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Physical Review A

Observation of picosecond superfluorescent pulses in rubidium atomic vapor pumped by 100-fs laser pulses

Gombojav O. Ariunbold, Michael M. Kash, Vladimir A. Sautenkov, Hebin Li, Yuri V. Rostovtsev, George R. Welch, Marlan O. Scully

Published Oct 20, 2010• 52 citations
Publisher

Abstract

We study the superfluorescence (SF) from a gas of rubidium atoms. The atoms of a dense vapor are excited to the $5D$ state from the $5S$ state by a two-photon process driven by 100-fs laser pulses. The atoms decay to the $6P$ state and then to the $5S$ state. The SF emission at 420 nm on the $6P$--$5S$ transition is recorded by a streak camera with picosecond time resolution. The time duration of the generated SF is tens of picoseconds, which is much shorter than the time scale of the usual relaxation processes, including spontaneous emission and atomic coherence dephasing. The dependence of the time delay between the reference input pulse and SF is measured as a function of laser power. The experimental data are described quantitatively by a simulation based on the semiclassical atom-field interaction theory. The observed change in scaling laws for the peak intensity and delay time can be elucidated by an SF theory in which the sample length is larger than the cooperation length.

DOI
10.1103/physreva.82.043421

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We study the superfluorescence (SF) from a gas of rubidium atoms. The atoms of a dense vapor are excited to the 5D5D5D state from the 5S5S5S state by a two-photon process driven by 100-fs laser pulses. The atoms decay to the 6P6P6P state and then to the 5S5S5S state. The SF emission at 420 nm on the 6P6P6P--5S5S5S transition is recorded by a streak camera with picosecond time resolution. The time duration of the generated SF is tens of picoseconds, which is much shorter than the time scale of the usual relaxation processes, including spontaneous emission and atomic coherence dephasing. The dependence of the time delay between the reference input pulse and SF is measured as a function of laser power. The experimental data are described quantitatively by a simulation based on the semiclassical atom-field interaction theory. The observed change in scaling laws for the peak intensity and delay time can be elucidated by an SF theory in which the sample length is larger than the cooperation length.
We demonstrate that collective atomic interferences can be investigated by measuring the superfluorescence (SF) time delay. A pair of broadband (≈20 nm), ultrashort (≈80 fs), collinear pulses with a variable delay coherently excites rubidium (Rb) atoms. The generated superfluorescent pulses at 420 nm on the cascade transition are recorded by a picosecond streak camera. Both intensity and SF time delay of the 420 nm pulse are altered as the delay between input pulses varies. In particular, the SF time delay of the normalized 420 nm pulse exhibits oscillations with different periods. This can be understood in terms of atomic and quantum interferences due to two possible two-photon excitation pathways through the intermediate levels (Rb D-lines).
We report the observation of coherent UV light pulses by the coherent scattering of IR pulses from atomic rubidium vapor. Rubidium atoms were first excited by a 100 fs pulse from the 5S ground state to the 5D state via a two-photon transition. The atoms were then pumped by an IR pulse resonant to the 5D–12P transition. The presence of the IR pulse triggered the instantaneous emission of a UV light pulse on the 12P–5S transition. The pulse had a time duration of tens of picoseconds, which was measured by a picosecond-resolution streak camera. The temporal shape of the generated light is explained by a simplified atom–field interaction theory.
We study superfluorescence (SF) from spherical and cigar-shaped clouds of laser-cooled Rubidium atoms from the 5D5/25{D}_{5/2}5D5/2​ level through the 6P3/26{P}_{3/2}6P3/2​ level to the 5S1/25{S}_{1/2}5S1/2​ ground level. The atomic system is initially excited to the 5D5/25{D}_{5/2}5D5/2​ level from the ground state via two-photon excitation through the intermediate 5P3/25{P}_{3/2}5P3/2​ level. The fluorescence on the $6P\text{\ensuremath{-}}5S$ transition at 420 nm is recorded using time-resolved measurements. The time delays of the observed SF emission peaks typically scale as $\ensuremath{\sim}{N}^{\ensuremath{-}1}$, where NNN is the atom number, and are much smaller than the time delay expected for uncorrelated cascade fluorescence. Since NNN is significantly smaller than the threshold number for SF on the 420 nm transition, and larger than the threshold number for the $5D\text{\ensuremath{-}}6P$ transition at $5.2\text{ }\ensuremath{\mu}\text{m}$, our observations suggest that the 420 nm SF emission is triggered by rapid deexcitation of the 5D5D5D to the 6P6P6P level via SF at $5.2\text{ }\ensuremath{\mu}\text{m}$. The observed SF time delays for 420 nm emission agree with SF time-delay estimates for the $5.2\text{ }\ensuremath{\mu}\text{m}$ transition. For spherical clouds, the SF is isotropic. For cigar-shaped clouds, the SF is highly anisotropic. Along the long axis of cigar-shaped atom clouds, SF and incoherent cascade fluorescence produce temporally well-resolved peaks in the detected signal. In this case, the SF component of the signal is highly concentrated along a direction in between the directions of the two almost parallel excitation beams. The observed SF intensities scale as NNN, suggesting that the 5D5D5D level is regeneratively pumped during the SF decay.
The conventional method to measure atomic interference is usually based on incoherent processes which can be scaled by nano or microseconds. However, atomic interference may be studied in association with coherent process such as superfluorescence. Producing superfluorescent picosecond pulses in 87Rb vapor pumped by ~100 fs laser pulses, we report an observation of quantum beat due to D-lines. The relative delay of the superfluorescent pulses is measured by the streak camera with picosecond time resolution, as a function of time interval between input pulses, which also enables us to study atomic interference.
We investigated the superfluorescent decay process of dense rubidium atomic vapor in a cell. Using a femtosecond laser pulse, the atoms were excited from the 5 S ground state to the 6 P state. The 2.73 μ m and 1.37 μ m fields were generated on the cascaded decay, 6 P → 6 S → 5 P , which further stimulated the 780 nm forward emission on the 5 P → 5 S transition. Using sum frequency generation (SFG) spectroscopy, we observed all emission fields and the time delay between them, with sufficient temporal resolution. The experimental results were successfully reproduced using semiclassical simulations.
We investigate picosecond cooperative emission in an ensemble of rubidium atoms coherently excited by 100-fs laser pulses that are three-photon resonant to the 6P6P6P-5S5S5S transition. The emitted 420-nm light is recorded by a streak camera with 2-ps resolution. The resultant pulse shape shows ringing typical for superradiance in extended sample. The pulse shape is measured as a function of input power and is compared to the solutions of Maxwell-Bloch equations. The observed superradiance, which is in the low-excitation regime, is found to be closely related to optical precursor behavior.