This thesis presents work aimed towards achieving sideband cooling of 40Ca+ ions in a Penning trap. The observation of an increase in the number of quantum jumps as a function of the trapping magnetic field is first presented. This observation is explained by the ion falling into a long-lived D5/2 state, out of which the ion is not being re-pumped. The ion can fall into this state due to mixing of the fine structure components with the same mJ quantum number induced by the applied magnetic field. A calculation of the mixing and shelving rate as a function of magnetic field strength is presented. This theory matches well with the experimental results observed. This work has been presented in a publication in which a perturbative analysis was used. An alternative analysis is presented here in which the full Hamiltonian is diagonalised. The essential conclusions however remain unchanged. This ‘J-state mixing’ effect means re-pumping from each of the six D5/2 state sub-levels of our ion is required for efficient laser cooling. This is achieved by the addition of a system comprising an 854 nm laser and a fibre EOM to provide the radiation required to re-pump these levels. The same EOM is then used to re-pump out of the four sub-levels of the D3/2 state using a single 866 nm laser. This is a great simplification of the experimental setup required to cool a 40Ca+ ion in a Penning trap which would otherwise require ten separate lasers to independently address each of the D sub-states. Achieving efficient repumping leads to the ability to perform pulsed spectroscopy on the quadrupole S1/2 → D5/2 transition in 40Ca+ . Preliminary results of this spectroscopy in a radio-frequency trap are presented.
This thesis presents work aimed towards achieving sideband cooling of 40Ca+ ions in a Penning trap. The observation of an increase in the number of quantum jumps as a function of the trapping magnetic field is first presented. This observation is explained by the ion falling into a long-lived D5/2 state, out of which the ion is not being re-pumped. The ion can fall into this state due to mixing of the fine structure components with the same mJ quantum number induced by the applied magnetic field. A calculation of the mixing and shelving rate as a function of magnetic field strength is presented. This theory matches well with the experimental results observed. This work has been presented in a publication in which a perturbative analysis was used. An alternative analysis is presented here in which the full Hamiltonian is diagonalised. The essential conclusions however remain unchanged. This ‘J-state mixing’ effect means re-pumping from each of the six D5/2 state sub-levels of our ion is required for efficient laser cooling. This is achieved by the addition of a system comprising an 854 nm laser and a fibre EOM to provide the radiation required to re-pump these levels. The same EOM is then used to re-pump out of the four sub-levels of the D3/2 state using a single 866 nm laser. This is a great simplification of the experimental setup required to cool a 40Ca+ ion in a Penning trap which would otherwise require ten separate lasers to independently address each of the D sub-states. Achieving efficient repumping leads to the ability to perform pulsed spectroscopy on the quadrupole S1/2 → D5/2 transition in 40Ca+ . Preliminary results of this spectroscopy in a radio-frequency trap are presented.
We report the laser cooling of a single 40Ca+ ion in a Penning trap to the motional ground state in one dimension. Cooling is performed in the strong binding limit on the 729-nm electric quadrupole ${S}_{1/2}\ensuremath{\leftrightarrow}{D}_{5/2}$ transition, broadened by a quench laser coupling the D5/2 and P3/2 levels. We find the final ground-state occupation to be 98(1)%. We measure the heating rate of the trap to be very low with $\stackrel{\ifmmode \dot{}\else \textperiodcentered \fi{}}{\overline{n}}\ensuremath{\approx}0.3(2)\text{ }\text{ }{\mathrm{s}}^{\ensuremath{-}1}$ for trap frequencies from 150--400 kHz, consistent with the large ion-electrode distance.
We report the laser cooling of a single 40Ca+ ion in a Penning trap to the motional ground state in one dimension. Cooling is performed in the strong binding limit on the 729-nm electric quadrupole S1/2↔D5/2 transition, broadened by a quench laser coupling the D5/2 and P3/2 levels. We find the final phonon number to be nˉ=0.014±0.009. We measure the heating rate of the trap to be very low with nˉ˙=2.5±0.3s−1 and a scaled spectral noise density of ωSE(ω)∼1.6−8V2m−2Hz−1s−1, which is consistent with the large ion-electrode distance. We perform Rabi oscillations on the sideband-cooled ion and observe a coherence time of 0.7±0.1ms, noting that the practical performance is currently limited by the intensity noise of the probe laser.
