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Optics Letters

Generation of phase-conjugated vector wave fronts in atomic vapors

S. Saikan, Masashi Kiguchi

Published Nov 1, 1982• 32 citations
Publisher

Abstract

Using counterrotating circularly polarized waves as the pumping sources, we have demonstrated the generation of phase-conjugated vector wave fronts in the D(2) resonance line of sodium. Experimental results that are consistent with the calculation of the third-order nonlinear susceptibility in atomic lines have been obtained.
DOI
10.1364/ol.7.000555

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It is often desirable that a phase conjugate mirror be able to correct for polarization distortions in addition to correcting for wavefront aberrations. Such a device is called a vector phase conjugate mirror. It has been predicted within the context of the third-order theory that vector phase conjugation can be achieved by degenerate four-wave mixing using atomic two-photon transitions between S-states.1 We recently developed a theory of the polarization properties of two-photon resonantly enhanced degenerate four-wave mixing which can treat saturation effects due to pump waves.2 Our results show that for the case of linear and parallel pump wave polarizations, vector phase conjugation occurs with high quality and high reflectivity for two-photon transitions for which the nonresonant Stark shift is very small. We have also found that for the case of circular and counterrotating pump wave polarizations, perfect vector phase conjugation occurs for equal pump wave intensities. We have studied experimentally the effects of saturation and Stark shifts for S → S two-photon transitions of atomic sodium. We have found that high fidelity vector phase conjugation can be obtained.
We have studied the polarization properties of phase conjugation by degenerate four-wave mixing resonantly enhanced by the sodium 3S1/2 → 6S1/2 two-photon-allowed transition. As predicted by third-order theories, this interaction leads to simultaneous conjugation of the optical wave front and state of polarization (vector phase conjugation) when the pump intensities are sufficiently weak. However, qualitatively different polarization behavior is observed for pump intensities near or above the two-photon saturation intensity.
We have studied the polarization properties of phase conjugation by degenerate four-wave mixing utilizing the 3S\ensuremath{\rightarrow}4S two-photon-allowed transition of sodium. We have observed high-fidelity vector phase conjugation (simultaneous conjugation of the optical wave front and the state of polarization) at a reflectivity of \ensuremath{\sim}1% for the case where the states of polarization of the two counterpropagating pump waves were circular and counterrotating. High-fidelity polarization conjugation with high reflectivity was obtained only when the forward pump wave was much stronger than the backward pump wave. To explain these results, it is necessary to include the effects of grating washout due to atomic motion in the theoretical analysis.
A study was made of the influence of autoionization-like resonances in the continuum, induced by strong optical radiation, on the nonlinear susceptibilities governing third harmonic generation and the optical activity of sodium vapor. It was demonstrated experimentally for the first time that it should be possible to study high-lying states of atoms and molecules by the method of nonlinear polarization spectroscopy of the fifth-order optical nonlinearity. The experimental results were compared with the theory. An analysis was made of the feasibility of using this effect for spectroscopy of the states in the continuum and for generation of short-wavelength radiation in gaseous media.