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Journal of Experimental and Theoretical Physics Letters

Aging and memory effects in the nonequilibrium critical behavior of structurally disordered magnetic materials in the course of their evolution from the low-temperature initial state

Vladimir V. Prudnikov, Pavel Vladimirovich Prudnikov, Evgenii A. Pospelov, P. N. Malyarenko

Published Aug 1, 2015• 9 citations
Publisher

Abstract

The Monte Carlo study of the nonequilibrium critical evolution of structurally disordered anisotropic magnetic materials from the low-temperature initial state with the reduced magnetization m 0 = 1 is performed within the broad range of spin densities, p = 1.0, 0.95, 0.8, 0.6, and 0.5. It is shown that, in such systems, the pinning of domain walls by structural defects occurring when the evolution starts from the low-temperature state leads to significant changes in the nonequilibrium “aging” and “memory” effects in comparison to those characteristic of the “pure” system. As a result, in the long-term regime at times t–t w » t w » 1, an anomalously strong slowing down in the correlation effects is revealed. It is shown that a decrease in the autocorrelation function with time occurs according to a power law typical of the critical relaxation of the magnetization in contrast to a usual scaling dependence. Eventually, the limiting value of the fluctuation–dissipation ratio X∞ for the structurally disordered systems with p < 1 vanishes, whereas for the pure system, we have X∞ = 0.784(5). The nonequilibrium critical “superaging” stage is found. This stage is characterized by the critical exponent µ = 2.30(6) for weakly disordered systems and by µ = 2.80(7) for the systems with strong disorder.

