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The European Physical Journal B

Optical Bloch equations in a bichromatic field; vibrational resonance

Shyamolina Ghosh, Deb Shankar Ray

Published Jan 1, 2015• 6 citations
Publisher
DOI
10.1140/epjb/e2014-50306-y

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Resonance-fluorescence and absorption spectra of a two-level atom driven by a strong bichromatic field

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We examine the radiative properties of a two-level atom driven by a strong bichromatic field with frequencies ${\mathrm{\ensuremath{\omega}}}_{1}$=${\mathrm{\ensuremath{\omega}}}_{0}$-${\mathrm{\ensuremath{\delta}}}_{1}$ and ${\mathrm{\ensuremath{\omega}}}_{2}$=${\mathrm{\ensuremath{\omega}}}_{0}$+${\mathrm{\ensuremath{\delta}}}_{2}$, which can be asymmetrically placed about the atomic transition frequency ${\mathrm{\ensuremath{\omega}}}_{0}$ and can have different Rabi frequencies ${\mathrm{\ensuremath{\Omega}}}_{1}$ and ${\mathrm{\ensuremath{\Omega}}}_{2}$. Applying the optical Bloch equations for the bichromatic excitation, we derive an infinite set of equations of motion for the time evolution of the atomic variables. The equations are solved numerically by matrix inversion and Laplace transforms. Using the quantum regression theorem, we then solve for the steady-state total fluorescence intensity, and the resonance-fluorescence and absorption spectra. The spectra are found to depend on the frequency difference 2\ensuremath{\delta}=${\mathrm{\ensuremath{\delta}}}_{1}$+${\mathrm{\ensuremath{\delta}}}_{2}$, the average detuning \ensuremath{\Delta}=${\mathrm{\ensuremath{\omega}}}_{0}$-1/2(${\mathrm{\ensuremath{\omega}}}_{1}$+${\mathrm{\ensuremath{\omega}}}_{2}$), and the Rabi frequencies of the driving fields. For ${\mathrm{\ensuremath{\Omega}}}_{1}$=${\mathrm{\ensuremath{\Omega}}}_{2}$=\ensuremath{\Omega}, the total fluorescent intensity displays a series of maxima for \ensuremath{\Delta}=\ifmmode\pm\else\textpm\fi{}n\ensuremath{\delta}\ensuremath{\mp}${\mathrm{\ensuremath{\Omega}}}^{2}$/4\ensuremath{\delta}, where the n are the odd integers. The intensity-dependent shift from the resonances n\ensuremath{\delta} is explained as an analog of the generalized Bloch-Siegert shift. The resonance-fluorescence spectrum for \ensuremath{\Delta}\ensuremath{\ne}0 appears to contain more peaks than that for \ensuremath{\Delta}=0.This is due to the splitting of the central peak and the even sidebands into doublets. The absorption spectrum of a weak-probe beam for \ensuremath{\Delta}=0 and equal Rabi frequencies consists of a symmetric series of dispersionlike sidebands separated from ${\mathrm{\ensuremath{\omega}}}_{0}$ by integer multiples of \ensuremath{\delta}, together with a central absorption peak at ${\mathrm{\ensuremath{\omega}}}_{0}$, whose amplitude oscillates with \ensuremath{\Omega}. For \ensuremath{\Delta}\ensuremath{\ne}0 and/or ${\mathrm{\ensuremath{\Omega}}}_{1}$\ensuremath{\ne}${\mathrm{\ensuremath{\Omega}}}_{2}$, the odd sidebands remain dispersionlike, while the central peak and the even sidebands split into absorption-emission doublets. A simple physical interpretation of the spectral features is given in terms of the dressed-atom model.

