Recent progress in quantum communication highlights the need of advanced non-Gaussian states exhibiting high purity and spatio-spectral single-mode characteristics. We employ tailored waveguides and photon counting to implement efficient state preparation suitable for quantum networks.
Advancements in photonic platforms have enabled the precise control of light’s spectral and temporal degrees of freedom, a capability crucial for the development of scalable quantum information systems. In this work, we address the challenge of implementing spectro-temporal mode-selective non-Gaussian quantum operations, specifically single-photon subtraction (SPS) and addition (SPA), in the telecom wavelength regime. Building on prior experimental demonstrations of mode-selective near-infrared SPS, we present the first design framework for achieving mode-selective SPA and SPS using thin-film lithium niobate nonlinear waveguide platforms. We introduce an inverse-design optimization scheme by modeling the quantum-optical response via the joint spectral amplitude (JSA) and transfer function (TF), in order to identify optimal waveguide and pump parameters that maximize mode selectivity and state purity. This approach is first tested on a metallic waveguide design. We then exploit the dispersion engineering capabilities of thin-film waveguides, which offer enhanced nonlinear interactions through tighter light confinement. Our findings demonstrate that tailored nonlinear processes, particularly parametric down-conversion and frequency up-conversion, can support high-fidelity non-Gaussian operations essential for next-generation quantum photonic networks.
Continuous-variable quantum networks constitute a valuable resource for a wide range of quantum communication and information protocols. While frequency- and fast time-multiplexing enable the implementation of scalable quantum architectures, a precise characterization of multimode squeezed-light sources is essential. In this work, we increase both the spectral resolution and the measured squeezing values. Both parameters are relevant for the improved generation of so-called cluster states, a key resource for measurement-based quantum computing. Our source is based on parametric down-conversion in a periodically poled KTP waveguide pumped by a pulsed laser. The source produces squeezed states over a specific set of optical spectra. Increased spectral resolution in spectrally resolved homodyne detection allowed us to enhance the squeezing per spectral mode, increasing it from 1 dB to more than 2.4 dB in the first mode when measuring with a homodyne detector with a bandwidth of a few MHz. Secondly, we implemented a pulse-by-pulse characterization of the resource using a fast homodyne detector with an electronic bandwidth on the order of the laser repetition rate (100 MHz). Using this approach, the fast measurements revealed squeezing values of up to 1.5 dB in the first few spectral modes. To fully access the multimode quantum resource and ultimately improve the amount of squeezing, a high quantum efficiency is required. To avoid limitations imposed by poor spatial mode matching between the quantum resource and the local oscillator in homodyne detection, we implemented a wavefront-shaping scheme to characterize and control both the intensity profile and phase of the local oscillator. In preliminary tests this approach increased the mode-matching between the reference beam and the quantum signal by more than 8% while simultaneously providing a detailed characterization of the beam shape and of the influence of waveguide transmission on the beam profile. To achieve a genuine advantage in quantum information processing over classical protocols, the generation of non-Gaussian states is necessary. We therefore present a complete scheme for the creation of non-Gaussian states in a multimode system via mode-selective single-photon addition and subtraction, implemented through nonlinear optical processes in second-order nonlinear materials. We introduce a simulation framework applied to our squeezing source, which can be adapted to other regimes as well. Based on this framework, we are able to predict specific waveguide configurations that enable full control over the generated quantum states while maintaining high purity, with each process exhibiting a Schmidt number close to K=1, corresponding to effective single-mode addressing. generated quantum states while maintaining high purity, with each process exhibiting a Schmidt number close to K=1, corresponding to effective single-mode addressing.
Hybrid quantum information processing combines the advantages of discrete and continues variable protocols by realizing protocols consisting of photon counting and homodyne measurements. However, the mode structure of pulsed sources and the properties of the detection schemes often require the use of optical filters in order to combine both detection methods in a common experiment. This limits the efficiency and the overall achievable squeezing of the experiment. In our work, we use photon subtraction to implement the distillation of pulsed squeezed states originating from a genuinely spatially and temporally single-mode parametric down-conversion source in non-linear waveguides. Due to the distillation, we witness an improvement of 0.17 dB from an initial squeezing value of -1.648 ± 0.002 dB, while achieving a purity of 0.58, and confirm the non-Gaussianity of the distilled state via the higher-order cumulants. With this, we demonstrate the source's suitability for scalable hybrid quantum network applications with pulsed quantum light.