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Physical Review B

Superfluidity of a nonequilibrium Bose-Einstein condensate of polaritons

Michiel Wouters, Vincenzo Savona

Published Feb 12, 2010• 59 citations
Publisher

Abstract

We study theoretically superfluidity in a driven-dissipative Bose gas out of thermal equilibrium, and discuss the relation with conventional superfluids. We show how the superfluid behavior is characterized by a dramatic increase in the lifetime of a quantized vortex and point out the influence of the spatial geometry of the condensate. We apply our study to a condensate of polaritons in a semiconductor microcavity, whose properties can be directly inferred from optical spectroscopy. We propose three different experimental schemes to measure the vorticity of the polariton condensate.

DOI
10.1103/physrevb.81.054508

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We study theoretically superfluidity in a driven-dissipative Bose gas out of thermal equilibrium, and discuss the relation with conventional superfluids. We show how the superfluid behavior is characterized by a dramatic increase in the lifetime of a quantized vortex and point out the influence of the spatial geometry of the condensate. We apply our study to a condensate of polaritons in a semiconductor microcavity, whose properties can be directly inferred from optical spectroscopy. We propose three different experimental schemes to measure the vorticity of the polariton condensate.
We review recent results on the coherence and superfluidity of driven dissipative condensates, i.e., systems of weakly interacting nonconserved bosons, such as polariton condensates. The presence of driving and dissipation has dramatically different effects depending on dimensionality and anisotropy. In three dimensions, equilibrium behaviour is recovered at large scales for static correlations, while the dynamical behaviour is altered by the microscopic driving. In two dimensions, for an isotropic system, drive and dissipation destroy the algebraic order that would otherwise exist; however, a sufficiently anisotropic system can still show algebraic phase correlations. We discuss the consequences of this behaviour for recent experiments measuring phase coherence and outline potential measurements that might directly probe superfluidity. Introduction This chapter is dedicated to superfluidity and its relation to Bose-Einstein condensation (BEC), a topic with a long history. Many reviews of the concepts of condensation and superfluidity in thermal equilibrium can be found; see for example Refs. [1, 2, 3, 4]. The focus of this chapter is on how these concepts apply (or fail to apply) to driven dissipative condensates – systems of bosons with a finite lifetime, in which loss is balanced by continuous pumping. We focus entirely on the steady state of such systems, neglecting transient, time-dependent behaviour. Experimentally, the most studied example of a driven dissipative condensate has been microcavity polaritons, an overview of which is given in Ref. [5] and Chapter 4. However, similar issues can arise in many other systems, most obviously photon condensates [6] (see also Chapter 19), magnon condensates [7] (see also Chapters 25–26), and potentially exciton condensates (although typical exciton lifetimes are much longer than for polaritons). Even experiments on cold atoms (see, e.g., Chapter 3) could be driven into a regime in which such physics occurs, when considering continuous loading of atoms balancing threebody losses [8] or atom laser setups [9, 10, 11]. Experiments on polaritons are two-dimensional, and in two dimensions it is particularly important to clearly distinguish three concepts often erroneously treated as equivalent: superfluidity, condensation, and phase coherence. This is because no true Bose-Einstein condensate exists in a homogeneous two-dimensional system.
We review, aiming at an audience of final year undergraduates, the phenomena observed in, and properties of, microcavity exciton–polariton condensates. These are condensates of mixed light and matter, consisting of superpositions of photons in semiconductor microcavities and excitons in quantum wells. Because of the imperfect confinement of the photon component, exciton–polaritons have a finite lifetime, and have to be continuously re-populated. Therefore, exciton–polariton condensates lie somewhere between equilibrium Bose–Einstein condensates and lasers. We review in particular the evidence for condensation, the coherence properties studied experimentally, and the wide variety of spatial structures either observed or predicted to exist in exciton–polariton condensates, including quantised vortices and other coherent structures. We also discuss the question of superfluidity in a non-equilibrium system, reviewing both the experimental attempts to investigate superfluidity to date, and the theoretical suggestions of how it may be further elucidated.
The experimental realization of Bose-Einstein condensation (BEC) with atoms and quasiparticles has triggered wide exploration of macroscopic quantum effects.Microcavity polaritons are of particular interest because quantum phenomena such as BEC and superfluidity can be observed at elevated temperatures.However, polariton lifetimes are typically too short to permit thermal equilibration.This has led to debate about whether polariton condensation is intrinsically a nonequilibrium effect.Here we report the first unambiguous observation of BEC of optically trapped polaritons in thermal equilibrium in a high-Q microcavity, evidenced by equilibrium Bose-Einstein distributions over broad ranges of polariton densities and bath temperatures.With thermal equilibrium established, we verify that polariton condensation is a phase transition with a well-defined density-temperature phase diagram.The measured phase boundary agrees well with the predictions of basic quantum gas theory.
We theoretically study the superfluidity properties of a nonequilibrium Bose-Einstein condensate of exciton polaritons in a semiconductor microcavity under incoherent pumping. The dynamics of the condensate is described at mean-field level in terms of a generalized Gross-Pitaevskii equation. The drag force on a small moving object and the onset of fringes in the density profile are shown to have a sharp threshold as a function of the velocity; a generalized Landau criterion is developed to explain this behavior in terms of the dispersion of elementary excitations. Metastability of supercurrents in multiply-connected geometries is shown to persist up to higher flow speeds.
Exciton-polaritons, mixed light-matter quasiparticles in semiconductors, have recently shown evidence for Bose-Einstein condensation. Some of the properties of condensates of exciton-polaritons are reviewed in this article. We first discuss the spontaneous appearance of long-range order and the way this can be easily accessed in the case of polariton fluids. We show that the Penrose-Onsager criterion is valid even for such a very special case of condensate. We then describe the experiments that allow observation of topological defects in the fluid: quantized vortices, half vortices, and hyperbolic spin vortices. We demonstrate through the comparison with the gross Pitaevskii equation that the appearance and stability of such vortices are linked with the dissipative nature of the condensate together with the presence of disorder. We then briefly summarize the experiments on superfluid behavior of the polaritons at large-enough densities and expand somewhat more on the dynamical behavior of turbulence in the wake of an obstacle, with the appearance of vortex streets. We finally show that the Bogoliubov transformation has been revealed through four-wave mixing experiments.