finite phase mismatch and of absorption of the generated waves are treated. Numexical calculations for an atomic system ma) and two molecular systems (HQ, CO) reveal acceptably low pump intensity requirements and suggest that such a device is potentidly an efficient, scalable source of tunable coherent radiation.
A theoretical investigation is made of parametric generation of light by four-wave mixing in an optical cavity with two pump fields of different frequencies. Mixing configurations resulting in the excitation of one and three cavity modes are considered taking into account the effects of phase modulation and of depletion of the pump fields. An analysis is made of stable steady-state oscillation regimes. Calculations are reported of the intensities of the generated radiation modes at the exit from the cavity above the threshold. An analysis is made of the conditions for the appearance of optical bistability at nonzero values of the cavity detuning.
The effect of electromagnetically induced transparency in resonant four-wave-mixing schemes is investigated in an analysis that goes beyond perturbation theory in the coherent driving field. In addition we examine the case where the two-photon pump field is sufficiently strong to necessitate a nonperturbative treatment. This allows us to examine the cases where either one or both of the driving fields are strong. Phase matching is included in a plane-wave propagation treatment that matches the situation most likely to be encountered in actual experiments. The calculations are in part intended to model real experimental situations and thus incorporate driving and pump-field linewidths via the phase-diffusion model and Doppler broadening. With a strong pump-field laser, large enhancements in the efficiency of light generation occur at frequencies corresponding to the Autler-Townes satellites induced by the strong driving field. In this situation gain and high four-wave-mixing efficiency are simultaneously present, resulting in the production of a large intensity of coherent radiation. \textcopyright{} 1996 The American Physical Society.
A theoretical investigation is made of parametric generation of light by four-wave mixing in an optical cavity with two pump fields of different frequencies. Mixing configurations resulting in the excitation of one and three cavity modes are are considered taking into account the effects of phase modulation and ef depletion of the pump fields. An analysis is made of stable steady-state oscillation regimes. Calculations are reported or the intensities of the generated radiation modes at the exit from the cavity above the threshold. An analysis is made of the conditions for the appearance of optical bistability at nonzero values of the cavity detuning.
A detailed model of two-photon-resonant four-wave mixing that includes the consideration of efficiency-limiting processes is presented. The model provides a generally applicable systematic approach for maximizing conversion efficiencies for both exact and near two-photon resonance. For exact two-photon resonance, an interference effect limits efficiency to a value determined by ratios of nonlinear susceptibilities and input intensities. For near two-photon resonance, nonlinear refractive indices limit efficiencies unless input intensities are properly balanced. For the specific case of 130.2-nm generation in Hg, we examine a number of potential additional efficiency-limiting processes, including amplified spontaneous emission, stimulated Raman and hyper-Raman gain, parametric gain, linear absorption, and population transfer. We include isotopic effects and Gaussian-profile beams. From our analysis, we conclude that efficiencies of approximately 10% should be feasible by using collimated light beams in an energy-scalable system.
We have developed a theory for nondegenerate oscillations in optical resonators containing an intracavity phase-conjugate element. The phase-conjugate element consists of a nonlinear transparent medium that is pumped externally by a pair of counterpropagating laser beams of the same frequency and intensity. Phase conjugation of an input beam of slightly different frequency occurs because of nondegenerate four-wave mixing. The theory takes into account linear absorption (or gain) in the medium and is applied to study the threshold behavior of phase-conjugate oscillators. For the special case of no conventional mirrors, the phase-conjugate oscillator reduces to an ordinary phase-conjugate mirror, and our general formulation yields the results of previous studies. Our analysis shows that the parametric gain required for oscillation increases (or decreases) as a result of linear absorption (or gain) in the medium, and oscillation can occur at a frequency different from that of the pump beams in the presence of large linear gain (or loss). The effects of linear absorption (or gain) on the filter operation are also examined.