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Proceedings of SPIE, the International Society for Optical Engineering/Proceedings of SPIE

Microscopic and macroscopic descriptions of electromagnetic-field propagation in nonlinear dispersive and absorbing media

V. L. Jacobs

Published Jan 13, 2012• 1 citation
Publisher

Abstract

Microscopic and macroscopic descriptions of electromagnetic-field propagation relevant to resonant pumpprobe optical phenomena, such as electromagnetically induced transparency, in quantized many-electron systems are formulated within the framework of a general reduced-density-matrix approach. Time-domain (equation-of-motion) and frequency-domain (resolvent-operator) formulations are developed in a unified and self-consistent manner. A semiclassical perturbation-theory treatment of the electromagnetic interaction is adopted, in which the electromagnetic field is described as a classical field satisfying either the microscopic form or the macroscopic form of the Maxwell equations. However, it is emphasized that a quantized-field approach is essential for a fully self-consistent quantummechanical formulation. Compact Liouville-space operator expressions are obtained for the linear and the general (n'th order) non-linear electromagnetic-response tensors for moving many-electron systems. These expressions can be evaluated for coherent initial electronic excitations and for the full tetradic-matrix form of the Liouville-space selfenergy operator in the Markov (short-memory-time) approximation. Environmental interactions can be treated in terms of the Liouville-space self-energy operator, and the influence of Zeeman coherences on electromagnetic-field propagation can be investigated by including an applied magnetic field together with the electromagnetic field.