We have laser cooled a small cloud of 40Ca+ ions stored in a Penning trap. The large Zeeman splittings that result from the presence of the imposed magnetic field necessitate the use of two cooling lasers tuned to the ${}^{2}{S}_{1/2}{\ensuremath{-}}^{2}{P}_{1/2}$ transition near 397 nm (whereas only a single blue laser frequency is required in an rf trap). The 397 nm radiation is provided by a pair of blue diode lasers operated in extended cavities. Ions can escape from the cooling cycle by falling into a 2D3/2 state. There is also a small probability that ions can be pumped into a 2D5/2 state. The presence of large Zeeman splittings complicates the provision of repumper radiation to empty the D states. We describe two repumping schemes. The first scheme employs five infrared extended cavity diode lasers (ECDL's). The second scheme employs three infrared ECDL's, two of which have their injection current modulated to produce sidebands. An upper bound to the temperature of 1 K is inferred from the linewidth of the 397-nm fluorescence for a small cloud of 40Ca+ ions in our Penning trap. This work is part of a program aimed at using atomic ions in a Penning trap for decoherence studies and quantum information processing.
The long term aim of this work is to study the suitability of using laser cooled Ca+ ions in Penning traps as the basic components of a quantum computer. A great deal of progress in the field of quantum computing has been made in recent years with laser cooled ions stored in radio frequency ion traps. Building a useful quantum computer with trapped ions is however extremely challenging. Penning traps offer some possible benefits over radio frequency traps. They also create some additional difficulties. The potential advantages and disadvantages of Penning traps are discussed throughout the thesis. We show that we are able to overcome the problems associated with laser cooling in Penning traps, and have trapped single ions for extended periods of time. Pairs of Ca+ ions have been aligned along the axis of a Penning trap, and have been optically resolved. A novel Penning trap array based on PCB boards has been developed. A prototype was built and tested, along with the electronics required to shuttle ions between different sub-traps. Ions have been shuttled a distance of 10 mm in 2.5 μs. A return trip efficiency of up to 75% was seen. A quantum effect – J-state mixing caused by large magnetic fields – has been observed for the first time in single atomic ions. The magnetic field causes a forbidden [Delta]J = 2 transition to become weakly allowed. This effect is of general interest in atomic physics, and is also very relevant for quantum computation studies. A quantitative prediction of the magnitude of the J-mixing effect has been derived theoretically. This is compared to experimental data, and is found to be in excellent qualitative and good quantitative agreement.
For 35 years, laser-cooled trapped ions have been at the frontier of progress in quantum computing, quantum simulation and precision measurement, and remain one of the most valuable tools in these fields to this day. Most of these experiments are predicated upon or benefit from the ability to place ions in the motional quantum ground state, a technique that was first demonstrated in radiofrequency ion traps 25 years ago. For a range of crucial experiments that are impossible to conduct in radiofrequency traps or are not well suited to this architecture, Penning traps provide an important alternative. However, the performance of Penning traps had been limited by the fact that ground-state cooling was yet to be achieved in such a system. This thesis reports the first demonstration of resolved-sideband cooling in a Penning trap, for 40Ca+ions cooled with light at 729-nm, achieving a ground state occupation of 99% in one dimension. Demonstrations of the coherent manipulations possible at this level of confinement are presented. The ion heating rate is measured and although higher than might be expected given the unusually large ion-electrode distance remains amongst the lowest reported in any trap to date. Achieving this result required the development of a number of new experimental systems and major upgrades to the stability and reliability of the experiment, the details of which are also given. The thesis also presents theoretical work into the use of two-dimensional Coulomb crystals in a Penning trap as a resource for quantum information. Using the symmetries of the crystal, we find that it is possible to engineer complex entangled states, specifically two small quantum error correcting codes, using a very small number of global entangling pulses. Efficient entanglement protocols such as these are vital for the implementation of useful quantum error correction.