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Ultra-bright and efficient single photon generation based on integrated nanodiamonds containing single defect centers

Tim Schröder, Andreas Wolfgang Schell, Friedemann Gädeke, Günter Kewes, Thomas Aichele, Oliver J. Benson

Published Jan 1, 2011• 1 citation
Publisher

Abstract

We present integrated and highly efficient single photon sources based on defect-centers in nanodiamonds as fundamental components for future implementations of quantum information technologies. We achieve count rates of 2.4 Mcts/s and source efficiencies of 20 %.
DOI
10.1364/qels.2011.qfg1

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Single photons are fundamental elements for quantum information technologies such as quantum cryptography, quantum information storage and optical quantum computing. Colour centres in diamond have proven to be stable single-photon sources and thus essential components for reliable and integrated quantum information technology. A key requirement for such applications is a large photon flux and a high efficiency. Paying tribute to various attempts to maximize the single-photon flux, we show that collection efficiencies of photons from colour centres can be increased with a rather simple experimental setup. To do so, we spin-coated nanodiamonds containing single nitrogen-vacancy (N-V) colour centres on the flat surface of a ZrO 2 solid immersion lens. We found stable single-photon count rates of up to 853 kcts s − 1 at saturation under continuous wave excitation while having access to more than 100 defect centres with count rates from 400 to 500 kcts s − 1 . For a blinking defect centre, we found count rates up to 2.4 Mcts s − 1 for time intervals of several tens of seconds. It seems to be a general feature that very high rates are accompanied by blinking behaviour. The overall collection efficiency of our setup of up to 4.2% is the highest yet reported for N-V defect centres in diamond. Under pulsed excitation of a stable emitter of 10 MHz, 2.2% of all pulses caused a click on the detector adding to 221 kcts s − 1 thus, opening the way towards diamond-based on-demand single-photon sources for quantum applications.
Defect centers in diamond are regarded as a promising candidate for future solid state quantum technology. In particular the nitrogen vacancy (NV) center attracts researchers attention, as it promises to emit indistinguishable single photons and provides a triplet ground state with ultra long spin coherence times. In particular NV centers in nano diamonds are attractive, since they can be integrated into quantum photonic hybrid devices with nano manipulation techniques. We report on first demonstrations of the integration of NV-centers into photonic hybrid devices, and point out future applications. Beside the striking demonstrations of the integrability, nanodiamonds have several drawbacks. In particular the spectral diffusion of the zero-phonon line is addressed.
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The nanodiamond technology has developed the first packaged, single-photon source that operates at room temperature and in well-lit environments, where an ideal single-photon source produces one photon per pulse. These sources are key components for building quantum information systems that can implement quantum-key distribution (QKD) for ultrasecure communications. The optically active color centers in diamond have been found to exhibit attractive optical properties through the nitrogen-vacancy (N-V) center emission ranging 600 to 750 nm, and that have realized the practical sources of single-photon emission. Photo statistics has to be determined to measure the performance of a single-photon source, which can be measured by the autocorrelation function g2 (0) using Hanbury-Brown and Twiss interferometer. The results showed that the SPS 1.01 demonstrates stable single-photon performance without requirement of recalibration.