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Generation ofSingle Photons ofAlternating Polarization

Tatjana Wilk, Holger Specht

Published Jan 1, 2005• 0 citations
OpenAlex

Abstract

Wepresent first results ofsingle-photon generation fromanatom-cavity system, where Ramantransitions aredriven between Zeeman sublevels. Theprocess results inphotons with alter- nating polarizations andrequires norepumping.

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The limits of the well-established single-atom model for describing photon-pair generation via four-wave mixing in a diamond configuration in atomic ensembles are experimentally tested. Using a cold-atom source, biphotons are generated and detected through polarization analyzers that resolve the emitted light into horizontal and vertical components in the laboratory frame. The pump lasers driving the first and second excitation transitions are horizontally and vertically polarized, respectively. To predict single-photon counts and coincidence rates in all polarization channels, the first- and second-order correlation functions are calculated directly using a comprehensive model that accounts for all Zeeman sublevels of the relevant hyperfine states. Furthermore, the population dynamics with and without the re-pump laser of the magneto-optical trap are compared, revealing substantial differences in the populations of the Zeeman sublevels. This motivates the inclusion of two additional hyperfine levels and their corresponding Zeeman sublevels in the final model. The resulting density matrix is used to calculate expectation values of the far-field electric-field operators and compare them with experimental measurements over a range of pump-laser powers. Excellent agreement with the measured photon counts is obtained over most of this range. For the coincidence measurements, good agreement is found when the polarization of the photon generated by the first (second) decay is parallel to that of the first (second) pump beam. In contrast, the model consistently underestimates the experimental coincidence rates for the opposite polarization configuration. These findings indicate that effects beyond the internal level dynamics of individual atoms, most notably collective phenomena, are required to fully account for photon coincidences generated by four-wave mixing in atomic ensembles.
We propose a mechanism for producing Fock states on demand leaking from a single mode optical cavity interacting with a single atom and a laser pulse. The number of photons can be chosen, as it is determined by the Zeeman substructure of the ground state of the atom and its initial state. The deterministic generation of a free-propagating Fock state of 1≤n≤2F1\leq n\leq2F1≤n≤2F photons is achieved, when a circularly polarized laser pulse completely transfers the atomic population between Zeeman sublevels of the ground hyperfine state FFF through far-detuned Raman scattering thus producing linearly polarized cavity photons. We describe analytically the evolution of optical field taking into account the spontaneous losses and the cavity damping. We demonstrate the possibility of production of Fock-state with different numbers of photons by using different transitions of the same atom. We show also that this technique provides a deterministic source of a train of identical multiphoton Fock-states, if a sequence of left- and right-circularly polarized laser pulses is applied. The resulting states have potential applications in quantum computation and simulation.