DOI
10.1117/12.914734

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Physical Review A•Sep 24, 2014•6 citations
Microscopic and macroscopic descriptions of electromagnetic-field propagation relevant to resonant pumpprobe optical phenomena, such as electromagnetically induced transparency, in quantized many-electron systems are formulated within the framework of a general reduced-density-matrix approach. Time-domain (equation-of-motion) and frequency-domain (resolvent-operator) formulations are developed in a unified and self-consistent manner. A semiclassical perturbation-theory treatment of the electromagnetic interaction is adopted, in which the electromagnetic field is described as a classical field satisfying either the microscopic form or the macroscopic form of the Maxwell equations. However, it is emphasized that a quantized-field approach is essential for a fully self-consistent quantummechanical formulation. Compact Liouville-space operator expressions are obtained for the linear and the general (n'th order) non-linear electromagnetic-response tensors for moving many-electron systems. These expressions can be evaluated for coherent initial electronic excitations and for the full tetradic-matrix form of the Liouville-space selfenergy operator in the Markov (short-memory-time) approximation. Environmental interactions can be treated in terms of the Liouville-space self-energy operator, and the influence of Zeeman coherences on electromagnetic-field propagation can be investigated by including an applied magnetic field together with the electromagnetic field.
Non-linear interactions involving pump-probe optical phenomena, such as electromagnetically induced transparency, in quantized many-electron systems are investigated using a reduced-density-matrix approach. Time-domain (equation-of-motion) and frequency-domain (resolvent-operator) formulations are developed in a unified manner and self-consistent manner. The standard Born (lowest-order perturbation-theory) and Markov (short-memory-time) approximations are systematically introduced within the framework of the general non-perturbative and non-Markovian formulations. A preliminary semiclassical perturbation-theory treatment of the electromagnetic interaction is adopted. However, it is emphasized that a quantized-electromagnetic-field approach is essential for a self-consistent quantum-mechanical formulation. Our primary result is the derivation of compact Liouville-space operator expressions for the linear and the general (n'th order) non-linear macroscopic electromagnetic-response tensors for moving many-electron system. These expressions can be evaluated for coherent initial electronic excitations and for the full tetradic-matrix form of the Liouville-space self-energy operator representing the environmental interactions in the Markov approximation. Environmental interactions can be treated in various approximations for the self-energy operator, and the influence of Zeeman coherences on electromagnetic-field propagation can be investigated by including an applied magnetic field on an equal footing with the electromagnetic fields.
Linear and non-linear interactions in electromagnetically induced transparency and related pump-probe optical phenomena involving moving many-electron atomic systems are investigated using a reduced-density-matrix approach. Time-domain (equation-of-motion) and frequency-domain (resolvent-operator) formulations are developed in a unified manner. The standard Born (lowest-order perturbation-theory) and Markov (short-memory-time) approximations are systematically introduced within the framework of the general non-perturbative and non-Markovian formulations. A preliminary semiclassical perturbation-theory treatment of the electromagnetic interaction is adopted. However, it is emphasized that a quantized-electromagnetic-field approach is essential for a self-consistent quantum-mechanical formulation. Our primary result is the derivation of compact Liouville-space operator expressions for the linear and the general (n'th order) non-linear macroscopic electromagnetic-response tensors. These expressions can be evaluated for coherent initial atomic excitations and for the full tetradic-matrix form of the Liouville-space self-energy operator representing the environmental interactions in the Markov approximation. Collisional interactions between atoms can be treated in various approximations for the self-energy operator, and the influence of Zeeman coherences on the electromagnetic-pulse propagation can be investigated by including an applied magnetic field on an equal footing with the electromagnetic fields.
Classical, semi-classical, and quantum-field descriptions for the interaction of light with matter are systematically discussed. Applications of interest include precise determinations of the linear and the non-linear electromagnetic response relevant to resonant pump-probe optical phenomena, such as electromagnetically induced transparency. In the quantum-mechanical description of matter systems, we introduce a general reduced-density-matrix framework. Time-domain (equation-of-motion) and frequency-domain (resolvent-operator) formulations are developed in a unified and self-consistent manner, using a Liouville-space operator representation. A preliminary semi-classical perturbation treatment of the electromagnetic interaction is adopted, in which the electromagnetic field is described as a classical field satisfying the Maxwell equations. Compact Liouville-space operator expressions are derived for the linear and the general (nth order) non-linear electromagnetic-response tensors describing moving many-electron systems. The tetradic matrix elements of the Liouville-space self-energy operators, which are introduced in the time-domain and frequency-domain formulations, are evaluated for environmental collisional and radiative interactions, in order to provide explicit forms for the quantum kinetic equations and the spectral-line shape formulas. It is emphasized that a quantized-field approach is essential for a fully self-consistent quantum-mechanical description of the interacting light-matter system.
Reduced density matrix descriptions are developed for linear and non-linear interactions in electromagnetically induced transparency and related pump-probe optical phenomena involving moving atomic systems. Applied magnetic fields as well as atomic collisions, together with other environmental decoherence and relaxation processes, are taken into account. Time-domain (equation-of-motion) and frequency-domain (resolvent-operator) formulations are developed in a unified manner. The standard Born (lowest-order perturbation-theory) and Markov (short-memory-time) approximations are systematically introduced within the framework of the general non-perturbative and non-Markovian formulations. A preliminary semiclassical treatment of the electromagnetic interaction is adopted. However, the need for a fully quantum mechanical approach is emphasized. Compact Liouville-space operator expressions are derived for the linear and the general (n'th order) non-linear macroscopic electromagnetic-response tensors within the framework of a perturbation-theory treatment of the semiclassical electromagnetic interaction. These expressions can be evaluated for coherent initial atomic excitations and for the full tetradic-matrix form of the Liouville-space self-energy operator representing the environmental interactions in the Markov approximation. Collisional interactions between atoms can be treated in various approximations for the self-energy operator, and the influence of Zeeman coherences on the electromagnetic-pulse propagation can be investigated.
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Linear and nonlinear (especially coherent) electromagnetic interactions of moving many-electron atoms are investigated using a reduced-density-matrix description, which is applied to electromagnetically induced transparency and related resonant pump-probe optical phenomena. External magnetic fields are included on an equal footing with the electromagnetic fields and spin-Zeeman interactions are taken into account. Complimentary time-domain (equation-of-motion) and frequency-domain (resolvent-operator) formulations of the reduced-density-matrix description are self-consistently developed. The general nonperturbative and non-Markovian formulations provide a fundamental framework for systematic evaluations of corrections to the standard Born (lowest-order-perturbation) and Markov (short-memory-time) approximations. The macroscopic electromagnetic response is described semiclassically, employing a perturbation expansion of the reduced-density operator in powers of the classical electromagnetic field. Our primary results are compact Liouville-space operator expressions for the linear and general (nthn\text{th}nth-order) nonlinear macroscopic electromagnetic-response tensors, which can be evaluated for nonlocal and nonstationary optical media described by multilevel atomic-system representations. Interactions among atoms and with environmental photons are treated as line-broadening effects by means of a general Liouville-space self-energy operator, for which the tetradic-matrix elements are explicitly evaluated in the diagonal, lowest-order, and Markov approximations. The compact Liouville-space operator expressions that are derived for the macroscopic electromagnetic-response tensors are introduced into the dynamical description of the electromagnetic-field propagation. It is pointed out that a quantized-electromagnetic-field approach will be required for a fully self-consistent quantum-mechanical treatment of local-field effects and radiative corrections.