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IEEE Journal of Quantum Electronics

Propagation of optical pulses in a saturable absorber

L. Davis, Yung‐Sen Lin

Published Dec 1, 1973• 7 citations
Publisher

Abstract

The coupled Maxwell-Schrodinger equations are used to describe propagation of a pulse in a nonlinear absorbing medium. The absorber is assumed to be comprised of a homogeneously broadened system of two-level atoms that are exactly resonant with the field. Numerical calculations have been performed for incident pulses of hyperbolic-secant shape and of duration that is long compared to the atomic phase-memory time. Selected values of input intensity are considered. For intensities below a certain level the calculations nearly agree with rate-equation predictions, but as the incident intensity is increased we find that optical nutation comes into play. The nutation effect leads to pulse breakup as the packet penetrates into the medium. An analytical calculation, for the case of an applied optical field of step-function form, has been performed in order to provide additional insight about the intensity threshold for nutation.

DOI
10.1109/jqe.1973.1077435

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Physical Review A•Jan 11, 2000•13 citations
The coupled Maxwell-Schrodinger equations are used to describe propagation of a pulse in a nonlinear absorbing medium. The absorber is assumed to be comprised of a homogeneously broadened system of two-level atoms that are exactly resonant with the field. Numerical calculations have been performed for incident pulses of hyperbolic-secant shape and of duration that is long compared to the atomic phase-memory time. Selected values of input intensity are considered. For intensities below a certain level the calculations nearly agree with rate-equation predictions, but as the incident intensity is increased we find that optical nutation comes into play. The nutation effect leads to pulse breakup as the packet penetrates into the medium. An analytical calculation, for the case of an applied optical field of step-function form, has been performed in order to provide additional insight about the intensity threshold for nutation.
A comprehensive model of intense laser light propagation in a fully saturable medium is presented. This model employs the Maxwell-Bloch equations for a two-level atomic system. Light propagating through a medium creates intensity-dependent index of refraction gradients that reduce to a Kerr nonlinearity only for a weak field. When the laser detuning is positive, self-induced index gradients cause the beam to self-focus. Stationary filaments occur when self-focusing exactly balances diffraction. There exists a unique set of two-dimensional fundamental (and higher mode) solutions for which the filament transverse profile (not Gaussian in general) depends on the following quantities: density of saturable absorbers, laser detuning from resonance, laser power, and natural linewidth. (In contrast the Kerr solution does not have a unique filament diameter.) Emphasis will be placed on propagation of Gaussian incident beams; deviations from the stationary solution in either shape or power generally give rise to oscillating spatial patterns, including donutlike profiles, or beam breakup.
For pt.I see ibid., vol.8, no.3, 339 (1975). The transient behaviour of two short optical pulses in two-photon coherent propagation is obtained by calculating numerically the coherent propagation equations which couple the two electromagnetic pulses and the atomic system in self-consistent fashion. The coherent interaction of the two different frequency pulses gives rise to lossless propagation in the absorptive medium. This description is characterized by a two-photon area theorem. Novel coherent propagation effects of peak amplification and multiple pulse breakup are found. These effects are ascribed to two-photon self-induced transparency analogous to that of a one-photon transition in a two-level system. A difference of input intensity between the two different frequency pulses yields curious modulation effects involving sharp peak amplification and marked pulse breakup for the low-intensity input. In contrast, the high-intensity input pulse displays a smooth variation with distance and time. Low-loss pulse transmission above threshold, and pulse advance and delay are found for the present case in contrast to that for one-photon self-induced transparency.
The generation of an optical breather in coherent, resonant pulse propagation is studied. The initial field envelope is assumed to be in the form of a hyperbolic secant, with one half inverted so that the total area of the pulse is equal to zero. The Maxwell–Bloch equations for an inhomogeneously broadened atomic line are solved by the inverse-scattering method for all values of the independent variables x and t. The scattering amplitudes are found for any value θ of the absolute area of the initial pulse. For θ = 2πn the reflection coefficients are rational functions of the spectral parameter, and the inverse problem can be solved exactly. It is shown that the x-dependent poles of the reflection coefficients are responsible for the transient pulse shape. Such poles appear only in the presence of inhomogeneous broadening. The threshold for transparency is found at θ = 2π. At this value of the area, a breatherlike decaying solution is obtained. At θ = 4π a breather appears. Its energy amounts to approximately 70% of the initial pulse energy. For θ = 2π and 0 = 4π the solutions are analyzed in detail.
In this paper we develop a theoretical analysis which describes a coherent transient effect of two entering pulses---one laser and one Stokes---in a Raman-active medium. The field (Maxwell) and atomic (Schr\"odinger, density-matrix representation) equations are coupled in a self-consistent manner in time and space by virtue of the resultant second-order nonlinear macroscopic polarizations at the two frequencies. This treatment is accomplished under the circumstances where atomic coherence plays a predominant role. The equations derived here may be referred to as "Raman Bloch-Maxwell equations." The resultant equations yield a new aspect of transient stimulated Raman scattering and thus coherent Raman propagation. The transient-pulse behavior may be understood as self-induced modulation of coherent amplification and absorption. The self-induced modulation for the step-function input pulse is described by a combination of Jacobian elliptic functions depending on the input intensity. Computer calculations of transient-pulse evolution reveal interesting pulse breakup phenomena with peak amplification, energy transmission, pulse advance or delay, and pulse-narrowing effects.
The authors develop a theoretical analysis which describes coherent nonlinear resonant effects where two optical pulses of different frequencies undergo two-photon self-induced transparency (two-photon SIT) in an inhomogeneously broadened three-level system. The field (Maxwell) and atomic (Schrodinger; density matrix representation) equations are coupled in a self-consistent manner by virtue of the resultant macroscopic polarizations at the two frequencies. This treatment is accomplished under circumstances where atomic coherence plays a predominant role. The resulting equations yield a new two-photon area theorem which gives first the intensity dependent, two-photon absorption law analogous to Beer's law for the one-photon transition. Secondly, a 2 pi Lorentzian pulse solution is derived which propagates without loss at the modified pulse velocity.
Reverse-saturable absorbers are of considerable interest for optical limiting. Using the electric dipole perturbation, we derived the rate equation for a five-level system describing reverse-saturable absorbers. Traditional theories for the propagating laser beam in these materials are expressed in terms of the optical intensity. However, with the introduction of high-power short-pulsed lasers, the propagation of light in these materials may be subject to nonlinear phenomena such as self-focusing and self-phase modulation. Furthermore, conventional theories treat the laser light as a continuous wave or as a very broad temporal pulse in which dispersive effects are neglected. In order to incorporate these other nonlinear or dispersive effects, and therefore determine their influence in reverse-saturable absorbers, we derived an equation for the propagation of the electromagnetic field, rather than the intensity, coupled to the rate equations for a five-level system. We also coupled our theory to experimentally measurable parameters for these materials and detailed the various physical approximations used to obtain the rate equations.