DOI
10.1134/s0021364015150072

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The Monte Carlo study of the nonequilibrium critical evolution of structurally disordered anisotropic magnetic materials from the low-temperature initial state with the reduced magnetization m 0 = 1 is performed within the broad range of spin densities, p = 1.0, 0.95, 0.8, 0.6, and 0.5. It is shown that, in such systems, the pinning of domain walls by structural defects occurring when the evolution starts from the low-temperature state leads to significant changes in the nonequilibrium “aging” and “memory” effects in comparison to those characteristic of the “pure” system. As a result, in the long-term regime at times t–t w » t w » 1, an anomalously strong slowing down in the correlation effects is revealed. It is shown that a decrease in the autocorrelation function with time occurs according to a power law typical of the critical relaxation of the magnetization in contrast to a usual scaling dependence. Eventually, the limiting value of the fluctuation–dissipation ratio X∞ for the structurally disordered systems with p < 1 vanishes, whereas for the pure system, we have X∞ = 0.784(5). The nonequilibrium critical “superaging” stage is found. This stage is characterized by the critical exponent µ = 2.30(6) for weakly disordered systems and by µ = 2.80(7) for the systems with strong disorder.
Abstract A numerical Monte Carlo study has been performed on the influence of various initial states, easy-axis-type magnetic anisotropy, and structural defects on a nonequilibrium critical behavior of the classical three-dimensional Heisenberg model. An analysis of the time dependence of the magnetization and the autocorrelation function for the isotropic Heisenberg model shows substantial influence of the initial states on the relaxation of the magnetization and the aging effects in the behavior of the autocorrelation function, which are characterized by anomalous slowing down of the relaxation and correlation in the system as the waiting time increases. The study of the anisotropic Heisenberg model shows that the behavior of the magnetization and the autocorrelation function in a long-time regime is characterized by the critical exponents of the three-dimensional Ising model with a faster time decay of the autocorrelation function than that for the isotropic model. It has been revealed that the existence of structural defects in the case of the evolution of the system from the low-temperature initial state leads to an anomalously significant slowing down of the autocorrelation function. These features in the behavior of the autocorrelation function are characterized by the “superaging” effect with “superaging” exponent μ = 2.6(1) and related to the pinning of domain walls on structural defects during a nonequilibrium change in the domain structure of the system. In the case of evolution from the high-temperature initial state, the structural defects enhance the aging effect in the aging regime but their influence is irrelevant in the long-time regime.
A numerical Monte Carlo study of different initial states, magnetic anisotropy of “easy axis” type, and structural defects influence on non-equilibrium critical behavior of the classical three-dimensional Heisenberg model has been carried out. Analysis of time dependence of the magnetization and the autocorrelation function for isotropic Heisenberg model has shown strong influence of initial states on relaxation of the magnetization and aging effects in behavior of the autocorrelation function, which are characterized by anomalous slowing down of relaxation and correlation in system with increasing waiting time. Study of the anisotropic Heisenberg model with magnetic anisotropy of “easy axis” type has revealed that behavior of the magnetization and autocorrelation function in long-time regime is characterized by critical exponents of the three-dimensional Ising model and more fast decay of the autocorrelation function than for isotropic Heisenberg model. It has been revealed that in structurally disordered isotropic Heisenberg model relaxing from the low-temperature initial state, the significant changes of non-equilibrium aging phenomena in comparison with pure model are observed due to the pinning of domain walls on defects. It has been shown that during this relaxation process a strong slowing-down of time dependence of the autocorrelation function is realized. As a result, superaging effects occur in long-term behavior of the autocorrelation function with values of the superaging exponent μ=2.6(1). During evolution of system from high-temperature initial state, the presence of structural defects leads to increase of aging effects in aging regime, but their influence is found irrelevant in long-time regime.
Abstract We have performed a numerical investigation of the influence of disorder on the dynamical non-equilibrium evolution of a 3D site-diluted Ising model from a low-temperature initial state with magnetization m 0 = 1. It is shown that two-time dependences of the autocorrelation and integrated response functions for systems with spin concentrations p = 1.0, 0.95, 0.8, 0.6 and 0.5 demonstrate ageing properties with anomalous slowing-down relaxation and violation of the fluctuation-dissipation ratio. It was revealed that during non-equilibrium critical dynamics in the long-time regime t − t w ≫ t w ≫ 1 the autocorrelation functions for diluted systems are extremely slow due to the pinning of domain walls on impurity sites. We have found that the fluctuation-dissipation ratio X ∞ = 0 for diluted systems with spin concentration p < 1 while the pure system is characterized by X ∞ = 0.784 ( 7 ) . The autocorrelation function power-law delay becomes the same as for the time dependence of the magnetization in the critical point and is characterized by exponent − β / z ν . Also, for diluted systems we reveal memory effects for critical evolution in the ageing regime with realization of cyclic temperature change and quenching at T < T c .
The effect of various initial magnetizations m0 and structural defects the nonequilibrium critical behavior of the three-dimensional Ising model is numerically studied. Based on an analysis of the time dependence of the magnetization and the two-time dependence of the autocorrelation function and dynamic susceptibility, the significant effect of initial states on relaxation magnetizations and aging effects characterized by anomalous relaxation inhibition and correlation in the system with increasing waiting time was revealed. The fluctuation–dissipation theorem violation was studied, and the values of the limit fluctuation–dissipation ratio (FDR) are calculated. It is shown that two universality subclasses can be distinguished in the nonequilibrium critical behavior of the three-dimensional Ising model with random initial magnetization m0 These subclasses correspond to the system evolution from the high-temperature (m0 = 0) and low-temperature (m0 = 1) initial states with limit FDRs characteristic of these states.
A Monte Carlo numerical simulation of the specific features of nonequilibrium critical behavior is carried out for the two-dimensional structurally disordered XY model during its evolution from a low-temperature initial state. On the basis of the analysis of the two-time dependence of autocorrelation functions and dynamic susceptibility for systems with spin concentrations of p = 1.0, 0.9, and 0.6, aging phenomena characterized by a slowing down of the relaxation system with increasing waiting time and the violation of the fluctuation–dissipation theorem (FDT) are revealed. The values of the universal limiting fluctuation–dissipation ratio (FDR) are obtained for the systems considered. As a result of the analysis of the two-time scaling dependence for spin–spin and connected spin autocorrelation functions, it is found that structural defects lead to subaging phenomena in the behavior of the spin–spin autocorrelation function and superaging phenomena in the behavior of the connected spin autocorrelation function.
The Monte Carlo study of nonequilibrium memory effects in the two-dimensional pure and structurally disordered XY model in the low-temperature Berezinskii phase has been performed. Features of the correlation between memory and aging effects have been demonstrated. A qualitatively novel phenomenon for memory effects has been revealed: dynamic curves of the autocorrelation function in the thermal cycling time interval tend to the dynamic curves with the initial temperature. A unique implementation of memory effects has been demonstrated at both cooling and heating cycling of the system under the condition that cooling and heating temperatures are in the low-temperature Berezinskii phase. The influence of structural disorder on memory effects has been analyzed. It has been found that they are enhanced in the structurally disordered system owing to the enhancement of aging effects.