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IEEE Journal of Quantum Electronics

Nonperturbative theory of inhomogeneous effects in gas lasers

Susan M. Scott

Published May 1, 1968• 4 citations
Publisher

Abstract

The self-consistent field approximation (SCFA)[1]-[4] is used to calculate the steady-state mode energies and frequency shifts for a gas laser. The SCFA is a statistical approximation which was shown[3] to be accurate for small values of a parameter (\gamma^{2}N), which is always small for gas lasers. The SCFA is simpler and more convenient for studying the complicated dynamical effects that occur in gas lasers than the more recent[5]-[8] quantum theoretical models. It does not, of course, give any new description of the laser photon statistics, since the approximation treats the field as a pure coherent state[9] and is, therefore, equivalent to the semiclassical theory. The main results of this paper are to show how dynamical effects can be calculated nonperturbatively for arbitrary values of the field strength, and to analyze the different roles played by different kinds of inhomogeneous effects in gas lasers. These inhomogeneous effects are due to the dependence of the atomic inversion density on the atomic positions and velocities. Some numerical results are given which show that the nonperturbative theory can explain some effects not previously explained by perturbation theories. [1], [2].

DOI
10.1109/jqe.1968.1075137

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The self-consistent field approximation (SCFA)[1]-[4] is used to calculate the steady-state mode energies and frequency shifts for a gas laser. The SCFA is a statistical approximation which was shown[3] to be accurate for small values of a parameter (\gamma^{2}N), which is always small for gas lasers. The SCFA is simpler and more convenient for studying the complicated dynamical effects that occur in gas lasers than the more recent[5]-[8] quantum theoretical models. It does not, of course, give any new description of the laser photon statistics, since the approximation treats the field as a pure coherent state[9] and is, therefore, equivalent to the semiclassical theory. The main results of this paper are to show how dynamical effects can be calculated nonperturbatively for arbitrary values of the field strength, and to analyze the different roles played by different kinds of inhomogeneous effects in gas lasers. These inhomogeneous effects are due to the dependence of the atomic inversion density on the atomic positions and velocities. Some numerical results are given which show that the nonperturbative theory can explain some effects not previously explained by perturbation theories. [1], [2].
This paper presents a semiclassical theory of a single-mode gas laser valid for essentially arbitrary values of field intensity. The theory is formulated in terms of an ensemble-averaged form of the density-matrix equations of motion involving a single set of coordinates. The polarization and the population-inversion density are expanded in spatial Fourier components. One obtains a set of coupled difference equations in the Fourier coefficients yn{y}_{n}yn​, which may be solved subject to appropriate boundary conditions on yn{y}_{n}yn​ for large nnn. The solutions may be expressed in terms of continued fractions in the general case, and in closed form in important special cases. Quantities of interest are evaluated by computer. The steady-state laser intensity and frequency are obtained from the coupled electromagnetic field equations as functions of the cavity parameters and the linear gain of the amplifying medium. At moderate values of field intensity, the velocity distribution of the space-averaged population inversion density exhibits a fine structure for low-velocity atoms superimposed on the usual broader depletion. This structure is a manifestation of the coherent ringing of the amplifying medium. The results are compared with those obtained in the rate-equation approximation, and with the recent work of Stenholm and Lamb. Discrepancies with the latter paper are explained.
We show that in a gas laser the inhomogeneity in the distribution of amplifying atoms and the transverse Gaussian distribution of the saturating electromagnetic field give rise to different lens effects which are generally opposite to each other and influence the line shapes in different ways, shifting the Lamb dip either to the blue or to the red. For those laser phenomena which increase one or the other of the lens effects, the role of a diaphragm is of particular importance, since it determines the spatial distribution of the resonant field. We present here a new method for studying the resonant diffracted field in a laser. Also, we give a unified description of the various inhomogeneities. Doing away with the usual method of mean-field approximation, we numerically calculate, for a diaphragmed, monomode weak-gain gas laser, the intensity, variation of the beam diameter, and the radius of curvature as functions of the frequency.
