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Physical Review A

Einstein-Podolsky-Rosen correlations in second-harmonic generation

Peter Lodahl

Published Aug 18, 2003• 23 citations
Publisher

Abstract

A quantum model for singly resonant second-harmonic generation in a cavity with transverse degrees of freedom is analyzed. An instability threshold for pattern formation exists in this system. Below threshold, a strong modulation of the noise is demonstrated in the transverse structure of the far field. The performed analysis encompasses both one- and two-point correlation functions. The noise in a single far-field point is generally above the classical vacuum noise level. In contrast, strong nonclassical two-point correlations are encountered between opposite emission directions in the far field. For the fundamental field the correlations are shown to be of the Einstein-Podolsky-Rosen type, thus establishing a remarkable analog to the quantum correlations found in a nondegenerate optical parametric oscillator.

DOI
10.1103/physreva.68.023806

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A quantum model for singly resonant second-harmonic generation in a cavity with transverse degrees of freedom is analyzed. An instability threshold for pattern formation exists in this system. Below threshold, a strong modulation of the noise is demonstrated in the transverse structure of the far field. The performed analysis encompasses both one- and two-point correlation functions. The noise in a single far-field point is generally above the classical vacuum noise level. In contrast, strong nonclassical two-point correlations are encountered between opposite emission directions in the far field. For the fundamental field the correlations are shown to be of the Einstein-Podolsky-Rosen type, thus establishing a remarkable analog to the quantum correlations found in a nondegenerate optical parametric oscillator.
We investigate the spatial quantum noise properties of the one-dimensional transverse pattern formation instability in intracavity second-harmonic generation. The Q representation of a quasi-probability distribution is implemented in terms of nonlinear stochastic Langevin equations. We study these equations through extensive numerical simulations and analytically in the linearized limit. Our study, made below and above the threshold of pattern formation, is guided by a microscopic scheme of photon interaction underlying pattern formation in second-harmonic generation. Close to the threshold for pattern formation, beams with opposite direction of the off-axis critical wave numbers are shown to be highly correlated. This is observed for the fundamental field, for the second-harmonic field, and also for the cross-correlation between the two fields. Nonlinear correlations involving the homogeneous transverse wave number, which are not identified in a linearized analysis, are also described. The intensity differences between opposite points of the far fields are shown to exhibit sub-Poissonian statistics, revealing the quantum nature of the correlations. We observe twin beam correlations in both the fundamental and second-harmonic fields, and also nonclassical correlations between them.
A Langevin model is introduced to study quantum fluctuations below the threshold of pattern formation for optical parametric oscillators (OPO's). In particular we compare analytical and numerical results for the OPO with one and two transverse spatial dimensions and in the presence of either plane or spherical cavity mirrors. The far-field structure and the correlation functions of the fluctuating signal field anticipate the onset of a transverse spatial pattern which arises classically even in the presence of Gaussian input beams. Correlation functions also reveal the squeezed nature of the OPO field. Numerical simulations of the Langevin model describe the result of short time measurements and show that close to threshold the near-field signal is a noisy spot pattern evolving on a time scale longer than the inverse decay rate of the resonator. This and other far-field features should be experimentally accessible.
We investigate theoretically the spatial quantum correlations of the light produced by spontaneous emission in type-I second-harmonic generation in the traveling-wave configuration. It is first shown that spontaneous emission occurs at both fundamental and second-harmonic frequency. Considering the quantum fluctuations of the intensities collected in symmetrical parts of the far-field plane, nonclassical correlations below the shot noise are predicted not only at fundamental frequency, but also at second-harmonic frequency. The latter cannot be traced back to any twin-photon emission mechanism, but are generated by a secondary process acting on twin photons. This mechanism also creates correlations between fundamental and second-harmonic field, at a given transverse wave number, and at opposite wave numbers. The analysis of a simplified few-mode model, on a quantum level, provides a good qualitative understanding of these correlations.
We study the far-field spatial distribution of the quantum fluctuations in the transverse profile of the output light beam generated by a type-II optical parametric oscillator below threshold, including the effects of transverse walk-off. We study how quadrature field correlations depend on the polarization. We find spatial Einstein-Podolsky-Rosen entanglement in quadrature-polarization components. For the far-field points not affected by walk-off there is almost complete noise suppression in the proper quadratures difference of any orthogonal polarization components. We show the entanglement of the state of symmetric, intense, or macroscopic, spatial light modes. We also investigate nonclassical polarization properties in terms of the Stokes operators. We find perfect correlations in all Stokes parameters measured in opposite far-field points in the direction orthogonal to the walk-off, while locally the field is unpolarized and we find no polarization squeezing.
SUMMARY Parametric processes in the interaction of electromagnetic field with a medium in an optical cavity are well known to produce states of light with nonclassical properties. The quantum correlations between these states can be employed for a realization of an EinsteinPodolsky-Rosen (EPR) paradox [l], in the original formulation using continuous variables, as proposed [2] and experimentally demonstrated [3] in the case of Nondegenerate Parametric Amplification below threshold. In this paper we study EPR-like behaviour between the signal and idler fields emitted by a degenerate optical parametric oscillator (OPO) above threshold; these fields, generated by conversion of a pump photon of frequency 2w0 in two photons of frequency w. , are spatially separated in the far field, showing non-local quantum correlations. The system is described by the full Hamiltonian for the operators associated with the pump and signal fields; the optical cavity introduces proper damping constants and corresponding vacuum field operators [4,5]. Above the threshold for the generation of the signal field, we consider the fluctuations in the intensity difference and in the phase sum of the signal beams, which are related to their degree of mutual correlation. By linearizing around the stationary state, we calculate the spectral variances of these quantities (i.e. the Fourier transform of the two time correlation functions). The Heisenberg uncertainty principle sets a lower limit to the product of the spectral variances for the fluctuations in the intensity and in the phase of each individual signal field; by using the idler beam to infer results of measurements on the correlated signal beam, we have an EPR paradox if the product of the spectral variances for the fluctuations in the intensity difference and phase sum of the fields, is below the uncertainty limit. This feature is apparent for a wide interval around zero frequency in the far field of the active OPO system, depending on the parameter space; in particular there is maximum correlation between signal beams, and therefore maximum breaking of the uncertainty limit, if the damping constant of the signal field is larger than that of the pump field.
We develop the quantum theory of a driven, damped intracavity parametric oscillator in the case of nondegenerate signal and idler modes. An analysis of the results of different types of local-oscillator measurements on the outgoing modes is presented. The frequency-domain squeezing is calculated below threshold including the effect of detunings and nonequal decay rates. We also calculate a nonclassical correlation in the quadrature amplitudes of the output beams. The existence of an Einstein-Podolsky-Rosen paradox is demonstrated through violations of the inferred Heisenberg uncertainty principle at causally unrelated locations in the output field. This provides a way of maintaining the commutation relations of the measured operators in the exact form envisaged originally by Einstein, Podolsky, and Rosen.