Saturation and Stark splitting of an atomic transition in a stochastic field
A. T. Georges, P. Lambropoulos
The authors investigate the saturation and Stark splitting of an atomic transition in (i) a phase-diffusion field and (ii) a chaotic field of arbitrary bandwidth. The theory takes into account the infinite sequence of field-correlation functions. It is shown that a chaotic field is less effective than a phase-diffusion field in saturating a single- or multiphoton transition. This is contrary to the weak-field case, where the intensity fluctuations and the associated photon bunching make the chaotic field more effective in exciting a multiphoton transition. It is also shown that the Stark splitting of an atomic transition, as observed in double resonance, is influenced dramatically by the intensity fluctuations in the chaotic field.
Physical Review A•Sep 1, 1979•98 citations