This paper extends the calculations of the semiclassical Lamb theory of a Doppler-broadened gas laser (optical maser) to arbitrary intensities for the case of single-mode operation. The coupled equations of the classical electromagnetic field and an ensemble of two-level atoms are set up, and a solution is obtained in the form of a continued fraction. This is used to compute intensity-detuning curves and atomic population inversion densities as functions of both the velocity and the position in the laser. When the laser is tuned to resonance, the velocity dependence of the inversion density shows a previously unknown fine structure consisting of a "bump" in the bottom of the hole. The calculations are compared to results obtained from a perturbation expansion in powers of the field and exact results known for atoms with zero velocity. The response of the laser output to a slow modulation and the buildup of oscillations are also discussed.
Up to this point we have always assumed that all the atoms which interact with the radiation field have the same atomic transition frequency, with an atomic linewidth given by γ ⊥ . This configuration is called homogeneous broadening. However, in the great majority of lasers the linewidth is inhomogeneously broadened , because the atomic frequency follows a distribution. For example, in solid-state lasers such as the ruby laser and fiber lasers the inhomogeneity is due to the imperfections in the crystalline structure of the material. In gas lasers, where the atoms or molecules are free to move, the inhomogeneous broadening is due to the Doppler effect, for which a molecule moving with velocity v in a field of frequency ω and wave vector k experiences an effective frequency ω ′ = ω − k · v [8]. Since what matters is the difference between the atomic transition frequency and the field frequency, we can keep the field frequency fixed and imagine that the field interacts with different groups of atoms that move with different velocities and therefore have different transition frequencies. The realistic velocity distribution is a Gaussian, for which the corresponding distribution for the modulus of the velocity is Maxwellian. However, in the following we will mainly analyze the case of a Lorentzian distribution for the atomic transition frequency, because this allows an analytical treatment. Again for the sake of simplicity, we will limit our analysis to the case of a ring cavity. In Section 15.1 we will generalize to the inhomogeneous-broadening configuration the modal equations for the case of homogeneous broadening, which were formulated in Chapter 12. In Section 15.2 we will specialize to the single-mode model and discuss its stationary solutions for the laser case. Multimode dynamical equations The atomic transition frequency of the generic group of atoms is given by ω a + δ D , where ω a is the central atomic frequency and δ D takes positive and negative values. We call ω c the frequency of the cavity mode nearest to ω a and denote by δ ac the difference ω a − ω c .
The effects of phase-interrupting and velocity-changing collisions between active and perturber atoms on the spectral profile of a gas laser are studied. Exact analytical results for the density matrix are presented for the case of strong collisions in a unidirectional ring laser, and the laser intensity is then evaluated in the Doppler limit under the condition of self-consistency. The washout of the hole burning in the steady-state population difference and the broadening of the laser line shape are discussed. The results of the third-order perturbation theory are compared with the exact calculations valid for an arbitrarily intense pump.
A unified quantum treatment is presented for bidirectional two-mode ring lasers using the approach of Haken and co-workers. Equations of motion for the reduced density matrix of the field have been derived and used to study the fluctuation properties of the radiation field in different kinds of active media. The steady-state photon number distribution for an inhomogeneously broadened gas ring laser is derived. It is shown that for equal losses the relative fluctuations and normalized cross correlation of the photon numbers approach values 13\frac{1}{3}31​ and $\ensuremath{-}\frac{1}{3}$, respectively, for large excitations. For unequal losses the laser may emit typical single-mode laser radiation in the direction of the favored mode and typical equilibrium blackbody radiation in the direction of the weaker mode. Our results generally agree with the predictions of earlier treatments when the losses are equal. However, for unequal losses we predict different behavior for large excitations. Effects of detuning, spatial, and temporal variation of atomic inversion on the fluctuation properties have been investigated in the coherent-state diagonal representation of the density matrix, and steady-state intensity distributions have been derived for various kinds of active atoms. It is shown that for inhomogeneously broadened solid-state ring lasers spatial inhomogeneities may couple the modes strongly and the statistical properties of such lasers, characterized by a double-peaked intensity distribution and large relative-intensity fluctuations, may be similar to those of a homogeneously broadened ring laser. Curves are presented to illustrate the behavior.