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Atoms

Two-Photon Collective Atomic Recoil Lasing

James McKelvie, Gordon R. M. Robb

Published Nov 20, 2015• 0 citations
Publisher

Abstract

We present a theoretical study of the interaction between light and a cold gasof three-level, ladder configuration atoms close to two-photon resonance. In particular, weinvestigate the existence of collective atomic recoil lasing (CARL) instabilities in differentregimes of internal atomic excitation and compare to previous studies of the CARL instabilityinvolving two-level atoms. In the case of two-level atoms, the CARL instability is quenchedat high pump rates with significant atomic excitation by saturation of the (one-photon)coherence, which produces the optical forces responsible for the instability and rapid heatingdue to high spontaneous emission rates. We show that in the two-photon CARL schemestudied here involving three-level atoms, CARL instabilities can survive at high pump rateswhen the atoms have significant excitation, due to the contributions to the optical forces frommultiple coherences and the reduction of spontaneous emission due to transitions betweenthe populated states being dipole forbidden. This two-photon CARL scheme may form thebasis of methods to increase the effective nonlinear optical response of cold atomic gases.

DOI
10.3390/atoms3040495

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We present a theoretical study of the interaction between light and a cold gasof three-level, ladder configuration atoms close to two-photon resonance. In particular, weinvestigate the existence of collective atomic recoil lasing (CARL) instabilities in differentregimes of internal atomic excitation and compare to previous studies of the CARL instabilityinvolving two-level atoms. In the case of two-level atoms, the CARL instability is quenchedat high pump rates with significant atomic excitation by saturation of the (one-photon)coherence, which produces the optical forces responsible for the instability and rapid heatingdue to high spontaneous emission rates. We show that in the two-photon CARL schemestudied here involving three-level atoms, CARL instabilities can survive at high pump rateswhen the atoms have significant excitation, due to the contributions to the optical forces frommultiple coherences and the reduction of spontaneous emission due to transitions betweenthe populated states being dipole forbidden. This two-photon CARL scheme may form thebasis of methods to increase the effective nonlinear optical response of cold atomic gases.
Collective scattering of light due to atomic recoil, also known as collective atomic recoil lasing (CARL), occurs when a gas of atoms coherently scatters light from a pump laser via a collective instability. The scattering process can become unstable due to the atoms in the gas recoiling under the influence of the dynamic optical forces which arise due to the interference of the pump and scattered fields. The atoms move to form a spatially periodic density grating, which in turn amplifies the scattered field. This paper presents a theoretical analysis of CARL phenomena in degenerate ultracold gases of bosons and fermions. In the case of bosons i.e. in a Bose-Einstein Condensate (BEC),the effect of atom-atom interactions due to collisions on the CARL instability in the case of both attractive and repulsive condensates, is investigated. In the case of fermionic gases, the effect of Fermi pressure, is also presented. The linear and nonlinear evolution of the optical field and the atomic momentum distribution are considered for both cases.
Cold atoms in optical high‐Q cavities are an ideal model system for long‐range interacting particles. The position of two arbitrary atoms is, independent on their distance, coupled by the back‐scattering of photons within the cavity. This mutual coupling can lead to collective instability and self‐organization of a cloud of cold atoms interacting with the cavity fields. This phenomenon (CARL, i.e. Collective Atomic Recoil Lasing) has been discussed theoretically for years, but was observed only recently in our lab. The CARL‐effect is closely linked to superradiant Rayleigh scattering, which has been intensely studied with Bose‐Einstein condensates in free space. By adding a resonator the coherence time of the system, in which the instability occurs, can be strongly enhanced. This enables us to observe cavity‐enhanced superradiance with both Bose‐Einstein condensates and thermal clouds and allows us to close the discussion about the role of quantum statistics in superradiant scattering.
Summary form only given. The collective atomic recoil laser (CARL) was proposed as an atomic analog of the free electron laser. Recently, there has been an increased interest in the CARL primarily because it can be regarded as a parametric amplifier for the momentum side modes. Our CARL model consists of a cavity CARL signal of wave number k/sub 1/, and an opposing non-depletion pump field of k/sub 2/, and a steady flow of an ultra-cold two-level atomic beam along a direction normal to the propagation of the fields. Both fields are assumed to be far-off resonance. A momentum change of /spl planck/K, where K = k/sub 1/ + k/sub 2/, takes place in each virtual two-photon process. This allows us to divide the total momentum space into different momentum families, and each momentum family into different diffraction groups.
A cloud of ultra-cold atoms is loaded into the attractive potential of a light wave that is generated by two counter-propagating modes of a high-finesse ring resonator. The two modes are coupled by the atoms due to coherent Rayleigh scattering and generate a potential which acts back on the motion of the atoms. This feedback leads to a new frequency component and can be described in terms of the long time proposed collective atomic recoil laser (CARL). This model is investigated experimentally and extended by introducing an optical friction force acting on the atoms. This allows for steady state operation of the CARL. Furthermore, it leads to a threshold behaviour of the CARL that translates into a novel type of phase transition: while passing the threshold the initially homogeneous atomic distribution is bunched in space and velocity. With this behaviour the system turns out to acquire some of the main features of the so-called Kuramoto model which provides a very general description of a network of limit cycle oscillators.
An ensemble of periodically ordered atoms coherently scatters the light of an incident laser beam. The scattered and the incident light may interfere and give rise to a light intensity modulation and thus to optical dipole forces which, in turn, emphasize the atomic ordering. This positive feedback is at the origin of the collective atomic recoil laser (CARL). We demonstrate this dynamics using ultracold atoms confined by dipole forces in a unidirectionally pumped far red‐detuned high‐finesse optical ring cavity. Under the influence of an additional dissipative force exerted by an optical molasses the atoms, starting from an unordered distribution, spontaneously form a density grating moving at constant velocity. Additionally, steady state lasing is observed in the reverse direction if the pump laser power exceeds a certain threshold. We compare the dynamics of the atomic trajectories to the behavior of globally coupled oscillators, which exhibit phase transitions from incoherent to coherent states if the coupling strength exceeds a critical value.