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Decoherence and relaxation of a pair of interacting spins coupled to independent environments

Peter Nägele

Published Jan 1, 2009• 0 citations
Publisher

Abstract

In this thesis, a scheme for calculating the dynamics of two coupled dissipative spins is developed, where each of the spins is coupled to its own boson bath. We derive analytic path sum results both in the Markov-regime and in the one-boson exchange regime. The analysis is also performed with the Bloch-Redfield method. It is shown that the two different approaches lead to identical results for the dynamics. This is not obvious a priori because both methods are based on different procedures. The path sum method gives detailed insight into the internal dynamics of two coupled spins because we consider every path sequence that contributes to the time evolution. While most studies of coupled spins are restricted to one type of coupling, e.g., Ising type, we will generalize here to linear combinations of possible couplings. Especially interesting is the occurrence of a frustration of decoherence, if the spins are interacting via a linear combination of longitudinal and transverse coupling and, when in addition, some of the eigenfrequencies become degenerate. Our analysis shows that degenerate but mutual exclusive ground states lead to increased coherence times. Maximization of coherence is one of the crucial goals of quantum state engineering. Another topic of interest is the impact of non-linear quantum environments, formed by surrounding dissipative spins. A distribution of bistable background charges is known to be responsible for $1/f$ noise in solid state devices, like the superconducting quantum interference devices. Since $1/f$ noise is seemingly the dominating source of decoherence at very low temperature, there is a profound theoretical interest in modeling it. Therefore, we analyze two interacting spins, where one of them is coupled to a boson bath and thereby represents a resonant non-linear quantum environment. We study the crossover from a non-linear to a linear bath and study the corresponding time scale for the relevant bath correlations. Interestingly, for large and increasing temperature we find a decreasing decoherence for the central spin.

