Challenges
Datasets
Workspaces
Papers
Discussions
Leaderboard
Log inSign up
Challenges
Datasets
Workspaces
Papers
Discussions
Leaderboard
Blog
Job Board
Q3AS

© 2026 Aqora Quantum S.A.S.

TermsPrivacyLegal Notice

physica status solidi (b)

Coherent control of excitonic excitations in II–VI quantum wells

T. Voss, Hans Georg Breunig, Ilja Rückmann, J. Gutowski

Published Jan 31, 2006• 1 citation
Publisher

Abstract

Abstract We present results of experimental work in which the coherent‐control technique has been applied to study the coherent manipulation of excitonic polarization in ZnSe quantum‐well samples. We will introduce the linear control of excitonic polarization in pulse‐transmission experiments and afterwards focus on the question if and how the optical transition from the excitonic states to the bound‐biexciton state can be subject to a directed coherent control. The experimental results will be compared to simulations based on a microscopic theory and will also be explained on the base of a phenomenological few‐level model. The overall suitability of coherent control for the investigation of exciton systems in low‐dimensional wide‐gap materials will be discussed. (© 2006 WILEY‐VCH Verlag GmbH & Co. KGaA, Weinheim)

DOI
10.1002/pssb.200564716

Related papers

Coherent control of exciton–biexciton beats: direction selectivity of four‐wave‐mixing signals in experiment and microscopic theory

T. Voss, Ilja Rückmann, J. Gutowski +2 more

Abstract In experiments and simulations based on a microscopic theory the optical coherent control of exciton–biexciton beats in coherent four‐wave‐mixing signals from a semiconductor quantum well is demonstrated. It is found that a reduction of the beat amplitude for one four‐wave‐mixing direction may at the same time coincide with a large beat amplitude for the other direction. The results can be understood by considering that at least two‐photon processes are required to coherently excite biexcitonic transitions which are responsible for the occurrence of the beat structure in the four‐wave‐mixing signals. (© 2006 WILEY‐VCH Verlag GmbH & Co. KGaA, Weinheim)

physica status solidi (b)•Jul 12, 2006•1 citation

Excitation-induced dephasing and biexcitonic effects in the coherent control of excitonic polarization in pulse-transmission experiments

T. Voss, Hans Georg Breunig, Ilja Rückmann +1 more

Optical coherent manipulation of excitonic polarization is studied in pulse-transmission experiments at medium to high excitation intensities. As a well-defined model system a ZnSe single-quantum well is used. It is found that for constant excitation intensities the dephasing time of the polarization in the sample changes significantly if the cases of coherent amplification and destruction are compared. This effect is explained in terms of an excitation-induced dephasing. The change of the dephasing time of the polarization is quantified. Furthermore, the simultaneous excitation of the exciton and exciton-biexciton resonances is shown to strongly influence the signal of the polarization in the coherent-control experiments. Both the excitation-induced dephasing and the biexcitonic effects are simulated by use of phenomenological models which give a good agreement with the experiments.

Physical Review B•May 27, 2004•12 citations

Real-time observation of the coherent control of linear- and four-wave-mixing polarization of excitons in a ZnSe single quantum well

T. Voss, Hans-Georg Breunig, Ilja Rückmann +1 more

The coherent control of excitonic and biexcitonic polarization in pulse-transmission and four-wave-mixing (FWM) experiments is analysed with real time resolution. As a model system a ZnSe single quantum well is exclusively excited at the heavy-hole exciton and exciton–biexciton resonance. In pulse-transmission experiments the coherent control of excitonic polarization is shown for low excitation intensities. At elevated excitation intensities the dephasing time of the polarization is found to be strongly dependent on the relative phase of two phase-locked laser pulses which perform the coherent manipulation of the polarization. In FWM experiments the separate coherent control of the excitonic and biexcitonic FWM polarization is demonstrated which enables a coherent manipulation of the amplitude and phase of exciton–biexciton beats which are observed on the FWM polarization transients.

Semiconductor Science and Technology•Mar 3, 2004•0 citations

Coherent control of the exciton and exciton-biexciton transitions in the generation of nonlinear wave-mixing signals in a semiconductor quantum well

T. Voss, Ilja Rückmann, J. Gutowski +2 more

By use of an optical coherent-control technique we demonstrate and analyze the control of transitions involved in the generation of four-wave-mixing signals in a semiconductor quantum well for the two different four-wave-mixing directions and for different sequences of the excitation pulses. Results are presented for frequency- as well as for time-resolved signals. A doubling of the coherent switching frequency is found which occurs if the laser pulses performing the control process contribute quadratically to the wave-mixing signal. A direct comparison between experiment and microscopic theory reveals how the coherent-control process acts on the coherent polarization of the exciton-biexciton system in all different configurations. An additional interpretation of the experimental results based on a simplified few-level model is able to provide an intuitive understanding of the relevant processes which govern the coherent control of the excitonic and biexcitonic wave-mixing polarizations.

