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Optics Letters

Velocity-specific atomic-state selection in an atomic beam by continuous-wave optical pumping

Duncan G. Steel, R. A. McFarlane

Published Jan 1, 1983• 4 citations
Publisher

Abstract

We present experimental results demonstrating strong velocity-distribution modification in a specific atomic state using optical pumping between hyperfine split levels. These results show that the velocity of a specific state can be defined within 6%, corresponding to a local temperature of 1 K. The velocity-specific-state selection is accomplished by using a nearly effusive atomic beam of sodium and a single frequency-stabilized dye laser.

DOI
10.1364/ol.8.000033

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Chinese Physics Letters•May 1, 1995•1 citation
We present experimental results demonstrating strong velocity-distribution modification in a specific atomic state using optical pumping between hyperfine split levels. These results show that the velocity of a specific state can be defined within 6%, corresponding to a local temperature of 1 K. The velocity-specific-state selection is accomplished by using a nearly effusive atomic beam of sodium and a single frequency-stabilized dye laser.
We describe optically pumping a beam of sodium atoms to >96% mS and >92% mS, mI state selection. (We have accurately measured the population of every mS, mI state in the optically pumped beam.) For the optical pumping both ground hyperfine states are pumped, using single-mode cw dye-laser radiation tuned to the 3S1/2–3P1/2 transition that is phase modulated in a LiTaO3 crystal to produce first-order sidebands at approximately the 1772-MHz hyperfine splitting of the ground state. The z-directed optical pumping is performed in a z-directed magnetic field of ~5 G. The state-selected atoms then move, in ~1 cm, into an ~200 G, z-directed field. The downstream probe laser beam is scanned through the 3S1/2 (mS, mI) → 3P3/2 (mS′, mI) transitions, which are spectroscopically resolved at 200 G, and the fluorescence intensities portray the residual populations in each of the eight 3S1/2 states.
The wavefunction of a moderately cold atom in a stationary near-resonant standing light wave delocalizes very fast due to wave packet splitting. However, we show that frequency modulation of the field may suppress packet splitting for some atoms having specific velocities in a narrow range. These atoms remain localized in a small space for a long time. We propose that in a real experiment with cold atomic gas this effect may decrease the velocity distribution of atoms (the field traps the atoms with such specific velocities while all other atoms leave the field).
The wave function of a moderately cold atom in a stationary near-resonant standing light wave delocalizes very fast due to wave packet splitting. However, we show that frequency modulation of the field may suppress packet splitting for some atoms having specific velocities in a narrow range. These atoms remain localized in a small space for a long time. We propose that in a real experiment with cold atomic gas this effect may decrease the velocity distribution of atoms (the field traps the atoms with such specific velocities while all other atoms leave the field)
We present a new scheme of sub-Doppler laser cooling for atoms used in atomic frequency standards, particularly for 40Ca. We perform calculations concerning optical pumping via a velocity- selective state based upon velocity-selective coherent population trapping. Optical pumping on the Raman transition 41S0- 41P1-31D2 leads to population of the metastable singlet state followed by a decay into the metastable triplet state 4P1. The momentum distribution of atoms in that state (with a half-maximum width of about one corresponding photon recoil momentum) is a direct replica of the distribution of atoms in the 3D2 state.