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Science

Bose-Einstein Condensation of Molecules

Selim Jochim, M. Bartenstein, A. Altmeyer, G. Hendl, S. Riedl, Cheng Chin, Johannes Hecker Denschlag, Rudolf Grimm

Published Nov 17, 2003• 1,186 citations
Publisher

Abstract

We report on the Bose-Einstein condensation of more than 10(5) Li2 molecules in an optical trap starting from a spin mixture of fermionic lithium atoms. During forced evaporative cooling, the molecules are formed by three-body recombination near a Feshbach resonance and finally condense in a long-lived thermal equilibrium state. We measured the characteristic frequency of a collective excitation mode and demonstrated the magnetic field-dependent mean field by controlled condensate spilling.

DOI
10.1126/science.1093280

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We report on the Bose-Einstein condensation of more than 10(5) Li2 molecules in an optical trap starting from a spin mixture of fermionic lithium atoms. During forced evaporative cooling, the molecules are formed by three-body recombination near a Feshbach resonance and finally condense in a long-lived thermal equilibrium state. We measured the characteristic frequency of a collective excitation mode and demonstrated the magnetic field-dependent mean field by controlled condensate spilling.
We have observed Bose-Einstein condensation of molecules. When a spin mixture of fermionic 6Li atoms was evaporatively cooled in an optical dipole trap near a Feshbach resonance, the atomic gas was converted into 6Li2 molecules. Below 600 nK, a Bose-Einstein condensate of up to 900 000 molecules was identified by the sudden onset of a bimodal density distribution. This condensate realizes the limit of tightly bound fermion pairs in the crossover between BCS superfluidity and Bose-Einstein condensation.
This thesis describes the production of molecular Bose-Einstein condensates (BEC) of 6Li2 dimers and binding energy measurements of p-wave Feshbach molecules. A σ− Zeeman slower is used to produce a continuous beam of isotopically enriched 6Li atoms at speeds low enough to load a magneto-optical trap (MOT). We currently have a flux of slowed atoms of ~ 5 · 106 atoms/s loading the MOT with more than 108 atoms. We then transfer up to 106 atoms in an almost equal spin mixture of the two lowest hyperfine states into an optical dipole trap. We achieved condensates in three different crossed optical dipole trap geometries. The initial low power optical dipole trap was formed using light from a 25WVersaDisk Yb:YAG laser at 1030 nm. It consisted of a 15 W beam crossed with a 13 W beam at about 80 degrees with a waist of approximately 30 μm in each beam. By translating the focus of the second beam we could change the trap geometry from near symmetric to elongated. Nowadays, we produce condensates in a crossed dipole trap formed by a 100 W fibre laser. Both arms are focussed to a waist of 40 μm, cross each other at 14 degrees and have laser powers of ~80 W and ~70 W, respectively. Evaporative cooling is achieved by reducing the laser power near the broad s-wave Feshbach resonance at 834 G. By tuning to the low magnetic field side (770 G) of the Feshbach resonance molecules are formed through three-body recombination at sufficiently low temperatures. Further evaporation leads to the creation of a molecular BEC. After reducing the laser power by a factor of about 1000 in approximately 3 s we have observed more than 30 000 condensed molecules. During the evaporation the temperature decreases from about 100 μK to below 100 nK. We present measurements of the binding energies of 6Li p-wave Feshbach molecules formed in combinations of the |F = 1/2,mF = +1/2i (|1i) and |F = 1/2,mF = −1/2i (|2i) states. The binding energies scale linearly with magnetic field detuning for all three resonances. The relative molecular magnetic moments are found to be 113 ± 7 μK/G, 111 ± 6 μK/G and 118 ± 8 μK/G for the |1i − |1i, |1i − |2i and |2i − |2i resonances, respectively, in good agreement with theoretical predictions.
We report on the achievement of Bose-Einstein condensation of erbium atoms and on the observation of magnetic Feshbach resonances at low magnetic fields. By means of evaporative cooling in an optical dipole trap, we produce pure condensates of 168Er, containing up to 7×10(4) atoms. Feshbach spectroscopy reveals an extraordinary rich loss spectrum with six loss resonances already in a narrow magnetic-field range up to 3 G. Finally, we demonstrate the application of a low-field Feshbach resonance to produce a tunable dipolar Bose-Einstein condensate and we observe its characteristic d-wave collapse.
The achievement of a Bose-Einstein condensate of cesium in the lowest internal state (F=3, m/sub F/=3) by evaporative cooling in an optical trap is reported. The corresponding scattering length shows a strong dependence on magnetic field, varying from large negative to large positive values in a conveniently accessible magnetic field range due to a unusual combination of broad and narrow Feshbach resonances. The inelastic processes resulting from this complex scattering behavior in thermal ensembles is studied. These measurements have been of crucial importance for identifying a suitable path in phase space towards condensation. In first experiments, the strong dependence of the condensate mean-field energy on the magnetic field is demonstrated. By briefly switching to different scattering lengths just before releasing the sample from the trap, imploding, exploding, and non-interacting 'frozen' condensates are produced. We will employ the tunable interaction in further experiments by looking at molecule formation on Feshbach resonances and exploring condensate dynamics at extreme values of the scattering length.