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Soviet Journal of Quantum Electronics

Four-photon mixing and squeezed states in a resonator

А. В. Белинский, Anatolii S Chirkin

Published Oct 31, 1988• 2 citations
Publisher

Abstract

The problems of eigenfunctions and eigenvalues of the modes in a confocal resonator, where counterpropagating four-photon mixing takes place as a result of planar pumping, is solved at the quantum level. It is shown that the quadrature components of the waves generated in such a resonator have different losses and an analytical solution is obtained for these waves. This provides an opportunity to describe correctly the process of formation of squeezed states allowing for the spatial configuration of the waves interacting in such a resonator.

DOI
10.1070/qe1988v018n10abeh012582

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The problems of eigenfunctions and eigenvalues of the modes in a confocal resonator, where counterpropagating four-photon mixing takes place as a result of planar pumping, is solved at the quantum level. It is shown that the quadrature components of the waves generated in such a resonator have different losses and an analytical solution is obtained for these waves. This provides an opportunity to describe correctly the process of formation of squeezed states allowing for the spatial configuration of the waves interacting in such a resonator.
The authors present a quantum analysis of four-wave mixing in a non-resonant nonlinear medium inside a cavity which is driven by two driving fields. In this process a nonlinear medium couples two pump modes with a signal mode of the frequency equal to the half-sum of the two pump field frequencies. Three types of stable steady-state solutions of the deterministic problem, describing three regimes of oscillation, are found: one below threshold and two different above-threshold regimes. The spectra of fluctuations of the quadrature-phase amplitudes for all three modes are calculated. It is found that in the above-threshold regime each of three modes may display a squeezed noise reduction. Below threshold a squeezing is realized for the central mode.
The possibility of generating light in a squeezed quantum state during saturated light amplification in a semiconductor amplifier is theoretically analyzed. Due to four-wave mixing process during amplification, weak components of the spontaneous emission of the medium with symmetric frequency shifts relative to the strong amplified wave acquire the quantum properties of two-mode squeezed light. The squeezing of quadrature components occurs in the range of frequency shifts of several GHz (∼\sim∼ the inverse relaxation time of the charge carrier density) and can reach 10 dB or more under optimal conditions. The formation of a two-mode squeezing phase facilitates the observation of the squeezing effect, in which a strong wave, playing the role of a local wave, exhibits quadrature noise suppression without additional homodyne detection.
Squeezed states of the electromagnetic field have been generated by nondegenerate four-wave mixing due to Na atoms in an optical cavity. The optical noise in the cavity, comprised of primarily vacuum fluctuations and a small component of spontaneous emission from the pumped Na atoms, is amplified in one quadrature of the optical field and deamplified in the other quadrature. These quadrature components are measured with a balanced homodyne detector. The total noise level in the deamplified quadrature drops below the vacuum noise level.
Squeezed states of the electromagnetic field have been generated by nondegenerate four-wave mixing due to Na atoms in an optical cavity. The optical noise in the cavity, comprised of primarily vacuum fluctuations and a small component of spontaneous emission from the pumped Na atoms, is amplified in one quadrature of the optical field and deamplified in the other quadrature. These quadrature components are measured with a balanced homodyne detector. The total noise level in the deamplified quadrature drops below the vacuum noise level.
The dynamical behavior of Kerr optical frequency combs is very well understood today from the perspective of the semiclassical approximation. These combs are obtained by pumping an ultrahigh-QQQ whispering-gallery mode resonator with a continuous-wave laser. The long-lifetime photons are trapped within the toruslike eigenmodes of the resonator, where they interact nonlinearly via the Kerr effect. In this article, we use quantum Langevin equations to provide a theoretical understanding of the nonclassical behavior of these combs when pumped below and above threshold. In the configuration where the system is under threshold, the pump field is the unique oscillating mode inside the resonator, and it triggers the phenomenon of spontaneous four-wave mixing, where two photons from the pump are symmetrically up- and down-converted in the Fourier domain. This phenomenon, also referred to as parametric fluorescence, can only be understood and analyzed from a fully quantum perspective as a consequence of the coupling between the field of the central (pumped) mode and the vacuum fluctuations of the various side modes. We analytically calculate the power spectra of the spontaneous emission noise, and we show that these spectra can be either single- or double-peaked depending on the value of the laser frequency, chromatic dispersion, pump power, and spectral distance between the central mode and the side mode of interest. We also calculate as well the overall spontaneous noise power per side mode and propose simplified analytical expressions for some particular cases. In the configuration where the system is pumped above threshold, we investigate the phenomena of quantum correlations and multimode squeezed states of light that can occur in the Kerr frequency combs originating from stimulated four-wave mixing. We show that for all stationary spatiotemporal patterns, the side modes that are symmetrical relative to the pumped mode in the frequency domain display quantum correlations that can lead to squeezed states of light under some optimal conditions that are analytically determined. These quantum correlations can persist regardless the dynamical state of the system (rolls or solitons), regardless of the spectral extension of the comb (number side modes) and regardless of the dispersion regime (normal or anomalous). We also explicitly determine the phase quadratures leading to photon entanglement and analytically calculate their quantum-noise spectra. For both the below- and above-threshold cases, we study with particular emphasis the two principal architectures for Kerr comb generation, namely the add-through and add-drop configurations. It is found that regardless of the configuration, an essential parameter is the ratio between out-coupling and total losses, which plays a key role as it directly determines the efficiency of the detected fluorescence or squeezing spectra. We finally discuss the relevance of Kerr combs for quantum information systems at optical telecommunication wavelengths below and above threshold.
Given one oscillating mode in a laser or an optical bistability cavity, can other modes build up, that is, is single-mode operation unstable? The answer depends on an interplay of spontaneous emission, saturated gain, and four-wave mixing processes that permit one or more sidemodes both to be resonant with cavity modes and to have more gain than loss. We discuss this problem for cavities containing one- or two-photon two-level media subjected to a classical wave of arbitrary intensity and one or two weak quantized sidemodes. While a single sidemode may have gain, two sidemodes symmetrically placed about a strong pump mode can have greater gain due to four-wave mixing contributions sometimes called combination tones. The theory is valid for the buildup of sidemodes from quantum noise until the sidemodes begin to saturate. Subsequent dynamics including chaos must be handled by a theory that allows all modes to saturate. The same physical mechanisms are important in saturation spectroscopy and control the generation of squeezed states in a cavity. However while the instabilities depend on sidemode gain and spontaneous emission, the generation of squeezed states of the vacuum avoids these phenomena, depending solely on quantum combination tones.