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Springer eBooks

Unconventional Fractionalization of Strongly Correlated Electrons

A. Moreno, J. M. P. Carmelo, A. Muramatsu

Published Jan 1, 2013• 0 citations
Publisher
DOI
10.1007/978-3-319-02165-2_6

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Spin-Orbit Coupled Quantum Magnetism in the 3D-Honeycomb Iridates

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In this doctoral dissertation, we consider the significance of spin-orbit coupling for the phases of matter which arise for strongly correlated electrons. We explore emergent behavior in quantum many-body systems, including symmetry-breaking orders, quantum spin liquids, and unconventional superconductivity. Our study is cemented by a particular class of Mott-insulating materials, centered around a family of two- and three-dimensional iridium oxides, whose honeycomb-like lattice structure admits peculiar magnetic interactions, the so-called Kitaev exchange. By analyzing recent experiments on these compounds, we show that this unconventional exchange is the key ingredient in describing their magnetism, and then use a combination of numerical and analytical techniques to investigate the implications for the phase diagram as well as the physics of the proximate three-dimensional quantum spin liquid phases. These long-ranged-entangled fractionalized phases should exhibit special features, including finite-temperature stability as well as unconventional high-Tc superconductivity upon charge-doping, which should aid future experimental searches for spin liquid physics. Our study explores the nature of frustration and fractionalization which can arise in quantum systems in the presence of strong spin-orbit coupling.

•Jan 1, 2015•1 citation
The phase diagram of the attractive Hubbard model with spatially inhomogeneous interactions is obtained using a single-site dynamical mean-field theory-like approach. The model is characterized by three parameters: the interaction strength, the active fraction (fraction of sites with the attractive interaction), and electron filling. The calculations indicate that in a parameter regime with intermediate values of interaction strength (compared to the bare bandwidth of the electrons), and intermediate values of the active fraction, unconventional superconductivity is obtained. The results of this work are likely to be relevant to many systems with spatially inhomogeneous superconductivity such as strongly correlated oxides, systems with negative UUU centers, and, in future, cold atom optical lattices.
In this doctoral dissertation, we consider the significance of spin-orbit coupling for the phases of matter which arise for strongly correlated electrons. We explore emergent behavior in quantum many-body systems, including symmetry-breaking orders, quantum spin liquids, and unconventional superconductivity. Our study is cemented by a particular class of Mott-insulating materials, centered around a family of two- and three-dimensional iridium oxides, whose honeycomb-like lattice structure admits peculiar magnetic interactions, the so-called Kitaev exchange. By analyzing recent experiments on these compounds, we show that this unconventional exchange is the key ingredient in describing their magnetism, and then use a combination of numerical and analytical techniques to investigate the implications for the phase diagram as well as the physics of the proximate three-dimensional quantum spin liquid phases. These long-ranged-entangled fractionalized phases should exhibit special features, including finite-temperature stability as well as unconventional high-Tc superconductivity upon charge-doping, which should aid future experimental searches for spin liquid physics. Our study explores the nature of frustration and fractionalization which can arise in quantum systems in the presence of strong spin-orbit coupling.