We report the demonstration of the Autler-Townes splitting and Mollow absorption spectrum by means of coherent optical spectroscopy of a strongly driven quantum dot.
Quantum dots are typically formed from large groupings of atoms and thus may be expected to have appreciable many-body behavior under intense optical excitation. Nonetheless, they are known to exhibit discrete energy levels due to quantum confinement effects. We show that, like single-atom or single-molecule two- and three-level quantum systems, single semiconductor quantum dots can also exhibit interference phenomena when driven simultaneously by two optical fields. Probe absorption spectra are obtained that exhibit Autler-Townes splitting when the optical fields drive coupled transitions and complex Mollow-related structure, including gain without population inversion, when they drive the same transition. Our results open the way for the demonstration of numerous quantum level-based applications, such as quantum dot lasers, optical modulators, and quantum logic devices.
Based on a calculation model, we study the interference phenomena of serially coupled V-type and Λ-type triple quantum dots (CTQDs) driven simultaneously by a strong driving field and a weak probe field. Strongly depending on the configuration of the three-level CTQD, the probe absorption spectra, which are shown in the tunneling current, exhibit various quantum coherence properties. In the case where the two pairs of transitions of the CTQD have a small eigenfrequency difference Δω, the double-coupling effect of the driving field results in two Autler—Townes doublets and one weak Mollow triplet in one spectrum. With the value of Δω increasing, only one Autler—Townes splitting remains due to the single-coupling of the field. We also find that the effect of spontaneous emission of phonons may lead to an obvious background current, which can be used to distinguish which transition is driven by the driving field in experiment. The interesting quantum property of a CTQD revealed in our results suggests its potential applications in quantum modulators and quantum logic devices.
Summary form only given.It is well known that a strongly driven transition exhibits a doublet splitting when probed by a weak field, commonly known as AC Stark splitting. It can be observed either by probing the driven two-level itself (Mollow-type spectrum) or via a third level (Autler-Townes-type spectrum). These two type splittings can have very different characteristics, particularly when driven resonantly. The absorptive Mollow spectrum consists of two dispersion-like features, whereas for the Autler-Townes spectrum there is a simple doublet splitting. In this paper we report the observation of both Mollow and Autler-Townes spectrum simultaneously by applying two strong driving fields in a three-level configuration.