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Optics Express

Fiber-microsphere system at cryogenic temperatures toward cavity QED using diamond NV centers

Hideaki Takashima, Takeshi Asai, Kiyota Toubaru, Masazumi Fujiwara, Keiji Sasaki, Shigeki Takeuchi

Published Jun 30, 2010• 15 citations
Publisher

Abstract

The coupling of a microsphere resonator to a tapered fiber was demonstrated at cryogenic temperatures (8 - 13 K) and investigated with a probe laser light whose frequency around the zero phonon line of nitrogen vacancy centers in diamond (638 nm). For this purpose, a liquid-helium-flow cryostat with a large sample chamber is developed and a resonance dip with a Q of 2 x 10(6) is observed. The resonance frequency and the coupling condition are found to be stable for a period of one hour.

DOI
10.1364/oe.18.015169

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The coupling of a microsphere resonator to a tapered fiber was demonstrated at cryogenic temperatures (8 - 13 K) and investigated with a probe laser light whose frequency around the zero phonon line of nitrogen vacancy centers in diamond (638 nm). For this purpose, a liquid-helium-flow cryostat with a large sample chamber is developed and a resonance dip with a Q of 2 x 10(6) is observed. The resonance frequency and the coupling condition are found to be stable for a period of one hour.
An ultrahigh-Q optical microcavity coupled with a tapered fiber is an ideal system for the cavity quantum electrodynamics (CQED). In particular realizing this system at cryogenic temperature is vitally important and has been recently explored for various CQED applications including solid-state atom-photon strong coupling, vibrational mode cooling, and photonic quantum gates. These cryogenic fiber-coupled microcavity systems, however, suffer from mechanical vibrations due to cooling systems and distortions caused by large temperature change. These factors may cause the degradation in polarization of probe light field in the system. Here we report the analysis of the polarization state in a tapered-fiber-coupled microsphere cavity at cryogenic temperatures. By scanning the wavelength of the probe light at around 637 nm, which can be used for the diamond nitrogen vacancy centers, the spectral analysis of the polarization state was performed at 8-30 K. We have found that the degree of polarization (DOP, classical analogue of purity) at cryogenic temperatures does not show significant change compared to that measured at room temperature. This fact indicates that the system can conserve the polarization at low temperature to the extent comparable to that at room temperature, which is enough for the evaluation of the quantum phase gate.
For cavity quantum electrodynamics systems (cavity-QED) to play a role in quantum information processing applications and in quantum networks, they must be robust and scalable in addition to having a suitable method for the generation, processing and storage of quantum bits. One solution is to develop a composite system that couples a nitrogen vacancy (NV) center in diamond to a whispering gallery mode supported by a fused silica microsphere. Such a system is motivated by the optical and electron-spin properties of the NV center. The NV center is the leading spin-qubit and exhibits atomic like linewidths at cryogenic temperatures and has spin coherence times greater than milliseconds at room temperature. These long coherence times, coupled with nanosecond scale spin readout and manipulation times, allow for millions of quantum operations to be processed. Silica whispering gallery resonators are the only class of microresonators with quality factor high enough to reach the strong coupling regime, which is necessary for some quantum information processing applications. \n \nIntegrating these two components into a system that could position a diamond nanopillar near the surface of a deformed-double stemmed microsphere system, with nanometer precision, at 10 K was a major achievement of this research. Cavity resonances in deformed microspheres can be excited with a free-space coupling technique which simplifies their integration into cryogenic environments. In these intentionally deformed resonators, an enhanced evanescent field decay length was observed at specific locations along the ray orbit. The double-stem arrangement enables the cavity resonance to be tuned over 450 GHz, with sub-10 MHz resolution, at 10 K. These two features, the enhanced decay length and broad range tuning with high resolution, are indispensible tools for cavity-QED studies with silica microspheres. \n \nDiamond nanopillars were fabricated from single crystal diamond with diameters as small as 140 nm in order to maintain a high quality factor. Studies were conducted on NV centers in nanopillars and bulk diamond to determine their suitability for cavity-QED applications. In an attempt to increase the light-matter interaction between NV centers and whispering gallery modes, diamond substrates were optically characterized that were irradiated with nitrogen ions.
We demonstrate successful cooling of ultrathin fiber tapers and their coupling with nitrogen vacancy (NV) centers in nanodiamonds at cryogenic temperatures. Nanodiamonds containing multiple NV centers are deposited on ultrathin fiber tapers with diameters ranging from 450-500 nm. The fiber tapers were successfully cooled down to 9 K with our special fiber mount and an optimization of cooling speed. The fluorescence coupled with the fiber tapers showed characteristic sharp zero-phonon lines of neutral and negatively charged NV centers. The present demonstration is important for the future NV-based quantum information devices and sensitive nanoscale cryogenic magnetometry.
We report the direct integration and efficient coupling of nitrogen vacancy (NV) color centers in diamond nanophotonic structures into a fiber-based photonic architecture at cryogenic temperatures. NV centers are embedded in diamond micro-waveguides (μWGs), which are coupled to fiber tapers. Fiber tapers have low-loss connection to single-mode optical fibers and hence enable efficient integration of NV centers into optical fiber networks. We numerically optimize the parameters of the μWG-fiber-taper devices designed particularly for use in cryogenic experiments, resulting in 35.6% coupling efficiency, and experimentally demonstrate cooling of these devices to the liquid helium temperature of 4.2 K without loss of the fiber transmission. We observe sharp zero-phonon lines in the fluorescence of NV centers through the pigtailed fibers at 100 K. The optimized devices with high photon coupling efficiency and the demonstration of cooling to cryogenic temperatures are an important step to realize fiber-based quantum nanophotonic interfaces using diamond spin defect centers.
We demonstrate cooling of ultrathin fiber tapers coupled with nitrogen vacancy (NV) centers in nanodiamonds to cryogenic temperatures. Nanodiamonds containing multiple NV centers are deposited on the subwavelength 480-nm-diameter nanofiber region of fiber tapers. The fiber tapers are successfully cooled to 9 K using our home-built mounting holder and an optimized cooling speed. The fluorescence from the nanodiamond NV centers is efficiently channeled into a single guided mode and shows characteristic sharp zero-phonon lines (ZPLs) of both neutral and negatively charged NV centers. The present nanofiber/nanodiamond hybrid systems at cryogenic temperatures can be used as NV-based quantum information devices and for highly sensitive nanoscale magnetometry in a cryogenic environment.
Scalable quantum information processing using nitrogen-vacancy (NV) centers in diamond will be difficult without the ability to couple the centers to optical microcavities and waveguides. Here we present our preliminary result of coupling a single NV center in a nanoparticle to a silica microdisk at cryogenic temperatures. The cavity-coupled NV photoluminescence is coupled out of the cavity through a tapered fiber. Although the current system is limited by the spectral properties of the NV center and the Q of the cavity, efficient particle-cavity and cavity-waveguide coupling should lead to the realization of a "one-dimensional atom" as needed for CQED, enable single-shot electron-spin readout, and increase the probability of success in entanglement schemes based on single-photon detection.