Physical Review A•Oct 1, 1993•110 citations
We identify discrepancies between two published predictions of the resonance fluorescence from a two-level atom driven by a strong bichromatic field [J. Opt. Soc. Am. B 8,8,8, 1163 (1991) and Phys. Rev. A 48,48,48, 3092 (1993)]. These discrepancies are shown to arise from subtleties in extracting the time-averaged resonance fluorescence from the expansions used to solve the optical Bloch equations. We construct a solution to these equations that corrects the results of the latter reference and reconciles the two predictions.
We consider the effect of the noise difference phase of a bichromatic field upon coherent population trapping resonances in the simplest three-level system in Λ configuration. The quasi-stationary solution of Bloch optical equations, which was found with some assumptions, shows that the presence of exciting short-correlated fluctuations of the phase of radiation reduces the contrast of the resonance line without affecting its spectral width. For the Gaussian phase noise the contrast suppression factor is χ = exp[−ϕ rms 2 ], where ϕ rms 2 is phase dispersion. The experimental results obtained earlier by our group are analyzed.
We examine the radiative properties of a two-level atom driven by a strong bichromatic field with frequencies ${\mathrm{\ensuremath{\omega}}}_{1}$=${\mathrm{\ensuremath{\omega}}}_{0}$-${\mathrm{\ensuremath{\delta}}}_{1}$ and ${\mathrm{\ensuremath{\omega}}}_{2}$=${\mathrm{\ensuremath{\omega}}}_{0}$+${\mathrm{\ensuremath{\delta}}}_{2}$, which can be asymmetrically placed about the atomic transition frequency ${\mathrm{\ensuremath{\omega}}}_{0}$ and can have different Rabi frequencies ${\mathrm{\ensuremath{\Omega}}}_{1}$ and ${\mathrm{\ensuremath{\Omega}}}_{2}$. Applying the optical Bloch equations for the bichromatic excitation, we derive an infinite set of equations of motion for the time evolution of the atomic variables. The equations are solved numerically by matrix inversion and Laplace transforms. Using the quantum regression theorem, we then solve for the steady-state total fluorescence intensity, and the resonance-fluorescence and absorption spectra. The spectra are found to depend on the frequency difference 2\ensuremath{\delta}=${\mathrm{\ensuremath{\delta}}}_{1}$+${\mathrm{\ensuremath{\delta}}}_{2}$, the average detuning \ensuremath{\Delta}=${\mathrm{\ensuremath{\omega}}}_{0}$-1/2(${\mathrm{\ensuremath{\omega}}}_{1}$+${\mathrm{\ensuremath{\omega}}}_{2}$), and the Rabi frequencies of the driving fields. For ${\mathrm{\ensuremath{\Omega}}}_{1}$=${\mathrm{\ensuremath{\Omega}}}_{2}$=\ensuremath{\Omega}, the total fluorescent intensity displays a series of maxima for \ensuremath{\Delta}=\ifmmode\pm\else\textpm\fi{}n\ensuremath{\delta}\ensuremath{\mp}${\mathrm{\ensuremath{\Omega}}}^{2}$/4\ensuremath{\delta}, where the n are the odd integers. The intensity-dependent shift from the resonances n\ensuremath{\delta} is explained as an analog of the generalized Bloch-Siegert shift. The resonance-fluorescence spectrum for \ensuremath{\Delta}\ensuremath{\ne}0 appears to contain more peaks than that for \ensuremath{\Delta}=0.This is due to the splitting of the central peak and the even sidebands into doublets. The absorption spectrum of a weak-probe beam for \ensuremath{\Delta}=0 and equal Rabi frequencies consists of a symmetric series of dispersionlike sidebands separated from ${\mathrm{\ensuremath{\omega}}}_{0}$ by integer multiples of \ensuremath{\delta}, together with a central absorption peak at ${\mathrm{\ensuremath{\omega}}}_{0}$, whose amplitude oscillates with \ensuremath{\Omega}. For \ensuremath{\Delta}\ensuremath{\ne}0 and/or ${\mathrm{\ensuremath{\Omega}}}_{1}$\ensuremath{\ne}${\mathrm{\ensuremath{\Omega}}}_{2}$, the odd sidebands remain dispersionlike, while the central peak and the even sidebands split into absorption-emission doublets. A simple physical interpretation of the spectral features is given in terms of the dressed-atom model.