Physical Review B•Mar 9, 2006•31 citations

Coherent control of the biexciton in a single quantum dot

Timur Flissikowski, Alexander Betke, Ilya A. Akimov +1 more

Abstract We report on coherent control of the two‐photon transition between the ground state and the biexciton state on a single quantum dot level. The population of the biexciton is monitored by the cascaded spontaneous emission of the biexciton complex via the exciton states. The signal shows interference pattern at the double laser frequency and its contrast decays non‐exponentially at the time scale of 10 ps. The contrast decrease is attributed to a dynamical inhomogeneous broadening of the energy levels due to long‐term fluctuations in the dot environment. (© 2005 WILEY‐VCH Verlag GmbH & Co. KGaA, Weinheim)

physica status solidi (a)•Feb 1, 2005•1 citation

Biexcitonic effects in the coherent control of the excitonic polarization detected in six-wave-mixing signals

T. Voss, Hans Georg Breunig, Ilja Rückmann +3 more

Coherently controlled six-wave-mixing experiments on a ZnSe single quantum well are performed with different polarizations of the excitation pulses to enable or disable the creation of a biexcitonic polarization. A significant contribution of the biexcitonic polarization and other two-pair correlations is observed in the signal which is mainly modulated with the exciton transition frequency. A microscopic theory based on the dynamics controlled truncation scheme including six-point correlations is able to reproduce the experimental results.

Physical review. B, Condensed matter•Oct 1, 2002•19 citations
Abstract We present results of experimental work in which the coherent‐control technique has been applied to study the coherent manipulation of excitonic polarization in ZnSe quantum‐well samples. We will introduce the linear control of excitonic polarization in pulse‐transmission experiments and afterwards focus on the question if and how the optical transition from the excitonic states to the bound‐biexciton state can be subject to a directed coherent control. The experimental results will be compared to simulations based on a microscopic theory and will also be explained on the base of a phenomenological few‐level model. The overall suitability of coherent control for the investigation of exciton systems in low‐dimensional wide‐gap materials will be discussed. (© 2006 WILEY‐VCH Verlag GmbH & Co. KGaA, Weinheim)
Abstract In experiments and simulations based on a microscopic theory the optical coherent control of exciton–biexciton beats in coherent four‐wave‐mixing signals from a semiconductor quantum well is demonstrated. It is found that a reduction of the beat amplitude for one four‐wave‐mixing direction may at the same time coincide with a large beat amplitude for the other direction. The results can be understood by considering that at least two‐photon processes are required to coherently excite biexcitonic transitions which are responsible for the occurrence of the beat structure in the four‐wave‐mixing signals. (© 2006 WILEY‐VCH Verlag GmbH & Co. KGaA, Weinheim)
Optical coherent manipulation of excitonic polarization is studied in pulse-transmission experiments at medium to high excitation intensities. As a well-defined model system a ZnSe single-quantum well is used. It is found that for constant excitation intensities the dephasing time of the polarization in the sample changes significantly if the cases of coherent amplification and destruction are compared. This effect is explained in terms of an excitation-induced dephasing. The change of the dephasing time of the polarization is quantified. Furthermore, the simultaneous excitation of the exciton and exciton-biexciton resonances is shown to strongly influence the signal of the polarization in the coherent-control experiments. Both the excitation-induced dephasing and the biexcitonic effects are simulated by use of phenomenological models which give a good agreement with the experiments.
The coherent control of excitonic and biexcitonic polarization in pulse-transmission and four-wave-mixing (FWM) experiments is analysed with real time resolution. As a model system a ZnSe single quantum well is exclusively excited at the heavy-hole exciton and exciton–biexciton resonance. In pulse-transmission experiments the coherent control of excitonic polarization is shown for low excitation intensities. At elevated excitation intensities the dephasing time of the polarization is found to be strongly dependent on the relative phase of two phase-locked laser pulses which perform the coherent manipulation of the polarization. In FWM experiments the separate coherent control of the excitonic and biexcitonic FWM polarization is demonstrated which enables a coherent manipulation of the amplitude and phase of exciton–biexciton beats which are observed on the FWM polarization transients.
By use of an optical coherent-control technique we demonstrate and analyze the control of transitions involved in the generation of four-wave-mixing signals in a semiconductor quantum well for the two different four-wave-mixing directions and for different sequences of the excitation pulses. Results are presented for frequency- as well as for time-resolved signals. A doubling of the coherent switching frequency is found which occurs if the laser pulses performing the control process contribute quadratically to the wave-mixing signal. A direct comparison between experiment and microscopic theory reveals how the coherent-control process acts on the coherent polarization of the exciton-biexciton system in all different configurations. An additional interpretation of the experimental results based on a simplified few-level model is able to provide an intuitive understanding of the relevant processes which govern the coherent control of the excitonic and biexcitonic wave-mixing polarizations.
Abstract We report on coherent control of the two‐photon transition between the ground state and the biexciton state on a single quantum dot level. The population of the biexciton is monitored by the cascaded spontaneous emission of the biexciton complex via the exciton states. The signal shows interference pattern at the double laser frequency and its contrast decays non‐exponentially at the time scale of 10 ps. The contrast decrease is attributed to a dynamical inhomogeneous broadening of the energy levels due to long‐term fluctuations in the dot environment. (© 2005 WILEY‐VCH Verlag GmbH & Co. KGaA, Weinheim)
Coherently controlled six-wave-mixing experiments on a ZnSe single quantum well are performed with different polarizations of the excitation pulses to enable or disable the creation of a biexcitonic polarization. A significant contribution of the biexcitonic polarization and other two-pair correlations is observed in the signal which is mainly modulated with the exciton transition frequency. A microscopic theory based on the dynamics controlled truncation scheme including six-point correlations is able to reproduce the experimental results.