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Journal of Modern Optics

Focusing on factorability: space–time coupling in the generation of pure heralded single photons

Peter J. Mosley, Jeff S. Lundeen, Brian J. Smith, Ian A. Walmsley

Published Nov 11, 2008• 2 citations
Publisher

Abstract

The interference of single heralded photons from multiple parametric downconversion sources requires photon pairs in factorable states. Typically, these are selected from an ensemble of pairs by narrow filters that remove any exhibiting correlations. In order to eliminate these lossy filters, factorable photon pairs free from any spatio-temporal correlations must be created directly at each source. This requires careful engineering of the group velocity dispersion of the nonlinear crystal in which pair generation takes place. Several schemes have been proposed to do this in the plane-wave regime, but in a realistic experiment one must also take into account the effects of focusing on the two-photon state. Focusing leads to space–time coupling between the pump structure and the downconverted pairs that has the potential to reduce their factorability, but if carefully managed can actually increase it. In this paper, we consider some of the effects of focusing and their consequences for pure single photon generation.

DOI
10.1080/09500340802187324

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The interference of single heralded photons from multiple parametric downconversion sources requires photon pairs in factorable states. Typically, these are selected from an ensemble of pairs by narrow filters that remove any exhibiting correlations. In order to eliminate these lossy filters, factorable photon pairs free from any spatio-temporal correlations must be created directly at each source. This requires careful engineering of the group velocity dispersion of the nonlinear crystal in which pair generation takes place. Several schemes have been proposed to do this in the plane-wave regime, but in a realistic experiment one must also take into account the effects of focusing on the two-photon state. Focusing leads to space–time coupling between the pump structure and the downconverted pairs that has the potential to reduce their factorability, but if carefully managed can actually increase it. In this paper, we consider some of the effects of focusing and their consequences for pure single photon generation.
From quantum computation to quantum key distribution, many quantum-enhanced applications rely on the ability to generate pure single photons. Even though the process of spontaneous parametric downconversion (SPDC) is widely used as the basis for photon-pair sources, the conditions for pure heralded single-photon generation, taking into account both spectral and spatial degrees of freedom, have not been fully described. We present an analysis of the spatio-temporal correlations present in photon pairs produced by type-I, non-collinear SPDC. We derive a set of conditions for full factorability in all degrees of freedom—required for the heralding of pure single photons—between the signal and idler modes. In this paper, we consider several possible approaches for the design of bright, fiber-coupled and factorable photon-pair sources. We show through numerical simulations of the exact equations that sources based on: (i) the suppression of spatio-temporal entanglement according to our derived conditions and (ii) a tightly focused pump beam together with optimized fiber-collection modes and spectral filtering of the signal and idler photon pairs, lead to a source brightness of the same order of magnitude. Likewise, we find that both of these sources lead to a drastically higher factorable photon-pair flux, compared to an unengineered source.
In an experiment reported recently (Mosley et al 2008 Phys. Rev. Lett. 100 133601), we demonstrated that, through group velocity matched parametric downconversion, heralded single photons can be generated in pure quantum states without spectral filtering. The technique relies on factorable photon pair production, initially developed theoretically in the strict collinear regime; focusing—required in any experimental implementation—can ruin this factorability. Here, we present the numerical model used to design our single photon sources and minimize spectral correlations in the light of such experimental considerations. Furthermore, we show that the results of our model are in good agreement with measurements made on the photon pairs and give a detailed description of the exact requirements for constructing this type of source.
Sources of single photons in pure quantum states are essential to many quantum optics applications. We explore a technique, known as group-velocity matching, that enables the heralded generation of pure single photons through nonlinear optical processes. It reduces or eliminates the requirement of spectral filtering that conventional sources rely on to achieve high purity, therefore increasing both heralding efficiency and photon flux. Implementation in both spontaneous parametric downconversion and spontaneous four-wave mixing is studied as we discuss several recent experimental realizations demonstrating purity of more than 0.84 for the heralded photons.
We present an experimental demonstration of heralded single photons prepared in pure quantum states from a parametric down-conversion source. It is shown that, through controlling the modal structure of the photon pair emission, one can generate pairs in factorable states and thence eliminate the need for spectral filters in multiple-source interference schemes. Indistinguishable heralded photons were generated in two independent spectrally engineered sources and Hong-Ou-Mandel interference observed between them without spectral filters. The measured visibility of 94.4% sets a minimum bound on the mean photon purity.
We explore a promising method of generating pure heralded single photons. Our approach is based on parametric down-conversion in a periodically-poled waveguide. However, unlike conventional downconversion sources, the photon pairs are counter-propagating: one travels with the pump beam in the forward direction while the other is backpropagating towards the laser source. Our calculations reveal that these downconverted two-photon states carry minimal spectral correlations within each photon-pair. This approach offers the possibility to employ a new range of downconversion processes and materials like PPLN (previously considered unsuitable due to its unfavorable phasematching properties) to produce heralded pure single photons over a broad frequency range.
Summary form only given. Parametric downconversion (PDC) allows the generation of highly coherent, spectrally pure single photons for quantum photonics. In a typical heralded PDC source, the signal photon emerges in a spectrally mixed state due to strong (anti)correlation in the joint spectrum of PDC photon pairs.One method for reducing spectral correlations is spectral filtering, but this compromises the heralding efficiency and the brightness of the source. A more sophisticated method for increasing the heralded photon purity is group-velocity matching, which works by erasing part of the timing information between the pump and PDC photons. What group-velocity matching cannot address, however, are the remaining correlations in the joint spectrum that come from the sinc-shaped phase-matching function (PMF) typical to standard PDC crystals. Further source engineering is therefore required to remove these correlations. Several studies have introduced domain-engineering techniques for shaping the phase matching function (PMF) in periodically poled crystals to improve single photon purities [1-4]. We present a new technique for tailoring crystal nonlinearities which combines the advantages of a deterministic method for domain engineering [4] and an annealing method developed for classical applications in higher-harmonic generation [5]. In our method, we first choose each domain orientation such that the generated field amplitude along the crystal matches the target field amplitude obtained by integrating the desired nonlinearity profile. Using a one-block structure instead of a two-blocks structure (as in [4]) results in a higher flexibility of the algorithm in tracking the target function and yields to more accurate results. We then use an annealing algorithm to slightly vary the width of each domain, further improving the effective PMF. Our technique outperforms its predecessors, particularly for short crystals, leading to high single photon purities, as shown in Fig.1. We experimentally characterise our method through a high-precision measurement of multiphoton interference between two heralded photons generated by two independent sources.We also notice that by considering a complex target field amplitude function it is possible to generalise the algorithm in [5] to any constant domain width (not necessarily equal to the coherence length), leading to a better approximation of the desired phase matching function, especially in the very short crystal regime. Moreover, tracking both the real and imaginary components of the target function allows us to approximate more exotic cases such as chirped nonlinearity profiles. Since scalable quantum photonics will require integrated architectures in which nonlinear processes are typically employed for single-photon generation, it will be interesting to explore new techniques similar to in-fibre Bragg grating structures which might yield quasi-periodic four-wave mixing and apply our algorithm to these new platforms.