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Optics Express

Squeezed state generation in photonic crystal microcavities

Mohamad G. Banaee, Jeff F. Young

Published Dec 3, 2008• 13 citations
Publisher

Abstract

The feasibility of using a parametric down-conversion process to generate squeezed electromagnetic states in three dimensional photonic crystal microcavity structures is investigated for the first time. The spectrum of the squeezed light is theoretically calculated by using an open cavity quantum mechanical formalism. The cavity communicates with two main channels, which model vertical radiation losses and coupling into a single-mode waveguide respectively. The amount of squeezing is determined by the correlation functions relating the field quadratures of light coupled into the waveguide. All of the relevant model parameters are realistically estimated for structures made in Al0.3Ga0.7As, using finite-difference time-domain simulations. Squeezing up to approximately 30% below the shot noise level is predicted for 10 mW average power, 80 MHz repetition, 500 ps excitation pulses using in a [111] oriented wafer.

DOI
10.1364/oe.16.020908

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The signal to noise ratio of optical systems is ultimately limited by the shot noise due to the Poissonian statistics of the light field. In recent years there has been a considerable effort to find ways to overcome this limitation by generating non-classical light with sub-shot noise statistics. Several groups have demonstrated non-classical light generation in diode lasers or light emitting diodes, and the amplitude fluctuations have been reduced substantially below the shot noise level [1,2]. However, for phase-sensitive measurements it is necessary to generate the more general quadrature squeezed states. Such quadrature squeezed light can be generated either by second-order or third-order nonlinear processes provided the nonlinear material has very low losses at the optical wavelength. To date, the successful generation schemes for quadrature squeezed light have been restricted to atomic vapours, optical fibres, or second-order nonlinear crystals [3]. The possibility of using the large χ(3) nonlinearities of semiconductors at frequencies below the band gap where the optical absorption is small has been discussed in the literature, but so far there have been no successful experiments [4-6]. In this paper we report measurements on GaAs/Al0.3Ga0.7As multiple quantum well waveguides and bulk ZnS in the wavelength range 750 - 890nm. Although we measure much larger nonlinearities in the quantum wells, the strong two-photon absorption is detrimental for squeezed light generation. However, in the ZnS where the laser frequency is below the two- photon absorption edge, we have succeeded in generating quadrature squeezed light in a semiconductor for the first time. On the basis of our results, we would expect that squeezed light could be generated in many other semiconductor systems provided the photon energy is less than half the band-gap energy.