DOI
10.18419/opus-4914

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In this thesis, a scheme for calculating the dynamics of two coupled dissipative spins is developed, where each of the spins is coupled to its own boson bath. We derive analytic path sum results both in the Markov-regime and in the one-boson exchange regime. The analysis is also performed with the Bloch-Redfield method. It is shown that the two different approaches lead to identical results for the dynamics. This is not obvious a priori because both methods are based on different procedures. The path sum method gives detailed insight into the internal dynamics of two coupled spins because we consider every path sequence that contributes to the time evolution. While most studies of coupled spins are restricted to one type of coupling, e.g., Ising type, we will generalize here to linear combinations of possible couplings. Especially interesting is the occurrence of a frustration of decoherence, if the spins are interacting via a linear combination of longitudinal and transverse coupling and, when in addition, some of the eigenfrequencies become degenerate. Our analysis shows that degenerate but mutual exclusive ground states lead to increased coherence times. Maximization of coherence is one of the crucial goals of quantum state engineering. Another topic of interest is the impact of non-linear quantum environments, formed by surrounding dissipative spins. A distribution of bistable background charges is known to be responsible for 1/f1/f1/f noise in solid state devices, like the superconducting quantum interference devices. Since 1/f1/f1/f noise is seemingly the dominating source of decoherence at very low temperature, there is a profound theoretical interest in modeling it. Therefore, we analyze two interacting spins, where one of them is coupled to a boson bath and thereby represents a resonant non-linear quantum environment. We study the crossover from a non-linear to a linear bath and study the corresponding time scale for the relevant bath correlations. Interestingly, for large and increasing temperature we find a decreasing decoherence for the central spin.
For the realistic theoretical descriptions of quantum devices, we have to take the unavoidable coupling to their surrounding environment into account. A lot of effort in theoretical physics has been made to describe decoherence effects and the corresponding quantum to classical transition in the past. In these studies, baths are coupled to certain observables making their behavior more classical. In the most general case, a quantum device is affected by environments coupled to different observables. In this thesis, we study the differences emerging from coupling the bath to different observables. In particular, we investigate the situation, where two baths are coupled simultaneously to two conjugate variables (e.g. xˆ and pˆ, denoted dissipative frustration). We study how the interplay of these two baths can lead to interesting effects. After an introduction of the topic, we discuss the results of this thesis in Part II and Part III. In Part II, we study the effect of quantum tunneling in presence of a dissipative interaction with two Ohmic environments to the position xˆ and/or to the momentum pˆ of a particle. In chapter 2, we consider a symmetric double well potential which is important in the context of coherent state preparation, as its ground state is a superposition of being in the left and in the right well. Using the semiclassical approximation to calculate instanton paths within the path integral method, we find that momentum dissipation enhances the coherent tunnel splitting. In presence of dissipative couplings to xˆ and pˆ, the momentum dissipation acts in favor of the delocalization of the particle shifting the critical coupling strength of the dissipative phase transition induced by the position dissipation. Chapter 3 contains a study of the escape rate out of a metastable well in presence of dissipation. Here we find that the incoherent tunneling rate is exponentially enhanced in presence of momentum dissipation. We further show that the influence of momentum dissipation depends on the slope of the part of barrier the particle escaping through. In presence of both dissipative couplings, we find a non-monotonic behavior of the escape rate as a function of the dissipative couplings strengths. In Part III, we show that it is possible to realize the situation of "dissipative frustration" in Josephson junction chains. In particular, we introduce charge dissipation as a physical realization of the afore introduced momentum coupling. After presenting the circuit elements needed for charge dissipation, we study a chain of Josephson junctions affected by Ohmic baths coupled to the charge and/or the phase. Using a self-consistent harmonic approximation, we determine the phase diagram at zero temperature which exhibits a quantum phase transition between an ordered phase, corresponding to the superconducting state, and a disordered phase, corresponding to the insulating state with localized superconducting charge. Interestingly, we find that the critical line separating the two phases has a non-monotonic behavior as a function of the dissipative coupling strength. Moreover, within the self-consistent harmonic approximation, we analyze the dissipation induced crossover between a first and second order phase transition, showing that dissipative frustration increases the range in which the phase transition is second order. The non-monotonic behavior is also reflected in the purity of the system that quantifies the degree of correlation between the system and the environment, and in the logarithmic negativity as an entanglement measure that encodes the internal quantum correlations in the chain.
We study the reduced dynamics of interacting spins, each coupled to its own bath of bosons. We derive the solution in analytic form in the white-noise limit and analyze the rich behaviors in diverse limits ranging from weak coupling and/or low temperature to strong coupling and/or high temperature. We also view the single spin as being coupled to a spin-boson environment and consider the regimes in which it is effectively nonlinear and in which it can be regarded as a resonant bosonic environment.
We study decoherence of one, two, and nnn non-interacting qubits. Decoherence, measured in terms of purity, is calculated in linear response approximation, making use of the spectator configuration. The environment and its interaction with the qubits are modelled by random matrices. For two qubits, numerical studies reveal a simple one to one correspondence between its decoherence and its internal entanglement decay. Using this relation we are able to give a formula for concurrence decay. For large environments the evolution induces a unital channel in the two qubits, providing a partial explanation for the relation above. Using a kicked Ising spin network, we study the exact evolution of two non-interacting qubits in the presence of a spin bath. We find that the entanglement (as measured by concurrence) of the two qubits has a close relation to the purity of the pair, and closely follows an analytic relation derived for Werner states. As a collateral result we find that an integrable environment causes quadratic decay of concurrence as well as of purity, while a chaotic environment causes linear decay. Both quantities display recurrences in some integrable environments. Good agreement with the results found using random matrix theory is obtained. Finally, we analyze decoherence of a quantum register in the absence of non-local operations. The problem is solved in terms of a sum rule which implies linear scaling in the number of qubits. Each term involves a single qubit and its entanglement with the remaining ones. Two conditions are essential: decoherence must be small and the coupling of different qubits must be uncorrelated in the interaction picture. We apply the result to the random matrix model, and illustrate its reach considering a GHZ state coupled to a spin bath.
We study the decoherence of a central spin-1∕21∕21∕2 induced by a spin bath with intrabath interactions. Since we are interested in the cumulative effect of interaction and disorder, we study baths comprising Ising spins with random ferromagnetic and antiferromagnetic interactions between the spins. Using the resolvent operator method which goes beyond the standard Born-Markov master equation approach, we show that, in the weak coupling regime, the decoherence of the central spin at all times is entirely determined by the local-field distribution or equivalently, the dynamical structure factor of the Ising bath. We present analytic results for the Ising spin chain bath at arbitrary temperature for different distributions of the intrabath interaction strengths. We find clear evidence of non-Markovian behavior in the low temperature regime. We also consider baths described by Ising models on higher-dimensional lattices. We find that interactions lead to a significant reduction of the decoherence. An important feature of interacting spin baths is the saturation of the asymptotic Markovian decay rate at high temperatures, as opposed to the conventional Ohmic boson bath.
Quantum information processing has greatly increased interest in the phenomenon of environmentally-induced decoherence. The spin boson model is widely used to study the interaction between a spin-modelling a quantum particle moving in a double well potential-and its environment-modelled by a heat bath of harmonic oscillators. This paper extends a previous analysis of the static spin boson study to the driven spin boson case, with the derivation of an exact integro-differential equation for the time evolution of the propagator of the reduced spin density matrix. This is the first main result. By specializing to weak damping we then obtain the next result, a set of Bloch-Redfield equations for the equilibrium fixed spin initial condition. Finally we show that these equations can be used to solve the classic dissipative Landau-Zener problem and illustrate these solutions for the weak damping case. The effect of dissipation is seen to be minimised as the speed of passage is increased, implying that qubits need to be switched as fast as possible.