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Nonequilibrium Relaxation and Aging Scaling Properties of the Coulomb Glass and Bose Glass

Matthew T. Shimer

Published Aug 26, 2011• 1 citation
OpenAlex

Abstract

We use Monte Carlo simulations in order to investigate the density of states and the two-time density autocorrelation function for the two- and three-dimensional Coulomb glass as well as the Bose glass phase of flux lines in type-II superconductors. We find a very fast forming gap in the density of states and explore the dependence of temperature and filling fraction. By studying two scaling methods, we find that the nonequilibrium relaxation properties can be described sufficiently by a full-aging scaling analysis. The scaling exponents depend on both temperature and filling fraction, and are thus non-universal. We look at the trends of these exponents and found that as either the temperature decreases or the filling fraction deviates more from half-filling, the exponents reflect slower relaxation kinetics. With two separate interaction potentials, a comparison of relaxation rates and the gap in the density of states is made.

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We use Monte Carlo simulations in order to investigate the density of states and the two-time density autocorrelation function for the two- and three-dimensional Coulomb glass as well as the Bose glass phase of flux lines in type-II superconductors. We find a very fast forming gap in the density of states and explore the dependence of temperature and filling fraction. By studying two scaling methods, we find that the nonequilibrium relaxation properties can be described sufficiently by a full-aging scaling analysis. The scaling exponents depend on both temperature and filling fraction, and are thus non-universal. We look at the trends of these exponents and found that as either the temperature decreases or the filling fraction deviates more from half-filling, the exponents reflect slower relaxation kinetics. With two separate interaction potentials, a comparison of relaxation rates and the gap in the density of states is made.
We employ Monte Carlo simulations to investigate the nonequilibrium relaxation properties of the two- and three-dimensional Coulomb glass with different long-range repulsive interactions. Specifically, we explore the aging scaling laws in the two-time density autocorrelation function. We find that, in the time window and parameter range accessible to us, the scaling exponents are not universal, depending on the filling fraction and temperature: As either the temperature decreases or the filling fraction deviates more from half filling, the exponents reflect markedly slower relaxation kinetics. In comparison with a repulsive Coulomb potential, appropriate for impurity states in strongly disordered semiconductors, we observe that, for logarithmic interactions, the soft pseudogap in the density of states is considerably broader, and the dependence of the scaling exponents on external parameters is much weaker. The latter situation is relevant for flux creep in the disorder-dominated Bose glass phase of type-II superconductors subject to columnar pinning centers.
We study the nonequilibrium aging behavior of the gauge glass model in three dimensions at the critical temperature. We perform Monte Carlo simulations with a Metropolis update, and correlation and response functions are calculated for different waiting times. We obtain a multiplicative aging scaling of the correlation and response functions, calculating the aging exponent bbb and the nonequilibrium autocorrelation decay exponent ${\ensuremath{\lambda}}_{c}/{z}_{c}$. We also analyze the fluctuation-dissipation relationship at the critical temperature, obtaining the critical fluctuation-dissipation ratio ${X}_{\ensuremath{\infty}}$. By comparing our results with the aging scaling reported previously for a model of interacting flux lines in the vortex-glass regime, we found that the exponents for both models are very different.
The crossover between quasiequilibrium and nonequilibrium spin-glass dynamics has been studied in Monte Carlo simulations of two- and three-dimensional short-range Ising spin-glass systems. The spin system was quenched in zero field to a low temperature T. After equilibrating for a time tw{\mathit{t}}_{\mathit{w}}tw​, a weak magnetic field was applied and the time dependence of the magnetization M(t) and the spin autocorrelation function q(t) was studied. Our results show that the relaxation rate S(t)=\ensuremath{\partial}M(t)/\ensuremath{\partial} log10{\mathrm{log}}_{10}log10​(t) exhibits a maximum at t\ensuremath{\approxeq}tw{\mathit{t}}_{\mathit{w}}tw​. If the temperature is lowered or raised, immediately prior to the field application, the apparent age (ta{\mathit{t}}_{\mathit{a}}ta​) of the system, as defined by the maximum in relaxation rate, is shifted to longer or shorter time scales, respectively. No significant differences between the aging behavior in two and three dimensions are found. The relation \ensuremath{\chi}(t)=[1-q(t)]/T holds only for short time scales (t\ensuremath{\ll}tw{\mathit{t}}_{\mathit{w}}tw​), clear deviations are found at longer time scales (t>tw{\mathit{t}}_{\mathit{w}}tw​). Since this relation should according to the fluctuation-dissipation theorem hold for a system in equilibrium, this result is interpreted as an indication of a crossover between equilibrium and nonequilibrium dynamics. Our results are qualitatively in agreement with experiments as well as with theoretical models for the nonequilibrium spin-glass dynamics.
We employ Monte Carlo simulations to study the nonequilibrium relaxation of driven Ising lattice gases in two dimensions. Whereas the temporal scaling of the density autocorrelation function in the nonequilibrium steady state does not allow a precise measurement of the critical exponents, these can be accurately determined from the aging scaling of the two-time autocorrelations and the order parameter evolution following a quench to the critical point. We obtain excellent agreement with renormalization group predictions based on the standard Langevin representation of driven Ising lattice gases.
Aging of two-dimensional (2D) Ising spin glasses with short-range interactions Rb2{\mathrm{Rb}}_{2}Rb2​${\mathrm{Cu}}_{1\mathrm{\ensuremath{-}}\mathit{x}}$Cox{\mathrm{Co}}_{\mathit{x}}Cox​F4{\mathrm{F}}_{4}F4​ (Tc{\mathit{T}}_{\mathit{c}}Tc​=0) is studied in the critical regime via the low-frequency ac susceptibility and via the dc magnetization for x=0.22 and 0.33. After quenching to low temperatures, slow logarithmic relaxation is observed for both the in-phase and out-of-phase ac susceptibilities. Using the droplet scaling model, the spin-glass correlation length R is concluded to increase after a temperature quench as R\ensuremath{\propto}(lnt${)}^{1/\mathrm{\ensuremath{\psi}}}$, with t in units of some microscopic time. The exponent \ensuremath{\psi}=1.0\ifmmode\pm\else\textpm\fi{}0.1 compares with recent theoretical results and numerical simulations for 2D short-range Ising spin glasses. The waiting-time dependence found for the field-cooled and zero-field-cooled dc magnetizations points to a markedly slower crossover from the quasiequilibrium to the nonequilibrium regime than in 3D. From experiments with different cooling histories, finally, the equilibrium spin-glass state is inferred to be strongly dependent on the temperature.