We examine the problem of line competition in an off-resonantly pumped three-level loop configuration that is encountered in four-wave mixing. Population and coherence pulsations play a key role during the competition. Analytical results in the small-signal-gain region provide some insight into the start-up of the loop oscillation. The general problem with saturating fields and strong line competition is solved numerically. We show that in the asymptotic regime of oscillation all the lines may survive, although some of them remain quite weak. We show also that our results are compatible with recent experiments.
We examine the problem of line competition in an off-resonantly pumped three-level loop configuration that is encountered in four-wave mixing. Population and coherence pulsations play a key role during the competition. Analytical results in the small-signal-gain region provide some insight into the start-up of the loop oscillation. The general problem with saturating fields and strong line competition is solved numerically. We show that in the asymptotic regime of oscillation all the lines may survive, although some of them remain quite weak. We show also that our results are compatible with recent experiments.
Exploring intermixing and interplay between different frequency-mixing processes has always been one of the interesting subjects at the interface of nonlinear optics with quantum optics. Here we investigate coherent competition and control between three-wave mixing (TWM) and four-wave mixing (FWM) in a cyclic $\mathrm{\ensuremath{\Delta}}$-type three-level superconducting quantum system. In the weak control-field regime, strong competition leads to an alternating oscillation between TWM and FWM signals and this oscillation is a signature of strong energy exchange between these two nonlinear processes. In particular, such oscillation is absent from conventional multiwave mixing in atomic systems. Surprisingly, synchronous TWM and FWM processes are demonstrated in the strong control-field regime and, at the same time, their efficiencies can be as high as 42 and 47%, respectively. Our paper shows that these competitive behaviors between TWM and FWM can be manipulated by tuning the control-field intensity.
In weakly, off-resonantly pumped multilevel systems gain is usually observed at the transition frequencies (line-center lines) and at the pump-offset-dependent frequencies (Raman lines). Modes developing at these frequencies are subject to strong mutual competition due to several coupling mechanisms. A general six-level system is investigated in this paper. Line competition effects are studied in particular in the simplified basic four-level cases comprising parallel, cascade, and V-\ensuremath{\Lambda} subsystems. We predict the type of transitions which survive and ultimately remain active. A comparison with experimental results using far-infrared lasers is made.
A nonperturbative theoretical study of four-wave-mixing processes in four-level systems is presented. Using the density-matrix formalism, numerical results are obtained for two arbitrarily intense pump fields with the third field a weak probe. The fourth wave, radiated by the system, is obtained analytically for some special cases. We find, for different frequency detunings, Rabi frequencies, and relaxation rates that the line shapes exhibit: (i) dynamic Stark splitting and shifting, and merging of resonances; (ii) power broadening with two-photon antiresonance behavior resulting from a destructive interference between different contributions to the optical polarization; and (iii) extra resonances induced by field intensities and saturation processes.
In this paper we present theoretical calculations relating to pump-probe and four-wave mixing spectroscopy. In pump-probe spectroscopy, one measures the absorption profile for the situation when an arbitrary strong pump field drives a given transition and a probe (weak) field drives the same transition. We have studied the influence of level degeneracy and field polarization on pump-probe and four-wave mixing signals. Our results indicate that for some closed systems (no population loss to the reservoir) it is possible to observe resonances that are characterized by the ground state width. Previous calculations indicate that for a nondegenerate system this resonance can appear only for an open system, the so-called "pressure induced resonances.”1 Our result, which contradicts this conclusion, can be understood by noting the fact that there are in general three irreducible tensor2 (in general) contributions to the line shape (K = 0 population, K = 1 orientation, and K = 2 alignment). Thus, even if the system is closed for the population it may still remain open for orientation or alignment; this effect is responsible for the narrow resonance. Specific calculations are presented for J = 1/2 → 1/2 and J = 1→2 transitions.
We analyze the properties of phase-conjugate (PC) emission via resonant, Doppler-broadened, backward four-wave mixing in the saturation regime, when both counterpropagating pump waves are arbitrarily intense. One considers two atomic situations, either a four-level system modeled as a pair of uncoupled transitions, or a three-level system. The first case leads to an analytical expression of the PC field, for arbitrary pump intensities, in the Doppler limit. The second case, in general, necessitates a numerical solution, except in the asymptotic regime when one pump is very intense compared to the other one. One finds that both cases lead to quite similar predictions: (i) two-peaked or four-peaked emission line shape, depending on the forward to backward pump intensity ratio; (ii) the maximum of PC reflectivity is obtained for infinite backward saturation, but for a fi-p nite value of the forward pump intensity; (iii) for backward saturation, the emission line shape is practically independent of the forward pump intensity. Finally, the theoretical analysis is extended to the case of a saturating probe and its effect on emission line shape and PC reflectivity, as well as its application to the properties of emission processes involving higher-order optical susceptibilities (degenerate multiwave mixing).
The nonlinear response of a two-level system interacting with two pump beams of different frequencies is studied with a view to examine several recent experiments on nonlinear mixing of high orders, instabilities in homogeneously broadened lasers, and holes in homogeneous lines. Such a nonlinear response is calculated with use of the continued fractions given in our earlier work [J. Opt. Soc. Am. B1, 164 (1984)]. Saturation effects lead to the appearance of many structures at submultiples of the Rabi frequency. The origin of these subharmonics in nonlinear-response functions is explained. It is shown that collisions not only lead to hole burning at the line center for weak fields but can also lead in moderate fields to the appearance of structures at subharmonics of the Rabi frequency. Existence of collision-induced coherences similar to those in four-wave mixing is shown in six-wave mixing. Exact results for the degenerate nonlinear mixing of arbitrary order are presented for arbitrary values of field strengths. Saturating fields create holes at the line center of such nonlinear mixing signals. Gain profiles of two modes symmetrically displaced from line center are also given. Numerical results, with complete account of saturation and collisions, for a variety of nonlinear-response functions are presented.