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The feasibility of using a parametric down-conversion process to generate squeezed electromagnetic states in three dimensional photonic crystal microcavity structures is investigated for the first time. The spectrum of the squeezed light is theoretically calculated by using an open cavity quantum mechanical formalism. The cavity communicates with two main channels, which model vertical radiation losses and coupling into a single-mode waveguide respectively. The amount of squeezing is determined by the correlation functions relating the field quadratures of light coupled into the waveguide. All of the relevant model parameters are realistically estimated for structures made in Al0.3Ga0.7As, using finite-difference time-domain simulations. Squeezing up to approximately 30% below the shot noise level is predicted for 10 mW average power, 80 MHz repetition, 500 ps excitation pulses using in a [111] oriented wafer.
Nonlinear optical phenomena associated with high-order soliton breakup in photonic crystal fibres and squeezed state generation in three dimensional photonic crystal microcavities are investigated. In both cases, the properties of periodically patterned, high-index contrast dielectric structures are engineered to control the dispersion and local field enhancements of the electromagnetic field. Ultra-short pulse propagation in a polarization-maintaining microstructured fibre (with 1 um core diameter and 1.1 m length) is investigated experimentally and theoretically. For an 80 MHz train of 130 fs pulses with average propagating powers in the fibre up to 13.8 mW, the output spectra consist of multiple discrete solitons that shift continuously to lower energies as they propagate in the lowest transverse mode of the fibre. The number of solitons and the amount that they shift both increase with the launched power. All of the data is quantitatively consistent with solutions of the nonlinear Schrodinger equation, but only when the Raman nonlinearity is treated without approximation, and self-steepening is included. The feasibility of using a parametric down-conversion process to generate squeezed electromagnetic states in 3D photonic crystal microcavity structures is investigated for the first time. The spectrum of the squeezed light is theoretically calculated by using an open cavity quantum mechanical formalism. The cavity communicates with two main channels, which model vertical radiation losses and coupling into a single-mode waveguide respectively. The amount of squeezing is determined by the correlation functions relating the field quadratures of light coupled into the waveguide. All of the relevant model parameters are realistically estimated using 3D finite-difference time-domain (FDTD) simulations. Squeezing up to ~20% below the shot noise level is predicted for reasonable optical excitation levels. To preserve the squeezed nature of the light generated in the microcavity, a unidirectional coupling geometry from the microcavity to a ridge waveguide in a slab photonic crystal structure is studied. The structure was successfully fabricated in a silicon membrane, and experimental measurements of the efficiency for the signal coupled out of the structure are in good agreement with the result of FDTD simulations. The coupling efficiency of the cavity mode to the output channel is ~60%.
We have generated squeezed states of light by the process of second harmonic conversion within an optical cavity resonant at both fundamental and harmonic frequencies. The experiment consists of a standing-wave cavity containing a crystal of lithium niobate doped with magnesium oxide and driven by the field from a frequency-stabilized Nd:YAG laser (incident power, ~10 mW). The total field reflected from the cavity illuminates a pair of high quantum efficiency photodiodes, whose individual photocurrents are summed. Observations of squeezing are made by analyzing the spectral density of fluctuations for this sum photo-current while the cavity detuning is scanned through resonance. An intensity regulator holds the reflected light intensity constant during the scan by control of the incident light level. Reductions in photocurrent fluctuations of 12% relative to the vacuum-state or shot-noise level are achieved for frequency offsets near 4 MHz. Since significantly higher degrees of squeezing are predicted by our theoretical analysis, we discuss those processes that currently limit the observed noise reduction, including phase noise produced by the intracavity crystal in the absence of nonlinear conversion.
Entangled multi-mode squeezed states of light have a wide variety of applications in quantum information systems, particularly in the generation of non-Gaussian states of light, which are central to continuous-variable quantum computing. Although theoretical approaches exist to model the nonlinear generation of one- and two-mode entangled states of light in ring resonator systems, these approaches are difficult to implement in modeling more complicated many-cavity systems. In this work, we present an efficient and accurate theoretical approach to modeling the generation and propagation of quantum states of light in lossy coupled-cavity systems containing a two- or three-mode nonlinear resonant structure. Our approach is general and computationally viable even in systems with hundreds of modes. We apply our method to the design and modeling of a multimode photonic crystal coupled-cavity system for the generation of entangled squeezed states of light on-chip. The system consists of a three-mode resonant structure coupled to three coupled-resonator optical waveguides (CROWs) in a square lattice silicon photonic crystal slab. The computational speed of the method allows us to efficiently optimize the system such that the signal and idler light in the two output CROWs remains entangled even after propagating tens of cavities down the CROWs.
We investigate theoretically the temporal evolution of a squeezed state in lossy coupled-cavity systems. We present a general formalism based upon the tight-binding approximation and apply this to a two-cavity system as well as to a coupled-resonator optical waveguide in a photonic crystal. We derive analytical expressions for the number of photons and the quadrature noise in each cavity as a function of time when the initial excited state is a squeezed state in one of the cavities. We also analytically evaluate the time-dependent cross correlation between the photons in different cavities to evaluate the degree of quantum entanglement. We demonstrate that loss in such coupled-cavity systems cannot be treated using simple exponential factors. Finally, we also derive approximate analytic expressions for the maximum photon number, maximum squeezing, and maximum entanglement for cavities far from the initially excited cavity in a lossless coupled-resonator optical waveguide.
We analyze the quantum properties of the light generated by a three-level laser with an open cavity and coupled to a two-mode squeezed vacuum reservoir via a single-port mirror. The three-level laser consists of three-level atoms available in an open cavity and pumped from the bottom to the top level by means of electron bombardment. Applying the large-time approximation scheme, we have obtained the steady-state solutions of the equations of evolution for the expectation values of the atomic operators and the quantum Langevin equations for the cavity mode operators. Using the resulting steady-state solutions, we have calculated the mean photon number, the variance of the photon number, and the quadrature variance for the two-mode cavity light. We have seen that the light generated by the three-level laser is in a squeezed state and the squeezing occurs in the plus quadrature. It so turns out that the maximum quadrature squeezing of the two-mode cavity light is 45:68% for M0 = 0:59 and N0 = 0:27 below the vacuum-state level. In addition, we have shown that the effect of the squeezed parameter is to increase the mean and variance of the photon number.
The signal to noise ratio of optical systems is ultimately limited by the shot noise due to the Poissonian statistics of the light field. In recent years there has been a considerable effort to find ways to overcome this limitation by generating non-classical light with sub-shot noise statistics. Several groups have demonstrated non-classical light generation in diode lasers or light emitting diodes, and the amplitude fluctuations have been reduced substantially below the shot noise level [1,2]. However, for phase-sensitive measurements it is necessary to generate the more general quadrature squeezed states. Such quadrature squeezed light can be generated either by second-order or third-order nonlinear processes provided the nonlinear material has very low losses at the optical wavelength. To date, the successful generation schemes for quadrature squeezed light have been restricted to atomic vapours, optical fibres, or second-order nonlinear crystals [3]. The possibility of using the large χ(3) nonlinearities of semiconductors at frequencies below the band gap where the optical absorption is small has been discussed in the literature, but so far there have been no successful experiments [4-6]. In this paper we report measurements on GaAs/Al0.3Ga0.7As multiple quantum well waveguides and bulk ZnS in the wavelength range 750 - 890nm. Although we measure much larger nonlinearities in the quantum wells, the strong two-photon absorption is detrimental for squeezed light generation. However, in the ZnS where the laser frequency is below the two- photon absorption edge, we have succeeded in generating quadrature squeezed light in a semiconductor for the first time. On the basis of our results, we would expect that squeezed light could be generated in many other semiconductor systems provided the photon energy is less than half the band-gap energy.