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Journal of Physics B Atomic Molecular and Optical Physics

Quantum statistical properties of the radiation field in spontaneous Raman and stimulated Raman processes

Biswajit Sen, Swapan Mandal, Jan Peřina

Published Mar 9, 2007• 18 citations
Publisher

Abstract

The initially prepared coherent state coupled to a third-order nonlinear medium is responsible for stimulated Raman and spontaneous Raman processes. By exploiting the analytical solutions of field operators for various modes, we investigate the quantum statistical properties for pure and two modes of the input coherent light responsible for stimulated Raman and spontaneous Raman processes. For spontaneous Raman processes the photons are unbunched for the pure and two-mode cases. By a suitable choice of phase, we obtain the bunching and antibunching of photons for stimulated Raman processes.

DOI
10.1088/0953-4075/40/7/010

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The initially prepared coherent state coupled to a third-order nonlinear medium is responsible for stimulated Raman and spontaneous Raman processes. By exploiting the analytical solutions of field operators for various modes, we investigate the quantum statistical properties for pure and two modes of the input coherent light responsible for stimulated Raman and spontaneous Raman processes. For spontaneous Raman processes the photons are unbunched for the pure and two-mode cases. By a suitable choice of phase, we obtain the bunching and antibunching of photons for stimulated Raman processes.
The light initially prepared in a coherent state runs the stimulated and spontaneous Raman processes in a second-order nonlinear medium. Using analytical expressions of field operators for the light modes, we determine the quantum statistical properties of the modes in the stimulated and spontaneous Raman processes. By a choice of phase, we obtain a boson-pair property correlating the pump and vibration modes and such a property correlating the pump and anti-Stokes modes. The Stokes and vibration modes exhibit the boson-pair property for all initial phase differences between the pump mode and the other ones. In the spontaneous Raman process only the Stokes and vibration modes show such a property.
An initially prepared coherent state coupled to a second-order nonlinear medium is responsible for stimulated and spontaneous hyper Raman processes. By using an intuitive approach based on perturbation theory, the Hamiltonian corresponding to the hyper Raman processes is analytically solved to obtain the temporal development of the field operators. It is true that these analytical solutions are valid for small coupling constants. However, the interesting part is that these solutions are valid for reasonably large time. Hence, the present analytical solutions are quite general and are fresh compared to those solutions under short-time approximations. By exploiting the analytical solutions of field operators for various modes, we investigate the squeezing, photon antibunching and nonclassical photon statistics for pure modes of the input coherent light responsible for hyper Raman processes. At least in one instance (stimulated hyper Raman processes for vibration phonon mode), we report the simultaneous appearance of classical (photon bunching) and nonclassical (squeezing) effects of the radiation field responsible for hyper Raman processes.
Coherent light coupled to a third-order nonlinear medium is responsible for spontaneous and for stimulated Raman processes. The analytical solutions up to second order in coupling constants of various field modes for spontaneous Raman and for stimulated Raman processes are utilized to obtain the amplitude-squared and amplitude-cubed squeezing of the input coherent light. The amplitude-squared and amplitude-cubed squeezing are completely ruled out for all modes for spontaneous Raman processes. For stimulated Raman processes, we observe that the squeezing for amplitude-squared and amplitude-cubed are possible for pump and for vibrational phonon modes. It is found that the percentage of higher ordered amplitude squeezing decreases with the increase of the orders. The squeezing in Stokes and in anti-Stokes modes are ruled out even for stimulated Raman processes.
The quantum statistical properties of a single mode of the radiation field, prepared in the coherent state, interacting with a nonlinear medium of inversion symmetry are studied with the help of the usual two photon correlation function for zero time delay. We report the photon antibunching and sub-Poissonian photon statistics in addition to the usual photon bunching and the super-Poissonian photon statistics for an input vacuum field. The manipulation of the phase of input coherent light gives rise to the well known self induced transparency. The possible physical explanations for these events are presented.
We develop the quantum theory of stimulated hyper-Raman scattering (HRS) and discuss the quantum statistics of pump and Stokes fields. We show that the initially coherent pump field acquires a strong squeezing that exceeds the similar squeezing in other nonlinear processes also involving two-photon absorption. Stokes field statistics are analysed in detail as a function of the initial statistics of both modes. Bunching effects are shown to be amplified in the short-time region, while in asymptotics the antibunching of Stokes photons becomes dominant, which in many cases results in sub-Poissonian statistics of Stokes mode. We also find a number of correlation effects between the photons of the two modes.
The Hamiltonian and the equations of motion for various modes involving spontaneous and stimulated Raman processes are derived. The coupled differential equations involving these modes are solved analytically by using an intuitive approach (IA). The solution of the present paper does not require any short time approximation. As a matter of fact, the present solution for field operators and hence the squeezing for various modes are valid for all interaction time t. In this way, the present paper is more general compared to the earlier investigations where short-time approximations were found a must. By exploiting the solutions for the field operators, we obtain the squeezing effects of input coherent light for pure and for mixed field modes. The IA employs the perturbation theory and hence we came across the secular terms in the solution. Of course, for small coupling constants these secular terms could be summed for all orders. To establish our claim, we remove the secular terms at least for one occasion.